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One of the most promising applications in nanoscience is the design of new materials to improve water permeability and selectivity of nanoporous membranes. Understanding the molecular architecture behind these fascinating structures and how…

Soft Condensed Matter · Physics 2021-09-10 João P. K. Abal , Rodrigo F. Dillenburg , Mateus H. Köhler , Marcia C. Barbosa

This work describes the behaviour of water molecules in 1-butyl-3-methylimidazolium tetrafluoroborate ionic liquid under nanoconfinement between graphene sheets. By means of molecular dynamics simulations, an adsorption of water molecules…

A comprehensive phase diagram of lowest-energy structures and compositions of the rutile TiO_2(110) surface in equilibrium with a surrounding gas phase at finite temperatures and pressures has been determined using density functional theory…

Materials Science · Physics 2009-11-13 Piotr M. Kowalski , Bernd Meyer , Dominik Marx

We use ab initio simulations to study the static and dynamic properties of a sodium borosilicate liquid with composition 3Na_2O-B_2O_3-6SiO_2, i.e. a system that is the basis of many glass-forming materials. In particular we focus on the…

Disordered Systems and Neural Networks · Physics 2018-02-28 Laurent Pedesseau , Simona Ispas , Walter Kob

Tungsten and cobalt carbonyls adsorbed on a substrate are typical starting points for the electron beam induced deposition of tungsten or cobalt based metallic nanostructures. We employ first principles molecular dynamics simulations to…

Materials Science · Physics 2015-06-16 Kaliappan Muthukumar , Roser Valenti , Harald O. Jeschke

Electronic and dielectric properties of vapor-phase grown MoS_{2} have been investigated in metal/MoS_{2}/silicon capacitor structures by capacitance-voltage and conductancevoltage techniques. Analytical methods confirm the MoS_{2} layered…

Materials Science · Physics 2019-07-19 M. Belete , S. Kataria , U. Koch , M. Kruth , C. Engelhard , J. Mayer , O. Engström , M. C. Lemme

The structures and energetics of organic molecules adsorbed onto clean and H-passivated Si(001)-(2$\times$1) surfaces have been calculated using density functional theory. For benzene adsorbed on the clean Si surface the tight-bridge…

Materials Science · Physics 2009-11-13 Karen Johnston , Risto M. Nieminen

We experimentally study steady Marangoni-driven surfactant transport on the interface of a deep water layer. Using hydrodynamic measurements, and without using any knowledge of the surfactant physico-chemical properties, we show that sodium…

Fluid Dynamics · Physics 2018-02-06 S. Mandre , V. S. Akella , D. K. Singh , R. S. Singh , M. M. Bandi

We investigate the aggregation of amphiphilic molecules by adapting the two-state Muller-Lee-Graziano model for water, in which a solvent-induced hydrophobic interaction is included implicitly. We study the formation of various types of…

Statistical Mechanics · Physics 2009-11-10 S. Moelbert , B. Normand , P. De Los Rios

Although medium chain length insoluble amphiphiles are well known to form gaseous and liquid expanded phases on an air/water interface, the situation for the soluble case is less clear. We perform molecular dynamics simulations of model…

Soft Condensed Matter · Physics 2007-05-23 M. S. Tomassone , A. Couzis , C. Maldarelli , J. R. Banavar , J. Koplik

The interaction of tungsten hexacarbonyl W(CO)$_6$ precursor molecules with SiO$_2$ substrates is investigated by means of density functional theory calculations with and without inclusion of long range van der Waals interactions. We…

Materials Science · Physics 2016-08-14 Kaliappan Muthukumar , Ingo Opahle , Juan Shen , Harald O. Jeschke , Roser Valentí

The mobility of water molecules confined in a silica pore is studied by computer simulation in the low hydration regime, where most of the molecules reside close to the hydrophilic substrate. A layer analysis of the single particle dynamics…

Statistical Mechanics · Physics 2009-11-10 P. Gallo , M. Rovere

We study numerically and experimentally the breakup of a pendant droplet loaded with a soluble surfactant. We consider the limit in which surfactant sorption is limited only by diffusion. Surfactant transfer toward the interface is enhanced…

Fluid Dynamics · Physics 2026-05-06 M. Rubio , S. Rodríguez-Aparicio , J. M. Montanero , M. A. Herrada

The adsorption of mixtures of poly(diallyldimethylammonium chloride) (PDADMAC) and sodium N-lauroyl-N-methyltaurate (SLMT) at the water / vapor interface has been studied using drop profile tensiometry and neutron reflectometry. This study…

Ion hydration and interfacial water play crucial roles in numerous phenomena ranging from biological to industrial systems. Although biologically relevant (and mostly smaller) ions have been studied extensively in this context, very little…

Soft Condensed Matter · Physics 2019-01-01 William Rock , Baofu Qiao , Tiecheng Zhou , Aurora E. Clark , Ahmet Uysal

First principle computer simulations of a thin parahydrogen film adsorbed on a silica substrate at low temperature (below 6 K) yield no evidence that the top layer is liquid and/or in the proximity of a superfluid transition, as claimed in…

Statistical Mechanics · Physics 2021-02-02 Massimo Boninsegni

Many ionic surfactants, such as sodium dodecyl sulphate (SDS) crystallize out of solution if the temperature falls below the crystallization boundary. The crystallization temperature is impacted by solution properties, and can be decreased…

By means of density, dielectric spectroscopy and sound velocity measurements we perform a systematic study on the polyoxyethylene $C_{12}E_{6}$ nonionic surfactant solutions as a function of temperature and concentration. Both density and…

Chemical Physics · Physics 2007-05-23 Luca Falconi , Marco Maccarini , Giuseppe Briganti , Giovanni D'Arrigo

The structure of an adsorption octadecanamide film at the planar toluene-water interface is studied by X-ray reflectometry using synchrotron radiation with photon energy of 15 keV. The electron density (polarizability) profiles, according…

Soft Condensed Matter · Physics 2020-04-22 Aleksey M. Tikhonov , Yurii O. Volkov

Pulmonary surfactant forms a sub-micrometer thick fluid layer that covers the surface of alveolar lumen and inhaled nanoparticles therefore come in to contact with surfactant prior to any interaction with epithelial cells. We investigate…

Soft Condensed Matter · Physics 2021-09-21 M. Radiom , M. Sarkis , O. Brookes , E. K. Oikonomou , A. Baeza-Squiban , J. -F. Berret