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This study examines the Raman scattering and charge transfer properties of molecules adsorbed on the surface of a tetrahedral Au$_{120}$ nanoparticle based on the time-dependent density functional tight-binding (TD-DFTB) method. We study…

Chemical Physics · Physics 2024-09-18 Sajal Kumar Giri , George C. Schatz

Raman scattering on phonon--plasmon coupled modes in high magnetic fields is considered theoretically. The calculations of the dielectric function were performed in the long-wave approximation for the semiclassical and ultra-quantum…

Materials Science · Physics 2007-05-23 L. A. Falkovsky

The probability of emission of a single photon via Raman scattering of laser pulse on the three-level $\Lambda$ - type atom in microcavity is studied. The duration of the pulse is considered to be short enough, so that the hyperfine…

Quantum Physics · Physics 2015-05-14 V. A. Reshetov , I. V. Yevseyev

Quantum squeezed states enable precision measurements beyond the standard quantum limit, but conventional solid-state media fundamentally limit pump intensities to the ionization threshold. We demonstrate that plasma waves can mediate…

Plasma Physics · Physics 2025-07-17 Kenan Qu , Nathaniel J. Fisch

We present a method for deriving limits on Raman scattering in structured media and exploit it to constrain the maximum Raman signal resulting from a planewave incident on either a single Raman molecule in the vicinity of a structured…

The microwave phonon stimulated emission (SE) has been experimentally and numerically investigated in a nonautonomous microwave acoustic quantum generator, called also microwave phonon laser or phaser (see previous works…

Chaotic Dynamics · Physics 2009-06-25 D. N. Makovetskii

The success of non-linear optics relies largely on pulse-to-pulse consistency. In contrast, covariance based techniques used in photoionization electron spectroscopy and mass spectrometry have shown that wealth of information can be…

We investigate the propagation of a coherent probe light pulse through a three-level atomic medium (in the $\Lambda$--configuration) in the presence of a pump laser under the conditions for gain without inversion. When the carrier frequency…

Quantum Physics · Physics 2007-05-23 Filippo Caruso , Ivan Herrera , Saverio Bartalini , Francesco Cataliotti

Raman scattering is the inelastic process where photons bounce off molecules, losing energy and becoming red-shifted. This weak effect is unique to each molecular species, making it an essential tool in e.g. spectroscopy and label-free…

Plasma is capable of mediating the conversion of two pump photons into two different photons through a relativistic four-wave mixing nonlinearity. Spontaneously created photon pairs are emitted at symmetric angles with respect to the…

Plasma Physics · Physics 2025-01-07 Kenan Qu , Nathaniel J. Fisch

Time-dependent nonlinear media, such as rapidly generated plasmas produced via laser ionization of gases, can increase the energy of individual laser photons and generate tunable high-order harmonic pulses. This phenomenon, known as photon…

We have investigated the effects of tuning the localized surface plasmon resonances (LSPRs) of silver nanoparticles on the fluorescence intensity, lifetime, and Raman signal from nearby fluorophores. The presence of a metallic structure can…

Other Condensed Matter · Physics 2009-11-13 N. I. Cade , T. Ritman-Meer , D. Richards

Stimulated Raman scattering of a laser pump pulse seeded by a Stokes pulse generically leaves a two-level medium initially at rest in an excited state constituted of static solitons and radiation. The soliton birth manifests as sudden very…

solv-int · Physics 2016-09-08 J. Leon , A. V. Mikhailov

We present a self-consistent quantum optics approach to calculating the surface enhanced Raman spectrum of molecules coupled to arbitrarily shaped plasmonic systems. Our treatment is intuitive to use and provides fresh analytical insight…

Optics · Physics 2017-06-26 Mohsen Kamandar Dezfouli , Stephen Hughes

Phonon-polaritons propagating in crystal volume offer the possibility of transferring information throughout matter (via phonons) at high (photon-like) velocity and tunable frequency/wavelength in the far-infrared. However, from the…

Optics · Physics 2025-09-03 Mayssoune Mina , Toni Alhaddad , Olivier Pagès

The "Impulsive Stimulated Raman Scattering" (ISRS), is generally performed using ultrashort laser pulses. It shifts the frequency of the laser beam without any change of the wave surfaces and any appearance of extra lines. ISRS works with…

Astrophysics · Physics 2007-05-23 Jacques Moret-Bailly

Steady-state plasmonic lasing is studied theoretically for a system consisting of many dye molecules arranged regularly around a gold nano-sphere. A three-level model with realistic molecular dissipation is employed to analyze the…

Optics · Physics 2018-01-31 Yuan Zhang , Klaus Mølmer

The hybrid Stimulated Raman Scattering - Two Plasmon Decay instability had shown to play the dominant role for plasma waves excitation and energy absorption at interaction of very intense femtosecond obliquely incident $p$-polarized laser…

Plasma Physics · Physics 2021-01-04 I. Tsymbalov , D. Gorlova , A. Savel'ev

Quantum electrodynamics theory of the resonance Raman scattering is developed for an atom in a close proximity to a carbon nanotube. The theory predicts a dramatic enhancement of the Raman intensity in the strong atomic coupling regime to…

Mesoscale and Nanoscale Physics · Physics 2015-12-07 I. V. Bondarev

Exact four-photon resonance of collinear planar laser pulses is known to be prohibited by the classical dispersion law of electromagnetic waves in plasma. We show here that the renormalization produced by an arbitrarily small relativistic…

Plasma Physics · Physics 2020-12-30 V. M. Malkin , N. J. Fisch