Related papers: Stochastic stimulated electronic x-ray Raman spect…
A quantum-mechanical model to calculate the electron energy-loss spectra (EELS) for the system of a closely located metallic nanoshell and a molecule has been developed. At the resonance between the molecular excitation and plasmon modes in…
A deep understanding of molecular photo-transformations is challenging because of the complex interaction between the configurations of electrons and nuclei. An initial optical excitation dissipates energy into electronic and structural…
This project explores the design and development of a transition edge sensor (TES) spectrometer for resonant soft X- ray scattering (RSXS) measurements developed in collaboration between Argonne National Laboratory (ANL) and the National…
In order to carry out inelastic X-ray scattering (IXS) experiment at BL15U1 beamline of Shanghai Synchrotron Radiation Facility (SSRF), the data acquisition and control system based on SPEC software has been developed. The IXS experimental…
We analyze the resonant x-ray scattering (RIXS) spectra from Sr$_2$IrO$_4$ in an itinerant electron approach. Employing a multi-orbital tight-binding model on the square lattice, we calculate the one-electron energy band within the…
Regularized imaging spectroscopy was introduced for the construction of electron flux images at different energies from count visibilities recorded by the Reuven Ramaty High Energy Solar Spectroscopic Imager (RHESSI). In this work we seek…
Stimulated Raman scattering, employing a pump and a Stokes beam, exhibits itself through both the Raman loss observed in the pump beam and the Raman gain in the Stokes beam. This phenomenon finds application in spectroscopy for chemical…
This paper reviews non-resonant meV-resolved inelastic x-ray scattering (IXS) as a complementary method to inelastic neutron scattering (INS). Two aspects of IXS that are notable in this context are (1) that IXS allows straightforward…
Advances in our ability to understand and utilize the world around us have always relied on the development of advanced tools for probing and manipulating materials properties. X-ray matter interactions played a critical role in the…
Resonant inelastic x-ray scattering (RIXS) spectra at the Fe K-edge were measured for a single crystal of the iron oxypnictide superconductor PrFeAsO0.7 (Tc=42 K). They disclose a weak, broad feature centered around 4.5 eV energy loss,…
Inelastic x-ray scattering (IXS) with very high (meV) energy resolution has become a valuable spectroscopic tool, complementing the well established coherent inelastic neutron scattering (INS) technique for phonon dispersion investigations.…
Using a quantum electrodynamic framework, we calculate the off-resonant scattering of a broad-band X-ray pulse from a sample initially prepared in an arbitrary superposition of electronic states. The signal consists of single-particle…
Resonant inelastic x-ray scattering (RIXS) at the copper K absorption edge has been performed for heavily overdoped samples of La$_{2-x}$Sr$_{x}$CuO$_{4}$ with $x= 0.25$ and 0.30. We have observed the charge transfer and molecular-orbital…
X-ray free electron lasers (X-FELs) present new opportunities to study ultrafast lattice dynamics in complex materials. While the unprecedented source brilliance enables high fidelity measurement of structural dynamics, it also raises…
Understanding the complex plasma dynamics in ultra-intense relativistic laser-solid interactions is of fundamental importance to the applications of laser plasma-based particle accelerators, creation of high energy-density matter,…
X-ray free-electron lasers (FELs) are promising tools for structural determination of macromolecules via coherent x-ray scattering. During ultrashort and ultraintense x-ray pulses with an atomic scale wavelength, samples are subject to…
We present a time-dependent Schr\"odinger equation (TDSE) approach within a non-relativistic quantum electrodynamics (QED) framework to investigate resonant x-ray scattering under intense x-ray pulses. This method enables us to explore how…
Nonresonant inelastic x-ray scattering (NIXS) is a possible tool to detect charge excitations in electron systems. In addition, multipole transitions at high-momentum-transfer region open a new possibility to determine orbital-selective…
Raman scattering, an inelastic scattering mechanism, provides information about molecular excitation energies and can be used to identify chemical compounds. Albeit being a powerful analysis tool, especially for label-free biomedical…
We measure the resonant forward scattering of light by a highly saturated atomic medium through the flashes emitted immediately after an abrupt extinction of the probe beam. The experiment is done in a dilute regime where the phenomena are…