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Over the last decade, frequency-domain in-situ high-pressure nuclear magnetic resonance (NMR) spectroscopy in diamond anvil cells (DACs) has been employed as a structural and electronic probe of condensed matter systems at pressures well…

Instrumentation and Detectors · Physics 2026-01-08 Thomas Meier , Meng Yang , Yishan Zhou , Yunhua Fu , Rui Zhang , Ziliang Wang , Tianyao Zheng , Rajesh Jana , Takeshi Nakagawa

Sensing the internal dynamics of individual nuclear spins or clusters of nuclear spins has recently become possible by observing the coherence decay of a nearby electronic spin: the weak magnetic noise is amplified by a periodic,…

Quantum Physics · Physics 2016-01-05 J. E. Lang , Ren-Bao Liu , T. S. Monteiro

Reorientational dynamics-motion defined by changes in the direction of a vector or tensor-determine relaxation behavior in nuclear magnetic resonance (NMR). However, if multiple processes exist that result in reorientation, then analyzing…

Chemical Physics · Physics 2021-11-18 Albert A. Smith

Nanoscale nuclear magnetic resonance (NMR) signals can be measured through hyperfine interaction to paramagnetic electron sensor spins. A heterodyne approach is widely used to overcome the electron spin lifetime limit in spectral…

Methods for achieving quantum control and detection of individual nuclear spins by single electrons of solid-state defects play a central role for quantum information processing and nano-scale nuclear magnetic resonance (NMR). However, with…

Quantum Physics · Physics 2017-03-06 Zhen-Yu Wang , Jorge Casanova , Martin B. Plenio

Much new solid state technology for single-photon sources, detectors, photovoltaics and quantum computation relies on the fabrication of strained semiconductor nanostructures. Successful development of these devices depends strongly on…

Spin defects in solids, such as the nitrogen-vacancy (NV) center in diamond, have emerged as a key tool for detecting nuclear spins at the nanoscale. While active nuclear spin control via radio-frequency (RF) irradiation is often…

Quantum sensors have attracted broad interest in the quest towards sub-micronscale NMR spectroscopy. Such sensors predominantly operate at low magnetic fields. Instead, however, for high resolution spectroscopy, the high-field regime is…

We demonstrate a wide-band all-optical method of nanoscale magnetic resonance (MR) spectroscopy under ambient conditions. Our method relies on cross-relaxation between a probe spin, the electronic spin of a nitrogen-vacancy centre in…

Achieving atomic resolution is the ultimate limit of magnetic resonance imaging (MRI), and attaining this capability offers enormous technological and scientific opportunities, from drug development to understanding the dynamics in…

Our recent developments in in-situ nuclear magnetic resonance (NMR) spectroscopy under extreme conditions led to the observation of a wide variety of physical phenomena not accessible with standard high pressure experimental probes.…

Identifying weakly coupled nuclear spins around single electron spins is a key step of implementing quantum information processing using coupled electron-nuclei spin systems or sensing like single spin nuclear magnetic resonance detection…

Mesoscale and Nanoscale Physics · Physics 2015-01-08 Nan Zhao , Jörg Wrachtrup , Ren-Bao Liu

The ongoing miniaturization in nanoscience and -technology challenges the sensitivity and selectivity of experimental analysis methods to the ultimate level of single atoms and molecules. A promising new approach, addressed here, focuses on…

Mesoscale and Nanoscale Physics · Physics 2014-03-28 Stefan Müllegger , Stefano Tebi , Amal K. Das , Wolfgang Schöfberger , Felix Faschinger , Reinhold Koch

Resistively-detected NMR (RDNMR) is a unique characterization method enabling highly-sensitive NMR detection for a single quantum nanostructure, such as a quantum point contact (QPC). In many studies, we use dynamic nuclear polarization and…

Mesoscale and Nanoscale Physics · Physics 2022-03-09 M. H. Fauzi , T. Sobue , A. Noorhidayati , K. Sato , K. Hashimoto , Y. Hirayama

Nuclear magnetic resonance (NMR) spectroscopy is widely used in fields ranging from chemistry, material science to neuroscience. Nanoscale NMR spectroscopy using Nitrogen-vacancy (NV) centers in diamond has emerged as a promising platform…

Quantum technologies have seen a rapid developmental surge over the last couple of years. Though often overshadowed by quantum computation, quantum sensors show tremendous potential for widespread applications in chemistry and biology. One…

Quantum Physics · Physics 2022-05-30 Robin D. Allert , Karl D. Briegel , Dominik B. Bucher

We present single- and multiple-quantum correlation $J$-spectroscopy detected in zero ($<\!\!1$~$\mu$G) magnetic field using a \Rb vapor-cell magnetometer. At zero field the spectrum of ethanol appears as a mixture of \carbon isotopomers,…

Chemical Physics · Physics 2020-08-26 Tobias F. Sjolander , John W. Blanchard , Dmitry Budker , Alexander Pines

Advances in sensing devices that utilize nitrogen-vacancy (NV) center ensembles in diamond are driving progress in microscale nuclear magnetic resonance spectroscopy. Utilizing quantum sensing techniques in the high-field regime…

Quantum Physics · Physics 2025-10-22 Ainitze Biteri-Uribarren , Ana Martin , Jorge Casanova

Nuclear Magnetic Resonance (NMR) was successfully employed to test several protocols and ideas in Quantum Information Science. In most of these implementations the existence of entanglement was ruled out. This fact introduced concerns and…

Quantum Physics · Physics 2012-09-14 D. O. Soares-Pinto , R. Auccaise , J. Maziero , A. Gavini-Viana , R. M. Serra , L. C. Céleri

Scalar couplings between covalently bound nuclear spins are a ubiquitous feature in nuclear magnetic resonance (NMR) experiments, imparting valuable information to NMR spectra regarding molecular structure and conformation. Such couplings…

Chemical Physics · Physics 2011-12-26 Micah Ledbetter , Giacomo Saielli , Alessandro Bagno , Nhan Tran , Michael Romalis