Related papers: Quantum optimal control of photoelectron spectra a…
It is control that turns scientific knowledge into useful technology: in physics and engineering it provides a systematic way for driving a system from a given initial state into a desired target state with minimized expenditure of energy…
A quantum fluid dynamic control formulation is presented for optimally manipulating atomic and molecular systems. In quantum fluid dynamic the control quantum system is expressed in terms of the probability density and the quantum current.…
We present a modified optimal control scheme based on the Krotov method, which allows for strict limitations on the spectrum of the optimized laser fields, without losing monotonic convergence of the algorithm. The method guarantees a close…
We use the numerical gradient ascent method from optimal control theory to extend efficient photon storage in Lambda-type media to previously inaccessible regimes and to provide simple intuitive explanations for our optimization techniques.…
Inhomogeneity, in its many forms, appears frequently in practical physical systems. Readily apparent in quantum systems, inhomogeneity is caused by hardware imperfections, measurement inaccuracies, and environmental variations, and…
We develop photoelectron interferometry based on laser-assisted extreme ultraviolet ionization for flexible and robust control of photoelectron circular dichroism in randomly oriented chiral molecules. A comb of XUV photons ionizes a sample…
We address the problem of reshaping light in the Schr\"odinger optics regime from the perspective of optimal control theory. In technological applications, Schr\"odinger optics is often used to model a slowly-varying amplitude of a…
Using a quantum wave packet simulation including the nuclear and electronic degrees of freedom, we investigate the femtosecond and picosecond energy- and angle-resolved photoelectron spectra of the E($^1\Sigma_g^+$) electronic state of…
A new concept of the molecular structure optimization method based on quantum dynamics computations is presented. Nuclei are treated as quantum mechanical particles, as are electrons, and the many-body wave function of the system is…
High-order harmonic generation (HHG), characterized by its highly nonlinear nature, often exhibits a complex spatio-temporal profile that poses challenges for practical applications. In this study, we unveil a method for manipulating the…
Most photocatalytic and photovoltaic devices operate under broadband, constant illumination. Electron and hole dynamics in these devices, however, are usually measured using ultrafast pulsed lasers in a narrow wavelength range. In this…
A theoretical optimization method of high-harmonic-generation (HHG) is developed in the framework of optimal-control-theory (OCT). The target of optimization is the emission radiation of a particular frequency. The OCT formulation includes…
The method of direct neutrino mass determination based on the kinematics of tritium beta decay, which is adopted by the KATRIN experiment, makes use of a large, high-resolution electrostatic spectrometer with magnetic adiabatic collimation.…
We apply theoretically open-loop quantum optimal control techniques to provide methods for the verification of various quantum coherent transport mechanisms in natural and artificial light-harvesting complexes under realistic experimental…
The angular distribution of the emitted electrons, following the two-photon ionization of the hydrogen-like ions, is studied within the framework of second order perturbation theory and the Dirac equation. Using a density matrix approach,…
We investigate the possibilities of preserving and manipulating the coherence of atomic two-level systems by ideal projective homodyne detection and feedback. For this purpose, the photon emission process is described on time scales much…
We use three dimensional time-dependent Schr\"odinger equation (3D--TDSE) to calculate angular electron momentum distributions and photoelectron spectra of atoms driven by spatially inhomogeneous fields. An example for such inhomogeneous…
A new method for controlling harmonic generation, in the framework of quantum optimal control theory (QOCT), is developed. The problem is formulated in the frequency domain using a new maximization functional. The relaxation method is used…
Nonlinear Thomson scattering of an electron motion in a combining field constituted by an elliptically polarized laser and a background magnetic field is investigated. The dependence of the electron trajectories, the fundamental frequency,…
The single ionization of noble gas atoms by the combined action of XUV attopulses and an infrared laser field is theoretically investigated by means of a non-perturbative model that under certain approximations gives closed-form expressions…