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We use first-principles electronic structure methods to calculate the electronic thermoelectric properties (i.e. due to electronic transport only) of single-crystalline bulk $n$-type silicon-germanium alloys vs Ge composition, temperature,…

Materials Science · Physics 2025-02-03 F. Murphy-Armando

The thermoelectric properties of 54 different group 4 half-Heusler (HH) alloys have been studied from first principles. Electronic transport was studied with density functional theory using hybrid functionals facilitated by the $\mathbf{k}…

Materials Science · Physics 2020-01-08 Kristian Berland , Nina Shulumba , Olle Hellman , Clas Persson , Ole Martin Løvvik

Motivated by recent experimental realizations of quintuple atomic layer films of Bi2Te3,the thermoelectric figure of merit, ZT, of the quintuple layer is calculated and found to increase by a factor of 10 (ZT = 7.2) compared to that of the…

Materials Science · Physics 2015-05-20 Ferdows Zahid , Roger Lake

As a result of suppressed phonon conduction, large improvements of the thermoelectric figure of merit, ZT, have been recently reported for nanostructures compared to the raw materials' ZT values. It has also been suggested that low…

Mesoscale and Nanoscale Physics · Physics 2011-04-11 Neophytos Neophytou , Hans Kosina

The design of uranium-based thermoelectric materials presents a novel and intriguing strategy for directly converting nuclear heat into electrical power. Using high-level first-principles approach combined with accurate solution of…

Materials Science · Physics 2019-12-30 Z. Z. Zhou , D. D. Fan , H. J. Liu , J. Liu

In this first-principles study, we investigated the thermoelectric properties of the full-Heusler compound CsK$_2$Sb at different compressive strains. This material exhibits a valence band structure with significant effective mass…

Materials Science · Physics 2025-05-14 Øven A. Grimenes , G. Jeffrey Snyder , Ole M. Løvvik , Kristian Berland

Both electron and phonon transport properties of single layer MoS2 (SLMoS2) are studied. Based on first-principles calculations, the electrical conductivity of SLMoS2 is calculated by Boltzmann equations. The thermal conductivity of SLMoS2…

Mesoscale and Nanoscale Physics · Physics 2015-12-07 Zelin Jin , Quanwen Liao , Haisheng Fang , Zhichun Liu , Wei Liu , Zhidong Ding , Tengfei Luo , Nuo Yang

The electronic and transport properties of the half-Heusler compound LaPtSb are investigated by performing first-principles calculations combined with semi-classical Boltzmann theory and deformation potential theory. Compared with many…

Materials Science · Physics 2016-06-13 Q. Y. Xue , H. J. Liu , D. D. Fan , L. Cheng , B. Y. Zhao , J. Shi

Using first-principles calculations and Boltzmann theory, we explore the feasibility to maximize the thermoelectric figure of merit (ZT) of topological insulator Bi2Te3 films in the few-quintuple layer regime. We discover that the delicate…

Mesoscale and Nanoscale Physics · Physics 2016-06-09 Jinghua Liang , Long Cheng , Jie Zhang , Huijun Liu , Zhenyu Zhang

The electronic and phonon transport properties of graphene-like boron phosphide (BP), boron arsenide (BAs), and boron antimonide (BSb) monolayers are investigated using first-principles calculations and Boltzmann theory. By considering both…

Materials Science · Physics 2019-07-24 Z. Z. Zhou , H. J. Liu , D. D. Fan , G. H. Cao

The electronic and transport properties of (10, 0) single-walled carbon nanotube are studied by performing the first-principles calculations and semi-classical Boltzmann theory. It is found that the (10, 0) tube exhibits considerably large…

Mesoscale and Nanoscale Physics · Physics 2016-01-06 P. H. Jiang , H. J. Liu , D. D. Fan , L. Cheng , J. Wei , J. Zhang , J. H. Liang , J. Shi

Over the last two decades a plethora of new thermoelectric materials, their alloys, and their nanostructures were synthesized. The ZT figure of merit, which quantifies the thermoelectric efficiency of these materials increased from values…

Materials Science · Physics 2023-07-27 Neophytos Neophytou , Pankaj Priyadarshi , Zhen Li , Patrizio Graziosi

We have combined the Boltzmann transport equation with an {\it ab initio} approach to compute the thermoelectric coefficients of semiconductors. Electron-phonon, ionized impurity, and electron-plasmon scattering rates have been taken into…

Materials Science · Physics 2018-10-26 Z. Wang , S. Wang , S. Obukhov , N. Vast , J. Sjakste , V. Tyuterev , N. Mingo

Bismuth telluride-based materials is the only commercially viable room-temperature thermoelectric material, despite its limited tellurium and poor mechanical properties. The search for materials with a high figure of merit (zT > 1.00) near…

Materials Science · Physics 2024-12-06 Bingquan Peng , Yinshuo Li , Liang Chen

The two-dimensional graphene-like carbon allotrope, graphyne, has been recently fabricated and exhibits many interesting electronic properties. In this work, we investigate the thermoelectric properties of {\gamma}-graphyne by performing…

Mesoscale and Nanoscale Physics · Physics 2016-08-19 P. H. Jiang , H. J. Liu , L. Cheng , D. D. Fan , J. Zhang , J. Wei , J. H. Liang

We theoretically study transport properties of a two-dimensional electron system on a hydrogen-passivated Si(111) surface in the field-effect-transistor (FET) configuration. We calculate the density and temperature dependent mobility and…

Materials Science · Physics 2009-11-11 E. H. Hwang , S. Das Sarma

Half-Heusler compounds usually exhibit relatively higher lattice thermal conductivity that is undesirable for thermoelectric applications. Here we demonstrate by first-principles calculations and Boltzmann transport theory that the BiBaK…

Materials Science · Physics 2020-08-26 S. H. Han , Z. Z. Zhou , C. Y. Sheng , J. H. Liu , L. Wang , H. M. Yuan , H. J. Liu

The electronic structures and thermoelectric properties of $\mathrm{Cs_2[PdCl_4]I_2}$ are investigated by the first-principles calculations and semiclassical Boltzmann transport theory. Both electron and phonon transport are considered to…

Materials Science · Physics 2016-06-21 San-Dong Guo

We investigated the thermoelectric properties of the 2D monolayer of WX2N4 using Density Functional Theory combined with Boltzmann Transport Equation. We obtained an outstanding thermoelectric figure of merit of 0.91 at 400K for p-type…

Materials Science · Physics 2023-04-03 Chayan Das , Dibyajyoti Saikia , Atanu Betal , Satyajit Sahu

The electronic and thermoelectric properties of one to four monolayers of MoS$_{2}$, MoSe$_{2}$, WS$_{2}$, and WSe$_{2}$ are calculated. For few layer thicknesses,the near degeneracies of the conduction band $K$ and $\Sigma$ valleys and the…

Materials Science · Physics 2014-04-03 Darshana Wickramaratne , Ferdows Zahid , Roger K. Lake