English

Dipolar Interactions and Origin of Spin Ice in Ising Pyrochlore Magnets

Disordered Systems and Neural Networks 2009-10-31 v1

Abstract

Recent experiments suggest that the Ising pyrochlore magnets Ho2Ti2O7{\rm Ho_{2}Ti_{2}O_{7}} and Dy2Ti2O7{\rm Dy_{2}Ti_{2}O_{7}} display qualitative properties of the spin ice model proposed by Harris {\it et al.} \prl {\bf 79}, 2554 (1997). We discuss the dipolar energy scale present in both these materials and consider how they can display spin ice behavior {\it despite} the presence of long range interactions. Specifically, we present numerical simulations and a mean field analysis of pyrochlore Ising systems in the presence of nearest neighbor exchange and long range dipolar interactions. We find that two possible phases can occur, a long range ordered antiferromagnetic one and the other dominated by spin ice features. Our quantitative theory is in very good agreement with experimental data on both Ho2Ti2O7{\rm Ho_{2}Ti_{2}O_{7}} and Dy2Ti2O7{\rm Dy_{2}Ti_{2}O_{7}}. We suggest that the nearest neighbor exchange in Dy2Ti2O7{\rm Dy_{2}Ti_{2}O_{7}} is {\it antiferromagnetic} and that spin ice behavior is induced by long range dipolar interactions.

Keywords

Cite

@article{arxiv.cond-mat/0001369,
  title  = {Dipolar Interactions and Origin of Spin Ice in Ising Pyrochlore Magnets},
  author = {Byron C. den Hertog and Michel J. P. Gingras},
  journal= {arXiv preprint arXiv:cond-mat/0001369},
  year   = {2009}
}

Comments

4 postscript figures included. Submitted to Physical Review Letters Contact: [email protected]