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We demonstrate a pump-probe scheme in which an atomic vapor is optically pumped with circularly polarized light and probed with a vector vortex beam. The pump induces a macroscopic magnetization in the medium, which gives rise to…
Rapidly developing science and technology demand new materials with versatile and promising properties for practical applications. In this context, pseudo-octahedral iron(II) spin crossover (SCO) complexes are particularly appealing - not…
Molecules with heavy, radioactive nuclei promise extreme sensitivity to fundamental nuclear and particle physics. However, these nuclei are available in limited quantities, which challenges their use in precision measurements. Here we…
The recoil optical force that acts on emitters near a surface or waveguide relies on near-field directionality and conservation of momentum. It features desirable properties uncommon in optical forces, such as the ability to produce it via…
We demonstrate and characterize a cryogenic buffer gas-cooled molecular beam source capable of producing bright beams of free radicals and refractory species. Details of the beam properties (brightness, forward velocity distribution,…
In this paper, we analyze electric deflection fields for polar molecules in terms of a multipole expansion and derive a simple but rather insightful expression for the force on the molecules. Ideally, a deflection field exerts a strong,…
We describe theoretically the resonant optical excitation of a trion with circularly polarized light and discuss how this trion permits the read-out of a single electron spin through a recycling transition. Optical pumping through…
Photons carry one unit of angular momentum associated with their spin~\cite{Beth1936}. Structured vortex beams carry additional orbital angular momentum which can also be transferred to matter~\cite{Allen1992}. This extra twist has been…
As a heavy molecule, barium monofluoride (BaF) presents itself as a promising candidate for measuring permanent electric dipole moment. The precision of such measurements can be significantly enhanced by utilizing a cold molecular sample.…
We observe clear precessional motion of highly birefringent liquid crystal (LC) particles trapped in a spherically aberrated optical trap which is built around a tilted refractive index stratified medium. For input circularly polarized…
The transport of relativistic electrons generated in the interaction of petawatt class lasers with solid targets has been studied through measurements of the optical emission from their rear surface. The high degree of polarization of the…
We investigate the recoil heating phenomenon experienced by a dielectric spherical particle when it interacts with a linearly polarized plane wave within the Rayleigh regime. We derive the fluctuating force acted upon the particle arising…
We have recently demonstrated that optical pumping methods combined with photoassociation of ultra-cold atoms can produce ultra-cold and dense samples of molecules in their absolute rovibronic ground state. More generally, both the external…
Non-invasive optical manipulation of particles has emerged as a powerful and versatile tool for biological study and nanotechnology. In particular, trapping and rotation of cells, cell nuclei and sub-micron particles enables unique…
We report optical trapping of laser-cooled molecules at sufficient density to observe molecule-molecule collisions for the first time in a bulk gas. SrF molecules from a red-detuned magneto-optical trap (MOT) are compressed and cooled in a…
We analyze the ponderomotive action experienced by a small spherical particle immersed in an optical field, in relation to the internal energy flows (optical currents) and their spin and orbital constituents. The problem is studied…
A novel deflection effect of an intense laser beam with spin angular momentum is revealed theoretically by an analytical modeling using radiation pressure and momentum balance of laser plasma interaction in the relativistic regime, as a…
We investigate optical forces on oscillating dipoles close to a phase-change vanadium dioxide (VO$_2$) film, which exhibits a metal-insulator transition around $340$ K and low thermal hysteresis. This configuration is related to one…
We propose that a radiative cycle operates in atoms (ions) located in a rarefied gas in the vicinity of a hot star. Besides spontaneous transitions the cycle includes a stimulated transition in one very weak intermediate channel. This…
We demonstrate sub-Doppler laser cooling and magneto-optical trapping of the rare earth element Holmium. Atoms are loaded from an atomic beam source and captured in six-beam $\sigma_+ - \sigma_-$ molasses using a strong $J=15/2…