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We observe ultralong-range blue-shifted Cs$_{2}$ molecular states near $ns_{1/2}$ Rydberg states in an optical dipole trap, where $31\leq n\leq34$. The accidental near degeneracy of $(n-4)l$ and $ns$ Rydberg states for $l>2$ in Cs, due to…
Rydberg atoms are remarkable tools for quantum simulation and computation. They are the focus of an intense experimental activity mainly based on low-angular-momentum Rydberg states. Unfortunately, atomic motion and levels lifetime limit…
Strong interactions can amplify quantum effects such that they become important on macroscopic scales. Controlling these coherently on a single particle level is essential for the tailored preparation of strongly correlated quantum systems…
Here, we explore the combination of sub-wavelength, two-dimensional atomic arrays and Rydberg interactions as a powerful platform to realize strong, coherent interactions between individual photons with high fidelity. In particular, the…
Rydberg states of atoms are of great current interest for quantum manipulation of mesoscopic samples of atoms. Long-range Rydberg-Rydberg interactions can inhibit multiple excitations of atoms under the appropriate conditions. These…
We observe long-range $^{85}$Rb and $^{87}$Rb (24$D$+5$S_{1/2}$) Rydberg molecules for eight different spin couplings, with binding energies up to 440~MHz and sub-percent relative uncertainty. Isotopic effects of the molecular binding…
We study a general problem of the translational/rotational/vibrational/electronic dynamics of a diatomic molecule exposed to an interaction with an arbitrary external electromagnetic field. The theory developed in this paper is relevant to…
The ability to generate and control strong long-range interactions via highly excited electronic states has been the foundation for recent breakthroughs in a host of areas, from atomic and molecular physics [1, 2] to quantum optics [3, 4]…
A theory of Rydberg atom interactions is used to derive analytical forms for the spin wave pair correlation function in laser-excited cold-atom vapors. This function controls the quantum statistics of light emission from dense,…
This paper reviews recent advances in the study of strongly interacting systems of dipolar molecules. Heteronuclear molecules feature large and tunable electric dipole moments, which give rise to long-range and anisotropic dipole-dipole…
We examine interactions between atoms continuously and coherently driven between the ground state and a Rydberg state, producing "Rydberg-dressed atoms." Because of the large dipolar coupling between two Rydberg atoms, a small admixture of…
The dipole-dipole interaction among ultra-cold Rydberg atoms is simulated. We examine a general interaction scheme in which two atoms excited to the x and x' states are converted to y and y' states via a Forster resonance. The atoms are…
We propose to sympathetically slow and cool polar molecules in a cold, low-density beam using laser-cooled Rydberg atoms. The elastic collision cross sections between molecules and Rydberg atoms are large enough to efficiently thermalize…
We have experimentally demonstrated both heating and cooling of electrons in an ultracold neutral plasma (UNP) by embedding Rydberg atoms into the plasma soon after its creation. We have determined the relationship between the initial…
We report on the observation of the scissors mode of a single dipolar quantum droplet. The existence of this mode is due to the breaking of the rotational symmetry by the dipole-dipole interaction, which is fixed along an external…
We propose a novel scheme to efficiently tune the scattering length of two colliding ground-state atoms by off-resonantly coupling the scattering-state to an excited Rydberg-molecular state using laser light. For the s-wave scattering of…
Devices capable of deterministically manipulating the photonic entanglement are of paramount importance, since photons are the ideal messengers for quantum information. Here, we report a Rydberg-atom-based entanglement filter that preserves…
The lifetimes and decay channels of ultralong-range Rydberg molecules created in a dense BEC are examined by monitoring the time evolution of the Rydberg population using field ionization. Studies of molecules with values of principal…
The quest to realize topological band structures in artificial matter is strongly focused on lattice systems, and only quantum Hall physics is known to appear naturally also in the continuum. In this letter, we present a proposal based on a…
Rydberg-atom ensembles are switched from a weakly- into a strongly-interacting regime via adiabatic transformation of the atoms from an approximately non-polar into a highly dipolar quantum state. The resultant electric dipole-dipole forces…