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Neutron scattering has played a significant role in characterizing magnetic and structural correlations in Fe$_{1+y}$Te$_{1-x}$Se$_x$ and their connections with superconductivity. Here we review several key aspects of the physics of iron…

Superconductivity · Physics 2020-08-26 J. M. Tranquada , Guangyong Xu , I. A. Zaliznyak

By applying density functional theory, we find strong evidence for an itinerant nature of magnetism in two families of iron pnictides. Furthermore, by employing dynamical mean field theory with continuous time quantum Monte Carlo as an…

Strongly Correlated Electrons · Physics 2011-05-12 Yu-Zhong Zhang , Hunpyo Lee , Ingo Opahle , Harald O. Jeschke , Roser Valenti

Recent inelastic neutron scattering (INS) measurements on FeSe and Fe(Te$_{1-x}$Se$_x$), have sparked intense debate over the nature of the ground state in these materials. Here we propose an effective bilinear-biquadratic spin model which…

Strongly Correlated Electrons · Physics 2017-11-09 Patricia Bilbao Ergueta , Wen-Jun Hu , Andriy H. Nevidomskyy

In this paper, we address a number of outstanding issues concerning the nature and the role of magnetic inhomogenities in the iron chalcogenide system FeTe1-xSex and their correlation with superconductivity in this system. We report…

Using a first-principles Green's function approach we study magnetic properties of the magnetic binary chalcogenides Bi2Te3, Bi2Se3, and Sb2Te3. The magnetic coupling between transition-metal impurities is long-range, extends beyond a…

Using neutron inelastic scattering, we investigate the role of interstitial iron on the low-energy spin fluctuations in powder samples of Fe_{1+x}Te_{0.7}Se_{0.3}. We demonstrate how combining the principle of detailed balance along with…

Superconductivity · Physics 2015-06-04 C. Stock , E. E. Rodriguez , M. A. Green

Cr$_{1+\delta}$Te$_2$, a two-dimensional van der Waals ferromagnet, displays a contested magnetic structure, poised between collinear and non-collinear spin configurations. In this work, we investigate the magnetic structure of…

We present a systematic study of the nematic fluctuations in the iron chalcogenide superconductor Fe$_{1+y}$Te$_{1-x}$Se$_{x}$ ($0 \leq x \leq 0.53$) using the elastoresistivity technique. Near $x = 0$, in proximity to the double-stripe…

The Fe intercalated transition metal dichalcogenide (TMD), Fe$_{1/3}$NbS$_2$, exhibits remarkable resistance switching properties and highly tunable spin ordering phases due to magnetic defects. We conduct synchrotron X-ray scattering…

We present the magnetic behavior and resulting transport properties of TaSe$_2$ when intercalated by magnetically active cobalt cations. Acting as the layered host, TaSe$_2$ is a transition metal dichalcogenide (TMD) that adopts the…

Iron chalcogenides display a rich variety of electronic orders in their phase diagram. A particularly enigmatic case is FeTe, a metal which possesses co-existing hole and electron Fermi surfaces as in the iron pnictides but has a distinct…

Strongly Correlated Electrons · Physics 2016-08-30 Hsin-Hua Lai , Shou-Shu Gong , Wen-Jun Hu , Qimiao Si

The complex interdigitated phases have greatly frustrated attempts to document the basic features of the superconductivity in the alkali metal intercalated iron chalcogenides. Here, using elastic neutron scattering, energy-dispersive x-ray…

Superconductivity · Physics 2016-03-09 Meng Wang , Ming Yi , Wei Tian , Edith Bourret-Courchesne , Robert J. Birgeneau

We show that the magnetic and vacancy orders in the 122 $(A_{1-y}Fe_{2-x}Se_2)$ iron-chalcogenides can be naturally derived from the $J_1-J_2-J_3$ model with $J_1$ being the ferromagnetic (FM) nearest neighbor exchange coupling and $J_{2},…

Strongly Correlated Electrons · Physics 2012-04-05 Chen Fang , Bao Xu , Pengcheng Dai , Tao Xiang , Jiangping Hu

The phase diagram of the iron arsenides is dominated by a magnetic and a structural phase transition, which need to be suppressed in order for superconductivity to appear. The proximity between the two transition temperature lines indicates…

Superconductivity · Physics 2013-09-27 R. M. Fernandes , A. E. Böhmer , C. Meingast , J. Schmalian

Motivated by the properties of the iron chalcogenides, we study the phase diagram of a generalized Heisenberg model with frustrated bilinear-biquadratic interactions on a square lattice. We identify zero-temperature phases with…

Strongly Correlated Electrons · Physics 2015-09-10 Rong Yu , Qimiao Si

It is assessed in detail both experimentally and theoretically how the interlayer coupling of transition metal dichalcogenides controls the electronic properties of the respective devices. Gated transition metal dichalcogenide structures…

Mackinawite is a naturally-occurring layer type FeS mineral well-known to be important in biogeochemical cycles and, more recently, to the development of microbial fuel cells. Conflicting results have been published as to the magnetic…

Superconductivity · Physics 2011-02-11 Kideok D. Kwon , Keith Refson , Sharon Bone , Ruimin Qiao , Wan-li Yang , Zhi Liu , Garrison Sposito

The level of electronic correlation has been one of the key questions in understanding the nature of superconductivity. Among the iron-based superconductors, the iron chalcogenide family exhibits the strongest electron correlations. To…

Iron-chalcogenide compounds with FeSe(Te, S) layers did not attract much attention until the discovery of high-Tc superconductivity (SC) in the iron-pnictide compounds at the begining of 2008. Compared with FeAs-based superconductors,…

Superconductivity · Physics 2015-06-16 ChiHeng Dong , Hangdong Wang , Minghu Fang

We report on the magnetic properties of the supra-molecular compound iron(II) phthalocyanine in its alpha-form. dc- and ac-susceptometry measurements and Mossbauer experiments show that the iron atoms are strongly magnetically coupled into…

Condensed Matter · Physics 2007-05-23 M. Evangelisti , J. Bartolome , L. J. de Jongh , G. Filoti