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We demonstrate ionization of a molecule with the bias voltage of a Scanning Tunnelling Microscope (STM) resulting in a coexistence of a neutral and ionic molecules, i.e. radical (paramagnetic) and non-radical (diamagnetic) states. This…

Mesoscale and Nanoscale Physics · Physics 2024-04-02 Yishay Manassen , Michael Averbukh , Zion Hazan , Yahel Tzuriel , Pino Boscolo , Alexsander Shnirman , Baruch Horovitz

Nuclear Magnetic Resonance (NMR) spans diverse fields from biology to quantum science. Employing NMR on a floating object could unveil novel possibilities beyond conventional operational paradigms. Here, we observe Nuclear Magnetic…

Quantum Physics · Physics 2024-07-30 J. Voisin , A. Durand , T. Copie , M. Perdriat , G. Hétet

Dynamic nuclear polarization (DNP) of molecules in a solution at room temperature has potential to revolutionize nuclear magnetic resonance spectroscopy and imaging. The prevalent methods for achieving DNP in solutions are typically most…

Chemical Physics · Physics 2016-03-02 Qiong Chen , Ilai Schwarz , Fedor Jelezko , Alex Retzker , Martin B Plenio

Solid state spins have demonstrated significant potential in quantum sensing with applications including fundamental science, medical diagnostics and navigation. The quantum sensing schemes showing best performance under ambient conditions…

Mesoscale and Nanoscale Physics · Physics 2023-06-14 Beat Bürgler , Tobias F. Sjolander , Ovidiu Brinza , Alexandre Tallaire , Jocelyn Achard , Patrick Maletinsky

Characteristic dips appear in the coherence traces of a probe qubit when dynamical decoupling (DD) is applied in synchrony with the precession of target nuclear spins, forming the basis for nanoscale nuclear magnetic resonance (NMR). The…

Dynamic nuclear polarization (DNP) is an NMR sensitivity enhancement technique that mediates polarization transfer from unpaired electrons to NMR-active nuclei. Despite its success in elucidating important structural information on…

High-fidelity control of quantum systems is crucial for quantum information processing, but is often limited by perturbations from the environment and imperfections in the applied control fields. Here, we investigate the combination of…

Quantum Physics · Physics 2021-01-12 Xiaodong Yang , Yunrui Ge , Bo Zhang , Jun Li

Single nitrogen vacancy (NV) centers in diamond have been used extensively for high-sensitivity nanoscale sensing, but conventional approaches use confocal microscopy to measure individual centers sequentially, limiting throughput and…

Nuclear Magnetic Resonance (NMR) spectroscopy is a widely-used technique in the fields of bio-medicine, chemistry, and biology for the analysis of chemicals and proteins. The signals from NMR spectroscopy often have low signal-to-noise…

Signal Processing · Electrical Eng. & Systems 2024-05-21 Zihao Zou , Shirin Shoushtari , Jiaming Liu , Jialiang Zhang , Patrick Judge , Emilia Santana , Alison Lim , Marcus Foston , Ulugbek S. Kamilov

The nitrogen-vacancy (NV) center has enabled widespread study of nanoscale nuclear magnetic resonance (NMR) spectroscopy at low magnetic fields. NMR spectroscopy at high magnetic fields significantly improves the technique's spectral…

Mesoscale and Nanoscale Physics · Physics 2021-09-15 Benjamin Fortman , Laura Mugica-Sanchez , Noah Tischler , Cooper Selco , Yuxiao Hang , Karoly Holczer , Susumu Takahashi

One-dimensional nuclear magnetic resonance (NMR) spectroscopy is essential for molecular structure elucidation in organic synthesis, drug discovery, natural product characterization, and metabolomics, yet its interpretation remains heavily…

We propose two dimensional x-ray coherent correlation spectroscopy (2DXCS) for the study of interactions between core-electron and valence transitions. This technique might find experimental applications in the future when very high…

Quantum Physics · Physics 2009-11-13 Igor V. Schweigert , Shaul Mukamel

Symmetry-resolved spectroscopies, such as angle-resolved photoemission spectroscopy and polarization-resolved Raman, are central for quantum material characterization, yet remain challenging at nanoscale dimensions and low frequencies.…

Quantum Physics · Physics 2026-04-27 Wenbo Sun , Zubin Jacob

A single nitrogen-vacancy (NV) center in diamond is a prime candidate for a solid-state quantum magnetometer capable of detecting single nuclear spins with prospective application to nuclear magnetic resonance (NMR) at the nanoscale.…

Quantum Physics · Physics 2020-02-07 Daiki Misonou , Kento Sasaki , Shuntaro Ishizu , Yasuaki Monnai , Kohei M. Itoh , Eisuke Abe

Quantum sensing exploits the strong sensitivity of quantum systems to measure small external signals. The nitrogen-vacancy (NV) center in diamond is one of the most promising platforms for real-world quantum sensing applications,…

Quantum Physics · Physics 2022-05-12 Ziwei Qiu , Uri Vool , Assaf Hamo , Amir Yacoby

Identification of individual cells within heterogeneous populations is essential for biomedical research and clinical diagnostics. Conventional labeling-based sorting methods, such as fluorescence-activated cell sorting and…

Quantum sensing exploits fundamental features of quantum mechanics and quantum control to realise sensing devices with potential applications in a broad range of scientific fields ranging from basic science to applied technology. The…

Mesoscale and Nanoscale Physics · Physics 2019-11-13 Wanlu Song , Tianyi Du , Haibin Liu , Martin B. Plenio , Jianming Cai

Distance measurements via the dipolar interaction are fundamental to the application of nuclear magnetic resonance (NMR) to molecular structure determination, but they only provide information on the absolute distance $r$ and polar angle…

Quantum Physics · Physics 2018-10-30 J. Zopes , K. Herb , K. S. Cujia , C. L. Degen

Nuclear magnetic resonance (NMR) spectroscopy has become a formidable tool for biochemistry and medicine. Although J-coupling carries essential structural information it may also limit the spectral resolution. Homonuclear decoupling remains…

Biomolecules · Quantitative Biology 2022-12-05 Tianyu Qiu , Amir Jahangiri , Xiao Han , Dmitry Lesovoy , Tatiana Agback , Peter Agback , Adnane Achour , Xiaobo Qu , Vladislav Orekhov

Studies of individual quantum systems, which have led to considerable progress in our understanding of quantum physics, have traditionally been associated with atomic gases. In the last decades however, the emphasis has shifted towards…

Materials Science · Physics 2020-11-26 J. -P. Tetienne , L. P. McGuinness , V. Jacques
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