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We introduce the Rydberg Composite, a new class of Rydberg matter where a single Rydberg atom is interfaced with a dense environment of neutral ground state atoms. The properties of the Composite depend on both the Rydberg excitation, which…

Atomic Physics · Physics 2020-09-02 Andrew L. Hunter , Matthew T. Eiles , Alex Eisfeld , Jan M. Rost

Cs$_2$ Rydberg-ground molecules consisting of a Rydberg, $nD_{J}$ (33 $\leq$ $n$ $\leq$ 39), and a ground state atom, 6$S_{1/2} (F=$3 or 4$)$, are investigated by photo-association spectroscopy in a cold atomic gas. We observe vibrational…

Atomic and Molecular Clusters · Physics 2020-10-07 Suying Bai , Xiaoxuan Han , Jingxu Bai , Yuechun Jiao , Jianming Zhao , Suotang Jia , Georg Raithel

Rydberg molecules, Rydberg-atom or Rydberg-molecule, are an essential ingredient of cold molecular sciences. However, due to the richness of Rydberg-neutral interactions, new kinds of Rydberg molecules and binding mechanisms are still to be…

Atomic Physics · Physics 2025-02-18 Mateo Londoño , Vanessa C. Olaya-Agudelo , Felipe Herrera , Jesús Pérez-Ríos

We explore the feasibility of optically forming long-range tetratomic and larger polyatomic molecules in their ground electronic state from ultracold pairs of polar molecules aligned by external fields. Depending on the relative orientation…

Atomic Physics · Physics 2021-06-16 Marko Gacesa , Jason N. Byrd , Jonathan Smucker , John A. Montgomery, , Robin Côté

Ultracold atomic gases have been used extensively in recent years to realize textbook examples of condensed matter phenomena. Recently, phase transitions to ordered structures have been predicted for gases of highly excited, 'frozen'…

Ensembles of atoms interacting via their Rydberg levels, known as "superatoms" for their ability to encode qubits and to emit single photons, attract increasing attention as building blocks for quantum network nodes. Assessing their…

Quantum Physics · Physics 2026-01-27 Valentin Magro , Sébastien Garcia , Alexei Ourjoumtsev

A spatial structure of the zone blocked by the dipolar electric field of a Rydberg atom is calculated taking into account a possibility of excitation to the states with neighboring values of the principal quantum number. As a result, it was…

Atomic Physics · Physics 2014-08-26 Yurii V. Dumin

A remarkable property of Rydberg atoms is the possibility to create molecules formed by one highly excited atom and another atom in the ground state. The first realisation of such a Rydberg molecule has opened an active field of physical…

Atomic Physics · Physics 2013-04-02 Andrej Junginger , Jörg Main , Günter Wunner

The electronic spectrum of a Rydberg atom immersed in a Bose-Einstein condensate is investigated. The Heisenberg equations of motions for the condensate and the Rydberg atom are derived. Neglecting the backaction of the Rydberg atom onto…

Other Condensed Matter · Physics 2008-11-17 Stephan Middelkamp , Igor Lesanovsky , P. Schmelcher

We report on the observation of two vibrational series of pure trilobite rubidium Rydberg molecules. They are created via three-photon photoassociation and lie energetically more than 15 GHz below the atomic 22$F$ state of rubidium. In…

Atomic Physics · Physics 2023-07-06 Max Althön , Markus Exner , Richard Blättner , Herwig Ott

In this work we discuss the rotational structure of Rydberg molecules. We calculate the complete wave function in a laboratory fixed frame and derive the transition matrix elements for the pho- toassociation of free ground state atoms. We…

Atomic Physics · Physics 2018-08-01 O. Thomas , C. Lippe , T. Eichert , H. Ott

We study the Rydberg blockade in a system of three atoms arranged in different 2D geometries (linear and triangular configurations). In the strong blockade regime, we observe high-contrast, coherent collective oscillations of the single…

Recent developments in the study of ultracold Rydberg gases demand an advanced level of experimental sophistication, in which high atomic and optical densities must be combined with excellent control of external fields and sensitive Rydberg…

We propose a quantum sensor for electric fields based on networks of Rydberg atoms. The sensing mechanism exploits the strong dependence of the Rydberg blockade on the applied electric field near a F\"orster resonance. In this regime,…

Quantum Physics · Physics 2026-05-28 Philip Kitson , Wayne J. Chetcuti , Gerhard Birkl , Luigi Amico , Juan Polo

We observe a series of conical intersections in the potential energy curves governing both the collision between a Rydberg atom and a ground-state atom and the structure of Rydberg molecules. By employing the electronic energy of the…

Atomic Physics · Physics 2021-07-14 Frederic Hummel , Matthew T. Eiles , Peter Schmelcher

We predict the existence of a class of ultracold giant molecules formed from trapped ultracold Rydberg atoms and polar molecules. The interaction which leads to the formation of such molecules is the anisotropic charge-dipole interaction…

Atomic Physics · Physics 2015-05-18 Seth T. Rittenhouse , H. R. Sadeghpour

The dynamics of Rydberg states of a hydrogen atom subject simultaneously to uniform static electric field and two microwave fields with commensurate frequencies is considered in the range of small fields amplitudes. In the certain range of…

Quantum Physics · Physics 2009-11-07 Krzysztof Sacha , Jakub Zakrzewski

We present combined measurements of the spatially-resolved optical spectrum and the total excited-atom number in an ultracold gas of three-level atoms under electromagnetically induced transparency conditions involving high-lying Rydberg…

We propose an experiment to demonstrate a novel blockade mechanism caused by long-range anisotropic interactions in an ultracold dipolar gas composed of the recently observed "butterfly" Rydberg molecules. At the blockade radius, the strong…

Atomic Physics · Physics 2017-09-21 Matthew T. Eiles , Hyunwoo Lee , Jesus Perez-Rios , Chris H. Greene

Double-resonant photoexcitation of nitric oxide in a molecular beam creates a dense ensemble of $50f(2)$ Rydberg states, which evolves to form a plasma of free electrons trapped in the potential well of an NO$^+$ spacecharge. The plasma…

Chemical Physics · Physics 2015-05-27 N. Saquet , J. P. Morrison , M. Schulz-Weiling , H. Sadeghi , J. Yiu , C. J. Rennick , E. R. Grant
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