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We study the electron-energy loss spectra of strongly correlated electronic systems doped away from half-filling using dynamical mean-field theory ($d=\infty$). The formalism can be used to study the loss spectra in the optical (${\bf…

Strongly Correlated Electrons · Physics 2009-10-31 Luis Craco , Mukul S. Laad

Transition-edge sensors (TESs) have the potential to perform electron spectroscopic measurements with far greater measurement rates and efficiencies than can be achieved using existing electron spectrometers. Existing spectrometers filter…

Instrumentation and Detectors · Physics 2024-03-05 K. M. Patel , S. Withington , A. G . Shard , D. J. Goldie , C. N. Thomas

Scanning Transmission Electron Microscopy (STEM) offers high-resolution images that are used to quantify the nanoscale atomic structure and composition of materials and biological specimens. In many cases, however, the resolution is limited…

Signal Processing · Electrical Eng. & Systems 2021-12-23 Daniel Nicholls , Alex Robinson , Jack Wells , Amirafshar Moshtaghpour , Mounib Bahri , Angus Kirkland , Nigel Browning

Focusing electromagnetic energy to sub-wavelength dimensions has become an increasingly active field of research for a variety of applications such as Heat Assisted Magnetic Recording (HAMR), nanolithography, and nanoscale optical…

Cathodoluminescence (CL) microscopy has emerged as a powerful tool for investigating the optical properties of materials at the nanoscale, offering unique insights into the behavior of photonic and plasmonic materials under electron…

Focused beams of electrons, which act as both sources, and sensors of electric fields, can be used to characterise the electric response of complex photonic systems by locally probing the induced optical near fields. This functionality can…

In this paper we provide a mathematical framework for localized plasmon resonance of nanoparticles. Using layer potential techniques associated with the full Maxwell equations, we derive small-volume expansions for the electromagnetic…

Mathematical Physics · Physics 2015-10-28 Habib Ammari , Youjun Deng , Pierre Millien

Noble metal nanoparticles show specific optical properties due to the excitation of localized surface plasmons that make them attractive candidates for highly sensitive bionanosensors. The underlying physical principle is either an…

Atomically resolved electron energy-loss spectroscopy experiments are commonplace in modern aberrationcorrected transmission electron microscopes. Energy resolution has also been increasing steadily with the continuous improvement of…

Materials Science · Physics 2014-03-10 R. Egoavil , N. Gauquelin , G. T. Martinez , S. Van Aert , G. Van Tendeloo , J. Verbeeck

Electron-boson coupling is central to a comprehensive understanding of the diverse physical phenomena emerging from many-body interactions. Yet less attention has been paid to how plasmons, collective bosonic modes of electron density…

Electron energy-loss spectroscopy (EELS) and cathodoluminescence (CL) are widely used experimental techniques for characterization of nanoparticles. The discrete dipole approximation (DDA) is a numerically exact method for simulating…

Optics · Physics 2023-03-03 Alexander A. Kichigin , Maxim A. Yurkin

Surface and volume plasmons excited in a metal cluster by moving electron and corresponding inelastic scattering spectra are studied based on the hydrodynamic approach. Along with the bulk losses traditionally taken into account, the…

Plasma Physics · Physics 2016-04-20 V. B. Gildenburg , V. A. Kostin , I. A. Pavlichenko

Aberration-corrected environmental transmission electron microscopy (ETEM) enables atomic-resolution imaging of dynamic catalytic processes. Correlating atomic-scale structural changes with reaction products detected by mass spectrometry…

Particle plasmons in metal nanoparticles have primarily been investigated through the use of local optical response approximations. However, as nanoparticle size approaches the average distance of electrons to the metal surface, mesoscopic…

Optics · Physics 2023-06-28 Weixiang Ye

Precise control of light-matter interactions at the nanoscale lies at the heart of nanophotonics. Experimental examination at this length scale is challenging, however, since the corresponding electromagnetic near-field is often confined…

Metal nanoparticle surfaces comprise of multiple planes with various atomic arrangements that interact with gases differently1,2. Identification of gas adsorption properties on all facets is an essential prerequisite for rational design of…

Materials Science · Physics 2015-07-28 Pin Ann Lin , Jonathan Winterstein , John Kohoutek , Henri Lezec , Renu Sharma

The next generation of ultra-low-noise cryogenic detectors for space science applications require continued exploration of materials characteristics at low temperatures. The low noise and good energy sensitivity of current Transition Edge…

Mesoscale and Nanoscale Physics · Physics 2011-02-01 D. J. Goldie , D. M. Glowacka , K. Rostem† , S. Withington

Reflection electron energy loss spectroscopy (EELS) in specular and off specular geometry has been employed to study the early stage of the copper phthalocyanine (CuPc) growth on Al (100) substrate. EEL spectroscopy has been a useful tool…

Materials Science · Physics 2009-11-10 A. Ruocco , M. P. Donzello , F. Evangelista , G. Stefani

Metasurfaces offer great potential to control near- and far-fields through engineering of optical properties of elementary cells or meta-atoms. Such perspective opens a route to efficient manipulation of the optical signals both at…

We demonstrate spatially-resolved measurements of spontaneous and stimulated electron-photon interactions in nanoscale optical near fields using electron energy-loss spectroscopy (EELS), cathodoluminescence spectroscopy (CL), and…