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A quantum spin liquid (QSL) is a state of matter in which magnetic spins interact strongly, but quantum fluctuations inhibit long-range magnetic order even at zero temperature. A QSL has been predicted to have a host of exotic properties,…

The face-centered-cubic lattice is composed of edge-sharing tetrahedra, making it a leading candidate host for strongly frustrated magnetism, but relatively few face-centered frustrated materials have been investigated. In the hydroxide…

A recently discovered material, 6H-B-Ba3NiSb2O9 was found to display unusual low-temperature phenomenology, interpreted as a quantum spin liquid with spin S = 1 on a triangular lattice. We study a spin S = 1 quantum exchange model on an AB…

Strongly Correlated Electrons · Physics 2012-08-27 Gang Chen , Michael Hermele , Leo Radzihovsky

By using a high pressure, high temperature (HPHT) technique, the antiferromagnetically ordered ($T_N$ = 13.5 K) 6H-A phase of Ba$_3$NiSb$_2$O$_9$ was transformed into two new gapless quantum spin liquid(QSL) candidates with S=1 (Ni$^{2+}$)…

Strongly Correlated Electrons · Physics 2011-11-08 J. G. Cheng , G. Li , L. Balicas , J. S. Zhou , J. B. Goodenough , Cenke Xu , H. D. Zhou

Geometrical frustration, quantum entanglement and disorder may prevent long-range order of localized spins with strong exchange interactions, resulting in a novel state of matter. $\kappa$-(BEDT-TTF)$_2$-Cu$_2$(CN)$_3$ is considered the…

Unlike conventional magnets where the magnetic moments are partially or completely static in the ground state, in a quantum spin liquid they remain in collective motion down to the lowest temperatures. The importance of this state is that…

The magnetic phase diagram and the thermodynamic properties of a square lattice containing antiferromagnetically coupled spin-1/2 triangles are studied. A Heisenberg Hamiltonian with three strong intra-triangle exchange coupling constants…

Strongly Correlated Electrons · Physics 2009-10-31 Stefan Wessel , Stephan Haas

We present data on the magnetic properties of two classes of layered spin S=1/2 antiferromagnetic quasi-triangular lattice materials: $Cu_{2(1-x)}Zn_{2x}(OH)_3NO_3$ ($0 < x < 0.65$) and its long chain organic derivatives…

Strongly Correlated Electrons · Physics 2011-04-11 Jian Wu , Julia S. Wildeboer , Fletcher Werner , Alexander Seidel , Z. Nussinov , S. A. Solin

The interplay between competing degrees of freedom can stabilize non-trivial magnetic states in correlated electron materials. Frustration-induced strong quantum fluctuations can evade long-range magnetic ordering leading to exotic quantum…

Strongly Correlated Electrons · Physics 2023-10-12 B. Sana , M. Barik , M. Pregelj , U. Jena , M. Baenitz , J. Sichelschmidt , K. Sethupathi , P. Khuntia

A triangular lattice selenide series of rare earth (RE), CsRESe2, were synthesized as large single crystals using a flux growth method. This series stabilized in either trigonal (R-3m) or hexagonal (P63/mmc) crystal systems. Physical…

Magneto-acoustic investigations of the frustrated triangular-lattice antiferromagnet Cs2CuCl4 were performed for the longitudinal modes c11 and c33 in magnetic fields along the a-axis. The temperature dependence of the sound velocity at…

Strongly Correlated Electrons · Physics 2016-09-21 P. T. Cong , L. Postulka , B. Wolf , N. van Well , F. Ritter , W. Assmus , C. Krellner , M. Lang

We study the energetics of Gutzwiller projected BCS states of various symmetries for the triangular lattice antiferromagnet with a four particle ring exchange using variational Monte Carlo methods. In a range of parameters the energetically…

Strongly Correlated Electrons · Physics 2011-01-04 Tarun Grover , N. Trivedi , T. Senthil , Patrick A. Lee

Frustration, spin correlations and interplay between competing degrees of freedom are some of the key ingredients that underlie exotic states with fractional excitations in quantum materials. Rare-earth based two dimensional magnetic…

Strongly Correlated Electrons · Physics 2022-09-13 J. Khatua , M. Pregelj , A. Elghandour , Z. Jaglicic , R. Klingeler , A. Zorko , P. Khuntia

We present a microscopic model of the spin-gap quantum magnet (CuCl)LaNb2O7 that was previously suggested as a realization of the spin-1/2 frustrated square lattice. Taking advantage of the precise atomic positions from recent crystal…

Strongly Correlated Electrons · Physics 2010-08-30 Alexander A. Tsirlin , Helge Rosner

1T-tantalum disulphide (1T-TaS2) is a promising material to realize quantum spin liquid state and fractional excitations. Here, we take a closer look on the temperature dependent magnetic susceptibility of 1T-TaS2 at low magnetic fields to…

Strongly Correlated Electrons · Physics 2022-07-28 Sudip Pal , S. B. Roy

Spinel-structured compounds serve as prototypical examples of highly frustrated systems, and are promising candidates for realizing the long-sought quantum spin liquid (QSL) state. However, structural disorder is inevitable in many real QSL…

We report on high-field electron spin resonance (ESR) studies of magnetic excitations in the spin-1/2 triangular-lattice antiferromagnet Cs$_2$CuBr$_4$. Frequency-field diagrams of ESR excitations are measured for different orientations of…

Triangular lattice antiferromagnets first attracted attention as a frustrated magnetic lattice which can serve as a platform to realize the resonating valence bond state. While the triangular lattice itself was shown to support classical…

Strongly Correlated Electrons · Physics 2026-05-25 Jazzmin Victorin , Shreenanda Ghosh , Seyed Koohpayeh , Chris Lygouras , Natalia Drichko

The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper…

Statistical Mechanics · Physics 2007-05-23 Hamid R. Molavian , Michel J. P. Gingras , Benjamin Canals

Cs2CoBr4 is a triangular-lattice antiferromagnet which can be viewed as weakly interacting spin chains due to spatially anisotropic frustrating exchange couplings. The spin-orbit interaction in Co(2+) spin-3/2 ions leads to a strong…

Strongly Correlated Electrons · Physics 2023-09-06 T. A. Soldatov , A. I. Smirnov , A. V. Syromyatnikov