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The influence of spin-orbit coupling (SOC) on the physical properties of the 5d2 system Sr2MgOsO6 is probed via a combination of magnetometry, specific heat measurements, elastic and inelastic neutron scattering, and density functional…

The so-called neutron spin resonance consists of a prominent enhancement of the magnetic response at a particular energy and momentum transfer upon entering the superconducting state of unconventional superconductors. In the case of…

Superconductivity · Physics 2019-06-21 Daniel D. Scherer , Brian M. Andersen

The role of spin-orbit coupling and Hund's rule coupling on magnetic ordering, anisotropy, and excitations are investigated within a minimal three-orbital model for the $5d^3$ compound $\rm Na Os O_3$. Asymmetry between the magnetic moments…

Strongly Correlated Electrons · Physics 2019-03-12 Avinash Singh , Shubhajyoti Mohapatra , Churna Bhandari , Sashi Satpathy

Entanglement of spin and orbital degrees of freedom drives the formation of novel quantum and topological physical states. Discovering new spin-orbit entangled ground states and emergent phases of matter requires both experimentally probing…

Strongly Correlated Electrons · Physics 2017-05-18 A. E. Taylor , S. Calder , R. Morrow , H. L. Feng , M. H. Upton , M. D. Lumsden , K. Yamaura , P. M. Woodward , A. D. Christianson

We investigate the antiferromagnetic insulating state of the recently discovered double perovskites Sr$_2$XOsO$_6$ (X$=$Sc, Mg) by using ab-initio calculations (based on Density Functional Theory and Dynamical Mean-Field Theory) to…

Strongly Correlated Electrons · Physics 2016-11-22 Gianluca Giovannetti

Magnetic anisotropy phenomena in bimetallic antiferromagnets Mn$_2$Au and MnIr are studied by first-principles density functional theory calculations. We find strong and lattice-parameter dependent magnetic anisotropies of the ground state…

We present a microscopic model for the anisotropic exchange interactions in Sr$_{2}$IrO$_{4}$. A direct construction of Wannier functions from first-principles calculations proves the $j_{\mathrm{eff}}$=1/2 character of the spin-orbit…

Strongly Correlated Electrons · Physics 2013-05-29 Hosub Jin , Hogyun Jeong , Taisuke Ozaki , Jaejun Yu

We study the low-lying excitations in 5d transition-metal oxide Sr_2IrO_4 on the localized electron picture. We find that Hund's coupling together with the spin-orbit interaction leads to exchange anisotropy which causes the spin wave gap.…

Strongly Correlated Electrons · Physics 2013-09-11 Jun-ichi Igarashi , Tatsuya Nagao

Sr$_2$FeOsO$_6$ is an insulating double perovskite compound which undergoes antiferromagnetic transitions at 140 K ($T_{N1}$) and 67 K ($T_{N2}$). To study the underlying electronic and magnetic interactions giving rise to this behavior we…

Transformation of Coulomb interaction terms to the pseudo-orbital basis constituted by $J=1/2$ and $3/2$ states arising from spin-orbit coupling provides a versatile tool. This formalism is applied to investigate magnetic anisotropy effects…

Strongly Correlated Electrons · Physics 2019-03-11 Shubhajyoti Mohapatra , Avinash Singh

To clarify a crucial role of a spin-orbit coupling in the emergence of novel spin-orbital states in $5d$-electron compounds such as Sr$_{2}$IrO$_{4}$, we investigate ground state properties of a $t_{\rm 2g}$-orbital Hubbard model on a…

Strongly Correlated Electrons · Physics 2015-06-17 Hiroaki Onishi

We determine theoretically the effect of spin-orbit coupling on the magnetic excitation spectrum of itinerant multi-orbital systems, with specific application to iron-based superconductors. Our microscopic model includes a realistic…

Superconductivity · Physics 2018-07-24 Daniel D. Scherer , Brian M. Andersen

Spin-orbit entangled magnetic dipoles, often referred to as pseudospins, provide a new avenue to explore novel magnetism inconceivable in the weak spin-orbit coupling limit, but the nature of their low-energy interactions remains to be…

We have studied the spin anisotropy in spin-singlet ground state compounds and the magnetic chirality, as measured by inelastic polarized neutron scattering techniques, in the chain-sublattice of Sr14Cu24O41. In-plane and out of plane…

Materials Science · Physics 2007-05-23 J. E. Lorenzo , C. Boullier , L. P. Regnault , U. Ammerahl , A. Revcolevschi

We propose an experiment, which would allow to pinpoint the role of spin-orbit coupling in the metal-nonmetal transition observed in a number of two-dimensional systems at low densities. Namely, we demonstrate that in a parallel magnetic…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Guang-Hong Chen , M. E. Raikh , Yong-Shi Wu

This article reviews the NMR and NQR studies on iron-based high-temperature superconductors by the IOP/Okayama group. It was found that the electron pairs in the superconducting state are in the spin-singlet state with multiple fully-opened…

Superconductivity · Physics 2012-05-31 Jie Yang , Guo-qing Zheng

The effect of the spin-orbit coupling on the ground state properties of the square-lattice three-band Hubbard model with a single electron per site is studied by a generalized Hartree-Fock approximation. We calculate the full phase diagram…

Strongly Correlated Electrons · Physics 2024-09-30 Petr A. Igoshev , Danil E. Chizhov , Valentin Yu. Irkhin , Sergey V. Streltsov

We report a neutron scattering study of the spin correlations for the spin 5/2, two-dimensional antiferromagnet Rb_2MnF_4 in an external magnetic field. Choosing fields near the system's bicritical point, we tune the effective anisotropy in…

Strongly Correlated Electrons · Physics 2009-10-31 R. L. Leheny , R. J. Christianson , R. J. Birgeneau , R. W. Erwin

The electronic ground state of Ca3LiOsO6 was recently considered within an intermediate coupling regime that revealed J=3/2 spin-orbit entangled magnetic moments. Through inelastic neutron scattering and density functional theory we…

Strongly Correlated Electrons · Physics 2017-11-29 S. Calder , D. J. Singh , V. O. Garlea , M. D. Lumsden , Y. G. Shi , K. Yamaura , A. D. Christianson

We develop anisotropic pseudo-spin antiferromagnetic Heisenberg models for monoclinically distorted double perovskites. We focus on these A$_2$BB'O$_6$ materials that have magnetic moments on the 4d or 5d transition metal B' ions, which…

Strongly Correlated Electrons · Physics 2011-12-12 Tyler Dodds , Ting-Pong Choy , Yong Baek Kim
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