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Optical forces allow manipulation of small particles and control of nanophotonic structures with light beams. Here, we describe a counter-intuitive lateral optical force acting on particles placed above a substrate, under uniform plane wave…
Barium monohydride (BaH) is an attractive candidate for extending laser cooling and trapping techniques to diatomic hydrides. The apparatus and high-resolution optical spectroscopy presented here demonstrate progress toward this goal. A…
We report on rotating an optically trapped silica nanoparticle in vacuum by transferring spin angular momentum of light to the particle's mechanical angular momentum. At sufficiently low damping, realized at pressures below $10^{-5}$ mbar,…
By analyzing the parameters of electronic transitions, we show how bosonic Sr atoms in planar optical lattices can be engineered to exhibit optical magnetism and other higher-order electromagnetic multipoles that can be harnessed for…
We consider deflection of polarizable molecules by inhomogeneous optical fields, and analyze the role of molecular orientation and rotation in the scattering process. It is shown that molecular rotation induces spectacular rainbow-like…
We report a series of experimental, analytical and numerical studies demonstrating strong circular dichroism in helically twisted hollow-core single-ring photonic crystal fiber (SR-PCF), formed by spinning the preform during fiber drawing.…
Cooling the rotation and the vibration of molecules by broadband light sources was possible for trapped molecular ions or ultracold molecules. Because of a low power spectral density, the cooling timescale has never fell below than a few…
Optically coupled nanoparticles suffer the action of multiple electromagnetic forces when they are illuminated by light. In general, two kinds of forces are commonly assumed: binding forces that make them attract/repel each other and…
Detecting the internal state of polar molecules is a substantial challenge when standard techniques such as resonance-enhanced multi photon ionization (REMPI) or laser-induced fluorescense (LIF) do not work. As this is the case for most…
Iron complexes with a suitable ligand field undergo spin-crossover (SCO), which can be induced reversibly by temperature, pressure or even light. Therefore, these compounds are highly interesting candidates for optical information storage,…
We consider deflection of polarizable molecules by inhomogeneous optical fields, and analyze the role of molecular orientation and rotation in the scattering process. It is shown that molecular rotation induces spectacular rainbow-like…
We report direct laser cooling of a symmetric top molecule, reducing the transverse temperature of a beam of calcium monomethoxide (CaOCH$_3$) to $1.8\pm0.7$ mK while addressing two distinct nuclear spin isomers. These results open a path…
We propose a general method to cool the translational motion of molecules. Our method is an extension of single photon atomic cooling which was successfully implemented in our laboratory. Requiring a single event of absorption followed by a…
Single-cycle optical pulses with a controlled electromagnetic waveform allow to steer the motion of low-energy electrons in atoms, molecules, nanostructures or condensed-matter on attosecond dimensions in time. However, high-energy…
Polariton formalism is applied for studying the propagation of a probe field of light in a cloud of cold atoms influenced by two control laser beams of larger intensity. The laser beams couple resonantly three hyperfine atomic ground states…
The helium dimer in its metastable triplet state is a promising candidate to be the first laser-cooled homonuclear molecule. An ultracold gas of He$_2^*$ would enable a new generation of precision measurements to test quantum…
In this paper, we present experimental evidence of a newly discovered third-order nonlinear optical process Self-Induced Spin-to-Orbital Conversion (SISTOC) of the photon angular momentum. This effect is the physical mechanism at the origin…
We consider the use of pulse-shaped broadband femtosecond lasers to optically cool rotational and vibrational degrees of freedom of molecules. Since this approach relies on cooling rotational and vibrational quanta by exciting an electronic…
We derive the force of the electromagnetic radiation on material objects by a direct application of the Lorentz law of classical electro-dynamics. The derivation is straightforward in the case of solid metals and solid dielectrics, where…
The traversal of an elliptically polarized optical field through a thermal vapour cell can give rise to a rotation of its polarization axis. This process, known as polarization self-rotation (PSR), has been suggested as a mechanism for…