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The electronic and phonon transport properties of quaternary tetradymite BiSbSeTe2 are investigated using first-principles approach and Boltzmann transport theory. Unlike the binary counterpart Bi2Te3, we obtain a pair of Rashba splitting…

Materials Science · Physics 2018-08-01 Z. Z. Zhou , H. J. Liu , D. D. Fan , B. Y. Zhao , C. Y. Sheng , G. H. Cao , S. Huang

Recent discovery of new materials for thermoelectric energy conversion is enabled by efficient prediction of materials' performance from first-principles, without empirically fitted parameters. The novel simplified approach for computing…

Materials Science · Physics 2018-05-02 Georgy Samsonidze , Boris Kozinsky

Heat transfer in layered metal-dielectric structures is considered theoretically based on an analytical solution of the Boltzmann transfer equation for the phonon distribution function. Taking into account the size effect, the problem of…

Materials Science · Physics 2023-11-27 A. I. Bezuglyj , I. V. Mironenko , V. A. Shklovskij

We theoretically investigate the thermoelectric properties of semiconducting (gapped) materials by varying the degrees of polynomials in their energy dispersion relations, in which either the valence or conduction energy dispersion depends…

The layered misfit cobaltate Ca$_3$Co$_4$O$_9$, also known as Ca$_2$CoO$_3$[CoO$_2$]$_{1.62}$, is a promising p-type thermoelectric oxide. Employing density functional theory, we study its electronic structure and determine, on the basis of…

Materials Science · Physics 2017-06-13 Bin Amin , Ulrich Eckern , Udo Schwingenschlögl

To increase the performance of thermoelectric materials, the electronic parameters in the figure of merit must be improved. In this paper, we use full, numerical band structures and solve the Boltzmann equation in the relaxation time…

Materials Science · Physics 2018-12-17 Evan Witkoske , Xufeng Wang , Jesse Maassen , Mark Lundstrom

We report a combined theoretical and experimental search for thermoelectric materials based on semiconducting zinc antimony. Influence of three new doping elements (sodium, potassium and boron) on the electronic properties is investigated…

Materials Science · Physics 2014-08-27 K Niedziolka , R Pothin , F Rouessac , R M Ayral , P Jund

We present first principles study of thermoelectric transport properties of sandwiched heterostructure of Graphene (G)/hexagonal Boron Nitride (BN)/G, based on Boltzmann transport theory for band electrons using the bandstructure calculated…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 Ransell D'Souza , Sugata Mukherjee

The thermoelectric properties of halide perovskites $\mathrm{CsMI_3}$ (M=Sn and Pb) are investigated from a combination of first-principles calculations and semiclassical Boltzmann transport theory by considering both the electron and…

Materials Science · Physics 2016-05-31 San-Dong Guo , Jian-Li Wang

Materials with reduced dimensionality offer beneficial density-of-states (DOS) profiles for thermoelectric energy conversion, but can be impractical in realistic devices. Encouragingly, bulk high-symmetry materials can also exhibit similar…

Materials Science · Physics 2026-03-10 Øven A. Grimenes , Ole M. Løvvik , Kristian Berland

In this work, we have investigated the electronic structure and thermoelectric properties of quaternary heusler alloy, FeRuTiSi, using first principle DFT tools implemented in WIEN2k and BoltzTraP code. Electronic structure calculations…

Strongly Correlated Electrons · Physics 2020-12-02 Saurabh Singh , Shubham Singh , Nitinkumar Bijewar , Ashish Kumar

We study the electronic transport coefficients and the thermoelectric figure of merit ZT in $n$-doped Mg$_3$Sb$_2$ based on density-functional electronic structure and Bloch-Boltzmann transport theory with an energy- and…

Materials Science · Physics 2019-01-07 Roberta Farris , Maria Barbara Maccioni , Alessio Filippetti , Vincenzo Fiorentini

We present ab initio electronic structure calculations based on density functional theory for the thermoelectric properties of Bi$_2$Te$_3$ films. Conductivity and thermopower are computed in the diffusive limit of transport based on the…

Materials Science · Physics 2014-02-04 F. Rittweger , N. F. Hinsche , P. Zahn , I. Mertig

Using first-principles pseudopotential method and Boltzmann transport theory, we give a comprehensive understanding of the electronic and phonon transport properties of thermoelectric material BiCuSeO. By choosing proper hybrid functional…

Materials Science · Physics 2017-06-28 D. D. Fan , H. J. Liu , L. Cheng , J. Zhang , P. H. Jiang , J. Wei , J. H. Liang , J. Shi

We report on the elaboration of germanium manganese nanostructured thin films and the measurement of their thermoelectric properties. We investigate the growth of Ge:Mn layers along with a thorough structural characterization of this…

Thermoelectric effects enable the direct conversion between thermal and electrical energy and provide an alternative route for power generation and refrigeration. The clathrate Ba8Ga16Ge30 has the highest figure of merit (ZT ~ 1) among…

Materials Science · Physics 2011-11-16 Deepa Kasinathan , Vicente Pacheco-Espejel , Helge Rosner

In Peierls-distorted materials, photoexcitation leads to a strongly coupled transient response between structural and electronic degrees of freedom, always measured independently of each other. Here we use transient reflectivity in the…

We compute both electron- and phonon transmissions in thin disordered silicon nanowires. Our atomistic approach is based on tight-binding and empirical potential descriptions of the electronic and phononic systems, respectively. Surface…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Troels Markussen , Antti-Pekka Jauho , Mads Brandbyge

We study the thermoelectric properties of three-dimensional topological Anderson insulators with line dislocations. We show that at high densities of dislocations the thermoelectric figure of merit ZT can be dominated by one-dimensional…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Oleg A. Tretiakov , Ar. Abanov , Shuichi Murakami , Jairo Sinova

The thermoelectric properties of 1.6 nm-thick Si square nanowires with [100] crystalline orientation are calculated over a wide temperature range from 0 K to 1000 K, taking into account atomistic electron-phonon interaction. In our model,…

Mesoscale and Nanoscale Physics · Physics 2019-09-27 Igor Bejenari , Peter Kratzer