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We have studied spin excitations in a single-domain crystal of antiferromagnetic LiCoPO4 by THz absorption spectroscopy. By analyzing the selection rules and comparing the strengths of the absorption peaks in the different antiferromagnetic…

A joint theoretical approach, combining macroscopic symmetry analysis with microscopic methods (density functional theory and model cluster Hamiltonian), is employed to shed light on magnetoelectricity in Ba2CoGe2O7. We show that the…

Strongly Correlated Electrons · Physics 2015-05-27 Kunihiko Yamauchi , Paolo Barone , Silvia Picozzi

The multiferroic compound CuO exhibits low temperature magnetic properties similar to antiferromagnetic iron oxides, while the electronic properties have much more in common with the high $T_c$ cuprate superconductors. This suggests novel…

Strongly Correlated Electrons · Physics 2016-11-02 Johan Hellsvik , Johan H. Mentink , José Lorenzana

A quasi-one dimensional antiferromagnet with a strong reduction of the ordered spin component, BaCu2Si2O7, is studied by the magnetic resonance technique in a wide field and frequency range. Besides of conventional spin-flop transition at…

Strongly Correlated Electrons · Physics 2009-11-11 V. N. Glazkov , A. I. Smirnov , A. Revcolevschi , G. Dhalenne

Magnetic excitations are investigated for a hexagonal polar magnet Fe2Mo3O8 by terahertz spectroscopy. We observed magnon modes including an electric-field active magnon, electromagnon, in the collinear antiferromagnetic phase with spins…

Strongly Correlated Electrons · Physics 2017-01-09 T. Kurumaji , Y. Takahashi , J. Fujioka , R. Masuda , H. Shishikura , S. Ishiwata , Y. Tokura

Recent spectroscopic studies at terahertz frequencies for a variety of multiferroics endowed with both ferroelectric and magnetic orders have revealed the possible emergence of a new collective excitation, frequently referred to as…

Strongly Correlated Electrons · Physics 2009-06-11 N. Kida , Y. Takahashi , J. S. Lee , R. Shimano , Y. Yamasaki , Y. Kaneko , S. Miyahara , N. Furukawa , T. Arima , Y. Tokura

We experimentally demonstrate that in magnetostrictive ferrimagnetic single crystal of CoFe2O4 there is clear correlation between magnetostriction and magnetoreflection of unpolarized light in the infrared range. The influence of magnetic…

Materials Science · Physics 2017-08-23 Yu. P. Sukhorukov , A. V. Telegin , N. G. Bebenin , A. P. Nosov , V. D. Bessonov , A. A. Buchkevich

Magnetic excitations in cycloidal magnet LiCu$_2$O$_2$ are explored using THz absorption spectroscopy in magnetic fields up to 12 T. Below the spin ordering temperature we observe eight optically active transitions in the spin system of…

Strongly Correlated Electrons · Physics 2015-05-13 D. Hüvonen , U. Nagel , T. Rõõm , Y. J. Choi , C. L. Zhang , S. Park , S. -W. Cheong

Photo-excitation in complex oxides1 transfers charge across semicovalent bonds, drastically perturbing spin and orbital orders2. Light may then be used in compounds like magnetoresistive manganites to control magnetism on nanometre…

We report ferroelectric ordering in Ni substituted CaBaCo4O7. Magnetization showed ferrimagnetic transition at 60 K and an additional transition is found ~ 82 K, further, enhanced antiferromagnetic interactions and decrease in saturation…

Materials Science · Physics 2017-10-18 C. Dhanasekhar , A. K Das , Ripandeep Singh , A. Das , G. Giovannetti , D. Khomskii , A. Venimadhav

Terahertz and far-infrared electric and magnetic responses of hexagonal piezomagnetic YMnO3 single crystals are investigated. Antiferromagnetic resonance is observed in the spectra of magnetic permeability mu_a [H(omega) oriented within the…

Materials Science · Physics 2012-02-13 C. Kadlec , V. Goian , K. Z. Rushchanskii , P. Kuzel , M. Lezaic , K. Kohn , R. V. Pisarev , S. Kamba

All-electrical control of a dynamic magnetoelectric effect is demonstrated in a classical multiferroic manganite DyMnO3, a material containing coupled antiferromagnetic and ferroelectric orders. Due to intrinsic magnetoelectric coupling…

Strongly Correlated Electrons · Physics 2017-04-06 A. Shuvaev , V. Dziom , Anna Pimenov , M. Schiebl , A. A. Mukhin , A. Komarek , T. Finger , M. Braden , A. Pimenov

Polarized far-infrared (FIR) spectroscopic measurements and FIR magneto-optical studies were performed on the inorganic spin-Peierls compound CuGeO_3. An absorption line, which was found at 98 cm$^{-1}$ in the dimerized phase (D phase), was…

Strongly Correlated Electrons · Physics 2009-10-31 K. Takehana , T. Takamasu , M. Hase , G. Kido , K. Uchinokura

We investigated the spin excitations of magnetoelectric $\text{LiFePO}_4$ by THz absorption spectroscopy in magnetic fields up to 33$\,$T. By studying their selection rules, we found not only magnetic-dipole, but also electric-dipole active…

Photons carrying a well-defined orbital angular momentum have been proven to modify spectroscopic selection rules in atomic matter. Excitation profiles of electric quadrupole transitions have been measured with single trapped $^{40}$Ca$^+$…

We provide a detailed study of the reflectivity of multiferroic TbMnO_3 for wave numbers from 40 cm^{-1} to 1000 cm^{-1} and temperatures 5 K < T < 300 K. Excitations are studied for polarization directions E || a, the polarization where…

Strongly Correlated Electrons · Physics 2010-01-22 M. Schmidt , Ch. Kant , T. Rudolf , F. Mayr , A. A. Mukhin , A. M. Balbashov , J. Deisenhofer , A. Loidl

In rhombohedral CaMn7O12, an improper ferroelectric polarization of magnitude 2870 {\mu}C m-2 is induced by an incommensurate helical magnetic structure that evolves below TN1 = 90 K. The electric polarization was found to be constrained to…

Strongly Correlated Electrons · Physics 2015-05-30 R. D. Johnson , L. C. Chapon , D. D. Khalyavin , P. Manuel , P. G. Radaelli , C. Martin

We calculate the effective charge for multimagnon infrared (IR) absorption assisted by phonons in a perovskite like antiferromagnet and we compute the spectra for two magnon absorption using interacting spin-wave theory. The full set of…

Condensed Matter · Physics 2008-06-16 J. Lorenzana , G. A. Sawatzky

When two-dimensional electron gases (2DEGs) are exposed to magnetic field, they resonantly absorb electromagnetic radiation via electronic transitions between Landau levels (LLs). In 2DEGs with a Dirac spectrum, such as graphene, theory…

Strongly Correlated Electrons · Physics 2019-07-15 Ievgeniia O. Nedoliuk , Sheng Hu , Andre K. Geim , Alexey B. Kuzmenko

In multiferroic TbMn$_2$O$_5$, the behavior of the terbium ions forms a crucial part of the magneto-electric coupling. The result is a magnetically induced reversal of the electric polarization at 2 T. In this article we present the first…

Strongly Correlated Electrons · Physics 2011-06-27 R. D. Johnson , C. Mazzoli , S. R. Bland , C-H. Du , P. D. Hatton