Related papers: Stepwise quantum phonon pumping in plasmon-enhance…
Raman backscattered radiation of intense laser pulses in plasma is investigated for a wide range of intensities relevant to laser wakefield acceleration. The weakly nonlinear dispersion relation for Raman backscattering predicts an…
We report plasmon-enhanced Raman scattering in graphene coupled to a single plasmonic hotspot measured as a function of laser energy. The enhancement profiles of the G peak show strong enhancement (up to $10^5$) and narrow resonances (30…
The physical processes associated with propagation of a high-power (power > critical power for self-focusing) laser beam in water include nonlinear focusing, stimulated Raman scattering (SRS), optical breakdown and plasma formation. The…
Plasmonic molecular nanojunctions exhibit opto-mechanical coupling at the nanoscale, enabling intertwined optical, vibrational and electronic phenomena. Here, we demonstrate plasmon-mediated phonon pumping, driven by inelastic electron…
The conventional explanation of plasmon-enhanced Raman scattering attributes the enhancement to the antenna effect focusing the electromagnetic field into sub-wavelength volumes. Here we introduce a new model that additionally accounts for…
Bloch equations for the atomic population and the polarization/coherence and the equation of motion for the photon number in a laser are solved in steady state as a function of the pump rate. Two level atom and two modes of three levels…
We present a detailed study of a phonon-assisted incoherent excitation mechanism of single quantum dots. A spectrally-detuned laser couples to a quantum dot transition by mediation of acoustic phonons, whereby excitation efficiencies up to…
We propose a method for increasing the Raman scattering from an ensemble of molecules by up to four orders of magnitude. Our method requires an additional coherent source of IR radiation with the half-frequency of the Stokes shift. This…
We study the quantum state of phonons propagating on top of a fluid of light coherently generated in a planar microcavity device by a quasi-resonant incident laser beam. In the steady-state under a monochromatic pump, because of the finite…
Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…
Surface-Enhanced Raman Scattering (SERS) allows for detection and identification of molecular vibrational fingerprints in minute sample quantities. The SERS process can be also exploited for optical manipulation of molecular vibrations. We…
In this work we develop an experimental procedure to interrogate the single- and multiphoton scattering matrices of an unknown quantum system interacting with propagating photons. Our proposal requires coherent state laser or microwave…
Spin-polarised atomic ensembles probed by light based on the Faraday interaction are a versatile platform for numerous applications in quantum metrology and quantum information processing. Here we consider an ensemble of Alkali atoms that…
Light amplification towards extremely high power in the infrared regime remains a significant challenge due to the lack of suitable gain media. Here we propose a new scheme to amplify a laser pulse with tunable wavelengths towards extremely…
We study coherent backscattering of a quasi-monochromatic laser by a dilute gas of cold two-level atoms. We consider the perturbative regime of weak intensities, where nonlinear effects arise from {\em inelastic} two-photon scattering…
Localized surface plasmon resonances have recently attracted considerable attention due to their ability to dramatically enhance near-field optical intensities and boost nanoscale light-matter interactions. Here we demonstrate unambiguously…
The interaction between ultrashort light pulses and non-absorbing materials is dominated by Impulsive Stimulated Raman Scattering (ISRS). The description of ISRS in the context of pump\&probe experiments is based on effective classical…
We present a novel approach to transient Raman spectroscopy, which combines stochastic probe pulses and a covariance-based detection to measure stimulated Raman signals in alpha-quartz. A coherent broadband pump is used to simultaneously…
Surface enhanced Raman scattering mediated by surface plasmons polaritons with wave vector much larger than those of light is considered. The excitation of these polaritons and their efficient Raman scattering due to low group velocity and…
We analyse recently measured nonlinear photoemission spectra from Ag surfaces that reveal resonances whose energies do not scale with the applied photon energy but stay pinned to multiples of bulk plasmon energy $\hbar\omega_p$ above the…