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The description of molecular motion by macroscopic hydrodynamics has a long and continuing history. The Stokes-Einstein relation between the diffusion coefficient of a solute and the solvent viscosity predicted using macroscopic continuum…

Disordered Systems and Neural Networks · Physics 2007-05-23 Xiaoyu Xia , Peter G. Wolynes

The diffusivity of tagged particles is demonstrated to be heterogeneous on time scales comparable to or less than the structural relaxation time %taking place at the interparticle distance in a highly supercooled liquid via 3D molecular…

Soft Condensed Matter · Physics 2009-10-31 Ryoichi Yamamoto , Akira Onuki

The diffusivity of tagged particles is demonstrated to be very heterogeneous on time scales comparable to or shorter than the $\alpha$ relaxation time $\tau_{\alpha}$ ($\cong$ the stress relaxation time) in a highly supercooled liquid via…

Soft Condensed Matter · Physics 2009-10-31 Ryoichi Yamamoto , Akira Onuki

It is widely believed that the breakdown of the Stokes-Einstein (SE) relation between the translational diffusivity and the shear viscosity in supercooled liquids is due to the development of dynamic heterogeneity i.e. the presence of both…

Statistical Mechanics · Physics 2015-06-12 Shiladitya Sengupta , Smarajit Karmakar

A simple model for viscous liquid dynamics is introduced. Consider the surface of the union of hyper-spheres centered at random positions inside a hypercube with periodic boundary conditions. It is argued and demonstrated by numerical…

Soft Condensed Matter · Physics 2022-06-08 Filip Samuelsen , Lorenzo Costigliola , Thomas B. Schrøder

The mean-squared displacement (MSD) of a hard sphere and of a dumbbell molecule consisting of two fused hard spheres immersed in a dense hard-sphere system is calculated within the mode-coupling theory for ideal liquid-glass transitions. It…

Soft Condensed Matter · Physics 2009-11-07 S. -H. Chong , W. Gotze , M. R. Mayr

The interplay between self-diffusion and excitation lines in space-time was recently studied in kinetically constrained models to explain the breakdown of the Stokes-Einstein law in supercooled liquids. Here, we further examine this…

Statistical Mechanics · Physics 2009-11-10 Ludovic Berthier , David Chandler , Juan P. Garrahan

We investigate the origin of the Stokes-Einstein relation in liquids. The hard-sphere dynamics is analyzed using a new measure of structural relaxation - the minimum Euclidean distance between configurations of particles. It is shown that…

Soft Condensed Matter · Physics 2007-05-23 Tomas Oppelstrup , Babak Sadigh , Srikanth Sastry , Mikhail Dzugutov

We study the mean-square displacement (MSD) of a tracer particle diffusing in a granular gas of inelastic hard spheres under homogeneous cooling state (HCS). Tracer and granular gas particles are in general mechanically different. Our…

Statistical Mechanics · Physics 2026-01-29 Santos Bravo Yuste , Rubén Gómez González , Vicente Garzó

State-of-the-art techniques for simulating deeply supercooled liquids require a high degree of size polydispersity to be effective. While these techniques have enabled great insight into the microscopic dynamics near the glass transition,…

Soft Condensed Matter · Physics 2023-08-10 Ilian Pihlajamaa , Corentin C. L. Laudicina , Liesbeth M. C. Janssen

The mean square displacement and instantaneous diffusion coefficient for different configurations of charged particles in stochastic motion are calculated by numerically solving the associated equations of motion. The method is suitable for…

Statistical Mechanics · Physics 2019-06-26 Gabriela Raluca Mocanu

Recent advances in light microscopy have spawned new research frontiers in microbiology by working around the diffraction barrier and allowing for the observation of nanometric biological structures. Microrheology is the study of the…

Probability · Mathematics 2016-07-27 Gustavo Didier , Kui Zhang

Non-Gaussian nature of the probability distribution of particles' displacements in the supercooled temperature regime in glass-forming liquids are believed to be one of the major hallmarks of glass transition. It is already been established…

Statistical Mechanics · Physics 2018-08-29 Bhanu Prasad Bhowmik , Indrajit Tah , Smarajit Karmakar

The mean square displacement $\langle\left(x(t)-x(0)\right)^2\rangle$ of the position $x$ of a free particle of mass $m$ at thermal equilibrium is evaluated quantum mechanically. An analytical expression is obtained which shows an initial…

Quantum Physics · Physics 2021-12-22 Roberto Marquardt

The mean square displacement per collision of a molecule immersed in a gas at equilibrium is given by its mean square displacement between two consecutive collisions (mean square free path) corrected by a prefactor in the form of a series.…

Soft Condensed Matter · Physics 2024-07-03 Santos Bravo Yuste , Rubén Gómez González , Vicente Garzó

We study the transport and the relaxation properties of a molecular supercooled liquid by molecular-dynamics numerical simulations. The focus is on the translational motion. Jump motion is detected. At lower temperature the Stokes-Einstein…

Statistical Mechanics · Physics 2007-05-23 Cristiano De Michele , Dino Leporini

The recently discovered scaling law for the relaxation times, tau=f(T,V^g), where T is temperature and V the specific volume, is derived by a revision of the entropy model of the glass transition dynamics originally proposed by Avramov [I.…

Soft Condensed Matter · Physics 2009-11-11 R. Casalini , U. Mohanty , C. M. Roland

Fundamental thermodynamics and an earlier elastic solid-state point defect model [P. Varotsos and K. Alexopoulos, Phys. Rev B 15, 4111 (1977); 18, 2683 (1978)] are employed to formulate an analytical second-order polynomial function…

Soft Condensed Matter · Physics 2009-03-31 A. N. Papathanassiou

Diffusive scaling of position moments and a central limit theorem are obtained for the mean position of a quantum particle hopping on a cubic lattice and subject to a random potential consisting of a large static part and a small part that…

Mathematical Physics · Physics 2015-12-11 Jeffrey Schenker

It was recently shown that the real part of the frequency-dependent fluidity for several glass-forming liquids of different chemistry conforms to the prediction of the random barrier model (RBM) devised for ac electrical conduction in…

Soft Condensed Matter · Physics 2020-04-10 Thomas B. Schrøder , Jeppe C. Dyre
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