Related papers: Optically induced dynamic nuclear spin polarisatio…
We experimentally isolate, characterize and coherently control up to six individual nuclear spins that are weakly coupled to an electron spin in diamond. Our method employs multi-pulse sequences on the electron spin that resonantly amplify…
Single NV centers in diamond coupled by hyperfine interaction to neighboring 13C nuclear spins are now widely used in the emerging quantum technologies as elements of quantum memory adjusted to NV center electron spin qubit. For nuclear…
We propose a nuclear-spin-polarization protocol in a general evolution-and-measurement framework. The protocol works in a spin-star configuration, where the central spin is coupled to the surrounding bath (nuclear) spins by flip-flop…
The application of magnetic resonance (MR) spectroscopy at progressively smaller length scales may eventually permit "chemical imaging" of spins at the surfaces of materials and biological complexes. In particular, the negatively charged…
We introduce a method for non-destructive quantification of nuclear spin polarization, of relevance to hyperpolarized spin tracers widely used in magnetic resonance from spectroscopy to in vivo imaging. In a bias field of around 30 nT we…
Following the recent successful formation and manipulation of entangled $C^{13}$ atoms on the surface of Diamond we calculate the decoherence of the electron spin polarization in Diamond via a nonperturbative treatment of the time-dependent…
Initializing quantum registers with high fidelity is a fundamental precondition for many applications like quantum information processing and sensing. The electronic and nuclear spins of a Nitrogen-Vacancy (NV) center in diamond form an…
We experimentally resolve several weakly coupled nuclear spins in diamond using a series of novelly designed dynamical decoupling controls. Some nuclear spin signals, hidden by decoherence under ordinary dynamical decoupling controls, are…
Nuclear spin imaging at the atomic level is essential for the understanding of fundamental biological phenomena and for applications such as drug discovery. The advent of novel nano-scale sensors has given hope of achieving the…
Magnetic spin resonance is a key non-invasive sensing and imaging technique across the life-, material- and fundamental sciences with further medical and commercial applications. Recent advances using paramagnetic color centers enable…
We propose a practical implementation of a two-qubit entanglement engine which denotes a scheme to generate quantum correlations through purely dissipative processes. On a diamond platform, the electron spin transitions of two…
Dynamical polarization of nuclear spin ensembles is of central importance for magnetic resonance studies, precision sensing and for applications in quantum information theory. Here we propose a scheme to generate long-lived singlet pairs in…
We demonstrate a wide-band all-optical method of nanoscale magnetic resonance (MR) spectroscopy under ambient conditions. Our method relies on cross-relaxation between a probe spin, the electronic spin of a nitrogen-vacancy centre in…
The nitrogen-vacancy (NV) centre, as a promising candidate solid state system of quantum information processing, its electron spin coherence is influenced by the magnetic field fluctuations due to the local environment. In pure diamonds,…
We present a study of the spin properties of dense layers of near-surface nitrogen-vacancy (NV) centres in diamond created by nitrogen ion implantation. The optically detected magnetic resonance contrast and linewidth, spin coherence time,…
Nuclear spins in solids exhibit long coherence times due to the small nuclear gyromagnetic ratio. This weak environmental coupling comes at the expense of slow quantum gate operations, which should be as fast as possible for many…
The ability to initialise nuclear spins, which are typically in a mixed state even at low temperature, is a key requirement of many protocols used in quantum computing and simulations as well as in magnetic resonance spectroscopy and…
We use microwave-induced dynamic nuclear polarization (DNP) of the substitutional nitrogen defects (P1 centers) in diamond to hyperpolarize bulk $^{13}$C nuclei in both single crystal and powder samples at room temperature at 3.34 T. The…
We present theoretical proposals for two-dimensional nuclear magnetic resonance spectroscopy protocols based on Nitrogen-vacancy (NV) centers in diamond that are strongly coupled to the target nuclei. Continuous microwave and…
Ionized nitrogen molecules ($^{15}$N$_{2}^+$) are used as efficient point sources for creating NV$^-$ pairs in diamond with nanoscale spatial separation and up to 55 kHz magnetic coupling strength. Co-implantation of $^{12}$C$^+$ increased…