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We argue that the experimentally easily accessible optical absorption spectrum can often be used to distinguish between a random alloy phase and a stoichiometrically equivalent core/shell realization of ensembles of monodisperse colloidal…

Chemical Physics · Physics 2017-09-13 Daniel Mourad

The role of electron-phonon scattering in finite-temperature anomalous Hall effect is still poorly understood. In this work, we present a Boltzmann theory for the side-jump contribution from electron-phonon scattering, which is derived from…

Mesoscale and Nanoscale Physics · Physics 2019-07-03 Cong Xiao , Ying Liu , Ming Xie , Shengyuan A. Yang , Qian Niu

We present a general harmonic theory for the temperature dependence of phonon-renormalized properties of solids. Firstly, we formulate a perturbation theory in phonon-phonon interactions to calculate the phonon renormalization of physical…

Materials Science · Physics 2015-10-28 Bartomeu Monserrat , G. J. Conduit , R. J. Needs

Topological insulator films are promising materials for optoelectronics due to a strong optical absorption and a thickness dependent band gap of the topological surface states. They are superior candidates for photodetector applications in…

Mesoscale and Nanoscale Physics · Physics 2018-09-11 Mathias Rosdahl Brems , Jens Paaske , Anders Mathias Lunde , Morten Willatzen

Optical transitions in a semiconductor quantum dot are theoretically investigated, with emphasis on the coupling to longitudinal optical phonons, and including excitonic effects. When limiting to a finite number of $m$ electron and $n$ hole…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 T. Stauber , R. Zimmermann

A comprehensive picture of polaron and bipolaron physics is essential to understand the optical absorption spectrum in many materials with electron-phonon interactions. In particular, the finite-temperature properties are of interest since…

Strongly Correlated Electrons · Physics 2022-10-27 David Jansen , Janez Bonča , Fabian Heidrich-Meisner

We describe a theoretical framework for the interpretation of time-resolved phonon absorption experiments carried out in the fractional quantum Hall regime of a magnetically quantized two-dimensional electron system (2des). The only phonons…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Keith A. Benedict , R. K. Hills , C. J. Mellor

We perform linear and non-linear photon absorption calculations in topological insulator ultra-thin films on a substrate. Due to the unique band structure of the coupled topological surface states, novel features are observed for suitable…

Mesoscale and Nanoscale Physics · Physics 2013-11-18 Jing Wang , Hideo Mabuchi , Xiao-Liang Qi

The effects of chemical disorder on the electronic and optical properties of semiconductor alloy multilayers are studied based on the tight-binding theory and single-site coherent potential approximation. Due to the quantum confinement of…

Mesoscale and Nanoscale Physics · Physics 2010-06-03 Alireza Saffarzadeh , Leili Gharaee

We develop a computational framework, based on the Boltzmann transport equation, with the ability to compute the thermal transport in nanostructured materials of any geometry using as the only input the bulk thermal conductivity…

Mesoscale and Nanoscale Physics · Physics 2014-10-20 Giuseppe Romano , Jeffrey C. Grossman

Temperature influences the performance of two-dimensional materials in optoelectronic devices. Indeed, the optical characterization of these materials is usually realized at room temperature. Nevertheless most {\it ab-initio} studies are…

Mesoscale and Nanoscale Physics · Physics 2016-06-06 Alejandro Molina-Sánchez , Maurizia Palummo , Andrea Marini , Ludger Wirtz

The electron-phonon interaction contribution to the electronic energies is included in density functional total energy calculations with ab initio pseudopotentials via the Allen formalism [Phys. Rev. B 18, 5217 (1978)] to obtain temperature…

Materials Science · Physics 2018-02-21 Vaishali Shah , Bhavik Sanghavi , Rahul Ramchandani , M. P. Gururajan , T. R. S. Prasanna

We present a non-Hermitian theory of atomic and molecular absorption, which enables computing the absorption spectrum of multi-electron atoms and molecules without using any fitting parameters. We propose a method for optically inducing…

Chemical Physics · Physics 2019-04-02 Adi Pick , Petra Ruth Kaprálová-Žďánská , Nimrod Moiseyev

We describe a method for calculating the probability with which the wall of a plasma absorbs an electron at low energy. The method, based on an invariant embedding principle, expresses the electron absorption probability as the probability…

Plasma Physics · Physics 2017-01-10 Franz X. Bronold , Holger Fehske

From ultraviolet to mid-infrared region, light-matter interaction mechanisms in semiconductors progressively shift from electronic transitions to phononic resonances and are affected by temperature. Here, we present a parallel…

Optics · Physics 2023-06-01 Zherui Han , Changkyun Lee , Jiawei Song , Haiyan Wang , Peter Bermel , Xiulin Ruan

The frequency-dependent conductivity is studied for the one-dimensional Hubbard model, using a selection rule, the Bethe ansatz, and symmetries associated with conservation laws. For densities where the system is metallic the absorption…

Strongly Correlated Electrons · Physics 2009-10-31 J. M. P. Carmelo , N. M. R. Peres , P. D. Sacramento

The optical absorption of a many (continuum) polaron gas is derived in the framework of a variational approach at zero temperature and weak or intermediate electron-phonon coupling strength. We derive a compact formula for the optical…

Strongly Correlated Electrons · Physics 2009-10-31 J. Tempere , J. T. Devreese

We present exact results for the optical response in the one-dimensional Holstein model. In particular, by means of a refined kernel polynomial method, we calculate the ac and dc electrical conductivities at finite temperatures for a wide…

Strongly Correlated Electrons · Physics 2007-05-23 G. Schubert , G. Wellein , A. Weiße , A. Alvermann , H. Fehske

We present a fully first-principles method for superconducting thin films. The layer dependent phonon spectrum is calculated to determine the layer dependence of the electron-phonon coupling for such systems, which is coupled to the…

Superconductivity · Physics 2016-10-19 Gábor Csire , Stephan Schönecker , Balázs Újfalussy

We present a systematic study of the photo-absorption spectra of various Si$_{n}$H$_{m}$ clusters (n=1-10, m=1-14) using the time-dependent density functional theory (TDDFT). The method uses a real-time, real-space implementation of TDDFT…

Mesoscale and Nanoscale Physics · Physics 2012-02-29 Juzar Thingna , R. Prasad , S. Auluck