Related papers: Candidate quantum spin ice in the pyrochlore Pr$_2…
Spin ice materials are the model systems that have a zero-point entropy as \textit{T} $\rightarrow$ 0 K, owing to the frozen disordered states. Here, we chemically alter the well-known spin ice Ho$_{2}$Ti$_{2}$O$_{7}$ by replacing Ti sites…
In this work we present inelastic neutron scattering experiments which probe the single ion ground states of the rare earth pyrochlores $R_2$Ti$_2$O$_7$ ($R$ = Tb, Dy, Ho). Dy$_2$Ti$_2$O$_7$ and Ho$_2$Ti$_2$O$_7$ are dipolar spin ices, now…
Recent experiments suggest that the Ising pyrochlore magnets ${\rm Ho_{2}Ti_{2}O_{7}}$ and ${\rm Dy_{2}Ti_{2}O_{7}}$ display qualitative properties of the spin ice model proposed by Harris {\it et al.} \prl {\bf 79}, 2554 (1997). We discuss…
Quantum spin ice materials, pyrochlore magnets with competing Ising and transverse exchange interactions, have been widely discussed as candidates for a quantum spin-liquid ground state. Here, motivated by quantum chemical calculations for…
Pyrochlore iridates and pyrochlore ices are two families of materials where novel quantum phenomena are intertwined with strong spin-orbit coupling, substantial electron correlation and geometrical frustration. Motivated by the puzzling…
We present new high resolution inelastic neutron scattering data on the candidate spin liquid Tb2Ti2O7. We find that there is no evidence for a zero field splitting of the ground state doublet within the 0.2 K resolution of the instrument.…
Quantum spin liquids are highly entangled ground states of quantum systems with emergent gauge structure, fractionalized spinon excitations, and other unusual properties. While these features clearly distinguish quantum spin liquids from…
We report structural and magnetic properties studies of large high quality single-crystals of the frustrated magnet, Nd$_2$Zr$_2$O$_7$. Powder x-ray diffraction analysis confirms that Nd$_2$Zr$_2$O$_7$ adopts the pyrochlore structure.…
The low-temperature spin dynamics of the orthorhombic TbFeO$_3$ perovskite has been studied. It has been found that the inelastic neutron scattering (INS) spectrum contains two modes corresponding to different sublattices in the compound.…
The search for two dimensional quantum spin liquids, exotic magnetic states with an entangled ground state remaining disordered down to zero temperature, has been a great challenge in frustrated magnetism during the last decades. Recently,…
Little is so far known about the magnetism of the $\rm A_2B_2O_7$ monoclinic layered perovskites that replace the spin-ice supporting pyrochlore structure for $r_A/r_B>1.78$. We show that high quality monoclinic Pr$_2$Ti$_2$O$_7$ single…
We report magnetization and ac susceptibility of single crystals of the spin ice compound Dy2Ti2O7. Saturated moments at 1.8 K along the charasteristic axes [100] and [110] agree with the expected values for an effective ferromagnetic…
Tb2Ti2O7 is a pyrochlore antiferromagnet that has dynamical spins and only short-range correlations even at 50 mK; the lowest temperature explored so far, which is much smaller than the scale set by the Curie-Weiss temperature T_{CW}~14 K.…
Geometrical frustration is a central challenge in contemporary condensed matter physics, a crucible favourable to the emergence of novel physics. The pyrochlore magnets, with rare earth magnetic moments localized at the vertices of…
The consecutive magnetic ordering of the Ho and Ru ions in the pyrochlore Ho2Ru2O7 and their interplay are investigated by neutron scattering, magnetic and specific heat measurements. The Ru moments order at 95 K into a $\Gamma_5$…
Two geometrically frustrated pyrochlore stannates, undergoing long range magnetic order below 1K, were investigated at very low temperature. Anomalies in the behaviour of hyperfine quantities are found, by 155Gd Mossbauer spectroscopy in…
Motivated by the potential chiral spin liquid in the metallic spin ice Pr2Ir2O7, we consider how such a chiral state might be selected from the spin ice manifold. We propose that chiral fluctuations of the conducting Ir moments promote…
Various physical properties of the pyrochlore oxide Y2-xBixIr2O7 have been studied. The magnetizations M measured under the conditions of the zero-field-cooling(ZFC) and the field-cooling(FC) have different values below the temperature…
We report neutron scattering studies of the spin correlations of the geometrically frustrated pyrochlore Tb2Mo2O7 using single crystal samples. This material undergoes a spin-freezing transition below Tg~24 K, similar to Y2Mo2O7, and has…
Rare-earth pyrochlores are known to exhibit exotic magnetic phenomena. We report a study of crystal growth and characterizations of a new rare-earth compound Er$_2$AlSbO$_7$, in which Al$^{3+}$ and Sb$^{5+}$ ions share the same positions…