Related papers: Ultralong-range triatomic Rydberg molecules in an …
Over the past few years we have built an apparatus to demonstrate the entanglement of neutral Rb atoms at optically resolvable distances using the strong interactions between Rydberg atoms. Here we review the basic physics involved in this…
It is common knowledge that atoms can form molecules if they attract each other. Here, we show that it is possible to create molecules where bound states of the atoms are not the result of attractive interactions but have the topological…
A detailed theoretical framework for highly excited Rydberg molecules is developed based on the generalized local frame transformation. Our approach avoids the use of pseudopotentials and yields analytical expressions for the body-frame…
We study Rydberg atoms modulated by strong radio-frequency (RF) fields with a frequency of 70 MHz. The Rydberg atoms are prepared in a room temperature cesium cell, and their level structure is probed using electromagnetically induced…
The dynamics of the outer electron in an alkali atom in the presence of structured electromagnetic waves is described. The interaction of the alkali Rydberg atom with twisted radiowaves is considered. The two schemes for Rydberg-atom based…
The spectrum of triatomic molecules with close rovibrational opposite parity levels is sensitive to the $\mathcal{P}$,$\mathcal{T}$-odd effects. This makes them a convenient platform for the experimental search of a new physics. Among the…
Ultracold molecules provide opportunities for exploring quantum matter, chemical dynamics and information processing thanks to their rich interactions, which can be controlled by external fields. Magnetic fields tune interactions through…
We demonstrate Rydberg blockade due to the charge-dipole interaction between a single Rb atom and a single RbCs molecule confined in optical tweezers. The molecule is formed by magnetoassociation of a Rb+Cs atom pair and subsequently…
We report on a novel method for photo-association of strongly polar trilobite Rydberg molecules. This exotic ultralong-range dimer, consisting of a ground-state atom bound to the Rydberg electron via electron-neutral scattering, inherits…
We calculate vibrational spectra of ultralong-range Cs(32p) Rydberg molecules which form in an ultracold gas of Cs atoms. We account for the partial-wave scattering of the Rydberg electrons from the ground Cs perturber atoms by including…
Laser cooled Rb atoms were optically excited to 46d Rydberg states. A microwave pulse transferred a fraction of the atoms to the 47p Rydberg state. The resonant electric dipole-dipole interactions between atoms in these two states were…
We present experimental evidence for spin-orbit interaction of an electron as it scatters from a neutral atom. The scattering process takes place within a Rb$_2$ ultralong-range Rydberg molecule, consisting of a Rydberg atomic core, a…
In this article we extend the theory of ultra-long-range giant dipole molecules, formed by an atom in a giant dipole state and a ground-state alkali atom, by angular-momentum couplings known from recent works on Rydberg molecules. In…
The electric fields near the heterogeneous metal/dielectric surface of an atom chip were measured using cold atoms. The atomic sensitivity to electric fields was enhanced by exciting the atoms to Rydberg states that are 10^8 times more…
Rydberg blockade sphere persists an intriguing picture by which a number of collective many-body effects caused by the strong Rydberg-Rydberg interactions can be clearly understood and profoundly investigated. In the present work, we…
We undertake a semiclassical analysis of the spectral properties (modulations of photoabsorption spectra, energy level statistics) of a simple Rydberg molecule in static fields within the framework of Closed-Orbit/Periodic-Orbit theories.…
We perform a comparative analysis of different computational approaches employed to explore the electronic structure of ultralong-range Rydberg molecules. Employing the Fermi pseudopotential approach, where the interaction is approximated…
Since their first experimental observation, ultralong-range Rydberg molecules consisting of a highly excited Rydberg atom and a ground state atom have attracted the interest in the field of ultracold chemistry. Especially the intriguing…
We analyze a model problem representing a multi-electronic molecule sitting on a metal surface. Working with a reduced configuration interaction Hamiltonian, we show that one can extract very accurate ground state wavefunctions as compared…
We analyze bound states of an electron in the field of a positively charged nanoshell. We find that the binding and excitation energies of the system decrease when the radius of the nanoshell increases. We also show that the ground and the…