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Organic molecules have recently gained attention as novel sources of single photons. We present a joint experiment--theory analysis of the temperature-dependent emission spectra, zero-phonon linewidth, and second-order correlation function…

We devise a theory of adsorption of low-energy atoms on suspended graphene membranes maintained at 10 K based on a model of atom-acoustic phonon interactions. Our primary technique includes a non-perturbative method which treats the…

Mesoscale and Nanoscale Physics · Physics 2020-01-06 Sanghita Sengupta

First-principles prediction of thermal conductivity and radiative properties is crucial. However, computing phonon scattering, especially for four-phonon scattering, could be prohibitively expensive, and the thermal conductivity even for…

Materials Science · Physics 2023-11-23 Ziqi Guo , Zherui Han , Dudong Feng , Guang Lin , Xiulin Ruan

We present a method for computing optical absorption spectra by means of a Bethe-Salpeter equation approach, which is based on a conserving linear response calculation for electron-hole coherences in the presence of an external…

Materials Science · Physics 2010-12-21 George Pal , Yaroslav Pavlyukh , Wolfgang Hübner , Hans Christian Schneider

Discovery of high-performance materials remains one of the most active areas in photovoltaics (PV) research. Indirect band gap materials form the largest part of the semiconductor chemical space, but predicting their suitability for PV…

We have combined the Boltzmann transport equation with an {\it ab initio} approach to compute the thermoelectric coefficients of semiconductors. Electron-phonon, ionized impurity, and electron-plasmon scattering rates have been taken into…

Materials Science · Physics 2018-10-26 Z. Wang , S. Wang , S. Obukhov , N. Vast , J. Sjakste , V. Tyuterev , N. Mingo

Results from four different approximations to the phonon-assisted quantum adsorption rate for cold atoms on a 2D material are compared and contrasted: (1) a loop expansion (LE) based on the atom-phonon coupling, (2) non-crossing…

Mesoscale and Nanoscale Physics · Physics 2018-12-18 Sanghita Sengupta , Dennis P. Clougherty

While using first-principles-based Boltzmann transport equation approach to predict the thermal conductivity of crystalline semiconductor materials has been a routine, the validity of the approach is seldom tested for high-temperature…

Mesoscale and Nanoscale Physics · Physics 2020-03-05 Xiaokun Gu , Shouhang Li , Hua Bao

We present a simple measurement and analysis technique to determine the fraction of optical loss due to both radiation (scattering) and linear absorption in microphotonic components. The method is generally applicable to optical materials…

Optics · Physics 2009-11-13 Matthew Borselli , Thomas J. Johnson , Oskar Painter

We develop an analytical model to describe sub-bandgap optical absorption in two-dimensional semiconducting transition metal dichalcogenide (s-TMD) nanoflakes. The material system represents an array of few-layer molybdenum disulfide…

Mesoscale and Nanoscale Physics · Physics 2016-10-11 Maxim Trushin , Edmund J. R. Kelleher , Tawfique Hasan

We calculate, as a function of temperature and conduction band electron density, the optical absorption of a weakly n-doped, idealized semiconductor quantum well. In particular, we focus on the absorption band due to the formation of a…

Strongly Correlated Electrons · Physics 2009-11-07 F. X. Bronold

Because of its low-cost, silicon is the standard material for photovoltaic conversion. Yet, its band-edge absorption spectrum is narrower than the spectrum of the solar radiation, which reduces its conversion efficiency. In this paper, it…

Applied Physics · Physics 2019-06-13 Valerio Apicella , Teslim Ayinde Fasasi , Antonio Ruotolo

For a one-dimensional electron-phonon system we consider the photon absorption involving electronic excitations within the pseudogap energy range. Within the adiabatic approximation for the electron - phonon interactions these processes are…

Strongly Correlated Electrons · Physics 2009-11-07 S. I. Matveenko , S. A. Brazovskii

For a one-dimensional electron-phonon system we consider the photon absorption involving electronic excitations within the pseudogap energy range. In the framework of the adiabatic approximation for the electron - phonon interactions these…

Strongly Correlated Electrons · Physics 2007-05-23 S. I. Matveenko , S. Brazovskii

The use of cryogenic silicon as a detector medium for dark matter searches is gaining popularity. Many of these searches are highly dependent on the value of the photoelectric absorption cross section of silicon at low temperatures,…

We present results for the optical absorption spectra of small-diameter single-wall carbon and boron nitride nanotubes obtained by {\it ab initio} calculations in the framework of time-dependent density functional theory. We compare the…

Materials Science · Physics 2010-07-01 A. G. Marinopoulos , Ludger Wirtz , Andrea Marini , Valerio Olevano , Angel Rubio , Lucia Reining

The photosensitivity of silicon is inherently very low in the visible electromagnetic spectrum, and it drops rapidly beyond 800 nm in near-infrared wavelengths. Herein, we have experimentally demonstrated a technique utilizing…

The optical properties of polarons are studied in the framework of the Holstein model by applying the dynamical mean-field theory. This approach allows to enlighten important quantitative and qualitative deviations from the limiting…

Strongly Correlated Electrons · Physics 2009-11-11 S. Fratini , S. Ciuchi

We report a photoluminescence study of high-quality Ge samples at temperatures 12 K $\leq$ T $\leq$ 295 K, over a spectral range that covers phonon-assisted emission from the indirect gap (between the lowest conduction band at the L point…

Materials Science · Physics 2020-05-28 José Menéndez , Christian D. Poweleit , Sean E. Tilton

The Allen-Heine-Cardona theory allows us to calculate phonon-induced electron self-energies from first principles without resorting to the adiabatic approximation. However, this theory has not been able to account for the change of the…

Materials Science · Physics 2024-10-17 Jae-Mo Lihm , Cheol-Hwan Park