Related papers: Proposal for Quantum Sensing Based on Two-Dimensio…
We propose a novel quantum sensing protocol that leverages the dynamical response of physical observables to quenches in quantum systems. Specifically, we use the nitrogen-vacancy (NV) color center in diamond to realize both scalar and…
The hyperpolarisation of nuclear spins within target molecules is a critical and complex challenge in magnetic resonance imaging (MRI) and nuclear magnetic resonance (NMR) spectroscopy. Hyperpolarisation offers enormous gains in signal and…
Dynamic nuclear polarization (DNP) is used in nuclear magnetic resonance (NMR) to transfer polarization from electron spins to nuclear spins. The resulting nuclear polarization enhancement can, in theory, be two or three orders of magnitude…
Methods and techniques to measure and image beyond the state-of-the-art have always been influential in propelling basic science and technology. Because current technologies are venturing into nanoscopic and molecular-scale fabrication,…
Dynamic nuclear polarization is widely used to enhance the sensitivity of nuclear magnetic resonance. It is presently the method of choice for enhancing the sensitivity of high-field solid state NMR experiments performed under cryogenic…
The spin state of two magnetically inequivalent protons in contiguous atoms of a molecule becomes entangeled by the indirect spin-spin interaction (j-coupling). The degree of entanglement oscillates at the beat frequency resulting from the…
Quantum sensing using optically addressable atomic-scale defects, such as the nitrogen--vacancy (NV) center in diamond, provides new opportunities for sensitive and highly localized characterization of chemical functionality. Notably,…
Nuclear Magnetic Resonance (NMR) spectroscopy is a cornerstone technique for determining the structures of small molecules and is especially critical in the discovery of novel natural products and clinical therapeutics. Yet, interpreting…
Modern experimental techniques can generate magnetic fields of the form H(t) = H0 z-hat + H1 [x-hat cos({\omega}t) + y-hat sin({\omega}t)], at frequencies within an order of magnitude of the nuclear magnetic resonance (NMR) and electron…
Dynamic nuclear polarization (DNP) has become a very important hyperpolarization method because it can dramatically increase the sensitivity of nuclear magnetic resonance (NMR) of various molecules. Liquid-state DNP based on Overhauser…
Optically-active solid-state systems such as self-assembled quantum dots, rare-earth ions, and color centers in diamond and SiC are promising candidates for quantum network, computing, and sensing applications. Although the nuclei in these…
Dynamic nuclear polarisation (DNP) refers to a class of techniques used to increase the signal in nuclear magnetic resonance measurements by transferring spin polarisation from ensembles of highly polarised electrons to target nuclear…
The correlations of fluctuations are key to studying fundamental quantum physics and quantum many-body dynamics. They are also useful information for understanding and combating decoherence in quantum technology. Nonlinear spectroscopy and…
We develop theoretically and demonstrate experimentally a universal dynamical decoupling method for robust quantum sensing with unambiguous signal identification. Our method uses randomisation of control pulses to suppress simultaneously…
We discuss advantages and limitations of the spin noise spectroscopy for characterization of interacting quantum dot systems on specific examples of individual singly and doubly charged quantum dot molecules (QDMs). It is shown that all the…
Entanglement and quantum discord for a pair of nuclear spins $s=1/2$ in a nanopore filled with a gas of spin-carrying molecules (atoms) are studied. The correlation functions describing dynamics of dipolar coupled spins in a nanopore are…
One of the key challenges in spectroscopy is inhomogeneous broadening that masks the homogeneous spectral lineshape and the underlying coherent dynamics. A variety of techniques including four-wave mixing and spectral hole-burning are used…
Nuclear Magnetic Resonance (NMR) spectroscopy is the cornerstone of small-molecule structure elucidation. While deep learning has demonstrated significant potential in automating structure elucidation and spectral simulation, current…
We show that it is possible to transfer two-bit information via encoding a single qubit in a conventional nuclear magnetic resonance (NMR) experiment with two very weakly polarized nuclear spins. Nevertheless, the experiment can not be…
Understanding and controlling decoherence in open quantum systems is of fundamental interest in science, while achieving long coherence times is critical for quantum information processing. Although great progress was made for individual,…