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Investigating electronic structure and excitations under extreme conditions gives access to a rich variety of phenomena. High pressure typically induces behavior such as magnetic collapse and the insulator-metal transition in 3d transition…

Strongly Correlated Electrons · Physics 2017-09-27 Jean-Pascal Rueff , Abhay Shukla

Resonant elastic x-ray scattering (REXS) is an exquisite element-sensitive tool for the study of subtle charge, orbital, and spin superlattice orders driven by the valence electrons, which therefore escape detection in conventional x-ray…

We propose a novel way to image dynamical properties of nonstationary electron systems using ultrafast resonant x-ray scattering. Employing a rigorous theoretical analysis within the framework of quantum electrodynamics, we demonstrate that…

Atomic Physics · Physics 2017-11-03 Daria Popova-Gorelova , Robin Santra

We explore the general phenomenology of resonant inelastic scattering (RIXS) using CuB2O4, a network of CuO4 plaquettes electronically isolated by B+3 ions. Spectra show a small number of well-separated features, and we exploit the simple…

Strongly Correlated Electrons · Physics 2013-05-29 J. N. Hancock , G. Chabot-Couture , Y. Li , G. Petrakovskii , K. Ishii , I. Jarrige , J. Mizuki , T. P. Devereaux , M. Greven

X-ray echo spectroscopy, a space-domain counterpart of neutron spin echo, is a recently proposed inelastic x-ray scattering (IXS) technique. X-ray echo spectroscopy relies on imaging IXS spectra, and does not require x-ray…

Optics · Physics 2017-08-04 Yuri Shvyd'ko

We have performed resonant inelastic x-ray scattering (RIXS) near the Cu-K edge on cuprate superconductors La(2-x)Sr(x)CuO(4), La(2-x)Ba(x)CuO(4), La(2-x)Sr(x)Cu(1-y)Fe(y)O(4) and Bi(1.76)Pb(0.35)Sr(1.89)CuO(6+d), covering underdoped to…

Superconductivity · Physics 2015-06-15 S. Wakimoto , K. Ishii , H. Kimura , K. Ikeuchi , M. Yoshida , T. Adachi , D. Casa , M. Fujita , Y. Fukunaga , T. Gog , Y. Koike , J. Mizuki , K. Yamada

Resonant inelastic X-ray scattering (RIXS) spectra of model copper- and nickel-based transition metal oxides are measured over a wide range of energies near the M-edge (h$\nu$=60-80eV) to better understand the properties of resonant…

Strongly Correlated Electrons · Physics 2012-11-20 L. Andrew Wray , Wanli Yang , Hiroshi Eisaki , Zahid Hussain , Yi-De Chuang

We study the magnetic excitation spectra of resonant inelastic x-ray scattering (RIXS) at the $L$-edge from undoped cuprates beyond the fast collision approximation. We analyse the effect of the symmetry breaking ground state on the RIXS…

Strongly Correlated Electrons · Physics 2015-06-24 Jun-ichi Igarashi , Tatsuya Nagao

X-ray Free Electron Lasers (XFELs) have been proven to generate short and powerful radiation pulses allowing for a wide class of novel experiments. If an XFEL facility supports the generation of two X-ray pulses with different wavelengths…

Accelerator Physics · Physics 2017-06-05 Gianluca Geloni , Vitali Kocharyan , Tommaso Mazza , Michael Meyer , Evgeni Saldin , Svitozar Serkez

We review the current state of efforts to use resonant soft x-ray scattering (RSXS), which is an elastic, momentum-resolved, valence band probe of strongly correlated electron systems, to study stripe-like phenomena in copper-oxide…

Strongly Correlated Electrons · Physics 2015-06-03 Peter Abbamonte , Eugene Demler , J. C. Seamus Davis , Juan-Carlos Campuzano

The real-space multiple-scattering (RSMS) approach is applied to model non-resonant inelastic scattering from deep core electron levels over a broad energy spectrum. This approach is applicable to aperiodic or periodic systems alike and…

Other Condensed Matter · Physics 2009-11-11 J. A. Soininen , A. L. Ankudinov , J. J. Rehr

We have investigated the local low-energy excitations in CeRu$_4$Sn$_6$, a material discussed recently in the framework of strongly correlated Weyl semimetals, by means of Ce $M_5$ resonant inelastic x-ray scattering (RIXS). The…

We study theoretically resonant inelastic x-ray scattering (RIXS) at the Cu $L_3$-edge in a typical parent compound of high-$T_c$ cuprate superconductors La$_2$CuO$_4$ on the basis of a detailed electronic band structure. We construct a…

Strongly Correlated Electrons · Physics 2015-08-20 Takuji Nomura

We study a nonlinear Schr\"odinger equation which arises as an effective single particle model in X-ray Free Electron Lasers (XFEL). This equation appears as a first-principles model for the beam-matter interactions that would take place in…

Numerical Analysis · Mathematics 2014-06-18 Paolo Antonelli , Agissilaos Athanassoulis , Zhongyi Huang , Peter A. Markowich

We present a theoretical investigation of the origin of Raman-like and fluorescencelike (FL) features of resonant inelastic x-ray scattering (RIXS) spectra. Using a combination of local-density approximation + dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2018-09-26 Atsushi Hariki , Mathias Winder , Jan Kuneš

We calculate the K-edge indirect bimagnon resonant inelastic X-ray scattering (RIXS) intensity spectra of the bicollinear antiferromagnetic order known to occur in the $\alpha$-FeTe chalcogenide system. Utilizing linear spin wave theory for…

Materials Science · Physics 2017-11-28 Zengye Huang , Sean Mongan , Trinanjan Datta , Dao-Xin Yao

We present a computational study of $L$-edge resonant inelastic x-ray scattering (RIXS) in correlated 3$d$ transition-metal oxides using an $ab$ $initio$ method based on local density approximation + dynamical mean-field theory (DMFT). The…

Strongly Correlated Electrons · Physics 2020-03-25 Atsushi Hariki , Mathias Winder , Takayuki Uozumi , Jan Kuneš

Interactions between electrons and lattice vibrations are responsible for a wide range of material properties and applications. Recently, there has been considerable interest in the development of resonant inelastic x-ray scattering (RIXS)…

We investigate resonant inelastic X-ray scattering (RIXS) at the O $K$-edge in insulating cuprates by means of three methods: cluster perturbation theory (CPT), Hartree--Fock approximation (HFA) and exact diagonalization (ED) method. We…

Strongly Correlated Electrons · Physics 2023-02-22 Yukihiro Matsubayashi , Sumio Ishihara

X-ray spectroscopy has been a key method to determine ground and excited state properties of quantum materials with atomic specificity. Now, new x-ray facilities are opening the door to the study of pump-probe x-ray spectroscopy -…

Strongly Correlated Electrons · Physics 2025-02-11 Daniel Jost , Eder G. Lomeli , Ta Tang , Joshua J. Kas , John J. Rehr , Wei-Sheng Lee , Hong-Chen Jiang , Brian Moritz , Thomas P. Devereaux
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