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Nuclear spin hyperpolarization enables real-time observation of metabolism and intermolecular interactions in vivo. 1-13C-Pyruvate is the leading hyperpolarized tracer currently under evaluation in several clinical trials as a promising…

Nitrogen vacancy (NV-) color centers in diamond are a prime candidate for use in quantum information devices, owing to their spin-1 ground state, straightforward optical initialization and readout, and long intrinsic coherence times in a…

Quantum Physics · Physics 2015-06-19 Anna J. Parker , Hai-Jing Wang , Yiran Li , Alexander Pines , Jonathan P. King

We demonstrate the coherent control and electrical readout of the nuclear spins of ionized phosphorus donors in natural silicon. By combining pulsed illumination with coherent electron spin manipulation, we selectively ionize the donor…

Materials Science · Physics 2012-01-17 Lukas Dreher , Felix Hoehne , Martin Stutzmann , Martin S. Brandt

We report record high Si-29 spin polarization obtained using dynamic nuclear polarization in microcrystalline silicon powder. Unpaired electrons in this silicon powder are due to dangling bonds in the amorphous region of this intrinsically…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 A. E. Dementyev , D. G. Cory , C. Ramanathan

Nitrogen-vacancy centers possessing nuclear spins are promising candidates for a novel nuclear spin gyroscope. Preparation of a nuclear spin state is a crucial step to implement a sensor that utilizes a nuclear spin. In a low magnetic…

We report the manipulation of nitrogen vacancy (NV) spins in diamond when nearby ferrimagnetic insulator, yttrium iron garnet, is driven into precession. The change in NV spin polarization, as measured by changes in photoluminescence, is…

The nitrogen-vacancy (N-V) center in diamond is a promising atomic-scale system for solid-state quantum information processing. Its spin-dependent photoluminescence has enabled sensitive measurements on single N-V centers, such as: electron…

Other Condensed Matter · Physics 2015-06-25 R. J. Epstein , F. M. Mendoza , Y. K. Kato , D. D. Awschalom

The nitrogen-vacancy (N-V) center in diamond is promising as an electron spin qubit due to its long-lived coherence and optical addressability. The ground state is a spin triplet with two levels ($m_s = \pm 1$) degenerate at zero magnetic…

Other Condensed Matter · Physics 2007-10-15 T. P. Mayer Alegre , C. Santori , G. Medeiros-Ribeiro , R. G. Beausoleil

In this work, we devise a fast and effective nuclear spin hyperpolarization scheme, which is in principle magnetic field and temperature independent. We use this scheme to experimentally demonstrate polarizations of up to 66% for phosphorus…

We report achieving enhanced nuclear magnetization in a magnetic resonance force microscope experiment at 0.6 tesla and 4.2 kelvin using the dynamic nuclear polarization (DNP) effect. In our experiments a microwire coplanar waveguide…

Dynamic nuclear polarization (DNP) is a method of enhancing NMR signals via the transfer of polarization from electron spins to nuclear spins using on-resonance microwave (MW) irradiation. In most cases, monochromatic continuous-wave (MCW)…

Chemical Physics · Physics 2022-11-17 Daphna Shimon , Kelly A. Cantwell , Linta Joseph , Chandrasekhar Ramanathan

Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Ramin M. Abolfath , Anna Trojnar , Bahman Roostaei , Thomas Brabec , Pawel Hawrylak

Using a Hartman-Hahn protocol, we demonstrate spin polarization transfer from a single, optically-polarized nitrogen-vacancy (NV) center to the ensemble of paramagnetic defects hosted by an individual diamond nanocrystal. Owing to the…

Mesoscale and Nanoscale Physics · Physics 2017-03-14 Abdelghani Laraoui , Carlos A. Meriles

Hyperpolarized nanoparticles (NPs) offer high polarization levels with room temperature relaxation times exceeding half an hour. In this work, we demonstrate that the achievable hyperpolarization enhancement and relaxation (decay) time at…

We study the dynamics of optically-induced nuclear spin polarization in a fluorine-doped ZnSe epilayer via time-resolved Kerr rotation. The nuclear polarization in the vicinity of a fluorine donor is induced by interaction with coherently…

Mesoscale and Nanoscale Physics · Physics 2016-02-24 F. Heisterkamp , E. Kirstein , A. Greilich , E. A. Zhukov , T. Kazimierczuk , D. R. Yakovlev , A. Pawlis , M. Bayer

We report on a polarized-neutron Laue diffraction experiment on a single crystal of neodynium doped lanthanum magnesium nitrate hydrate containing polarized proton spins. By using dynamic nuclear polarization to polarize the proton spins,…

Shallow nitrogen-vacancy (NV) centers in diamond are promising for nano-magnetometry for they can be placed proximate to targets. To study the intrinsic magnetic properties, zero-field magnetometry is desirable. However, for shallow NV…

Mesoscale and Nanoscale Physics · Physics 2021-09-14 Ning Wang , Chu-Feng Liu , Jing-Wei Fan , Xi Feng , Weng-Hang Leong , Amit Finkler , Andrej Denisenko , Jörg Wrachtrup , Quan Li , Ren-Bao Liu

The nature of the nano-scale environment presents a major challenge for solid-state implementation of spin-based qubits. In this work, a single electron spin in an optically pumped nanometer-sized III-V semiconductor quantum dot is used to…

Single-molecule nuclear magnetic resonance (NMR) is a crown-jewel challenge in the field of magnetic resonance spectroscopy and has important applications in chemical analysis and in quantum computing. Recently, it becomes possible to…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Fazhan Shi , Xi Kong , Pengfei Wang , Fei Kong , Nan Zhao , Ren-Bao Liu , Jiangfeng Du

Recently, Pang et al reported a novel polarization transfer scheme applicable to three-spin systems, whereby a rotating-frame NMR analogue of the cross effect could transfer polarization between; e.g., two 13Cs and an 15N in a single…

Quantum Physics · Physics 2026-04-21 Sundaresan Jayanthi , Adonis Lupulescu , Julia Grinshtein , Lucio Frydman