Related papers: Optical Control of Fluorescence through Plasmonic …
The combination of single photon emitters (quantum dots) and tailored metal nanoparticles with defined size and shape allows a detailed study of the interaction between light and matter. The enhanced optical near-field of the nanoparticles…
Controlling and confining light by exciting plasmons in resonant metallic nanostructures is an essential aspect of many new emerging optical technologies. Here we explore the possibility of controllably reconfiguring the intrinsic optical…
Manipulating the spontaneous emission of a fluorescent emitter can be achieved by placing the emitter in a nanostructured environment. A privileged spot is occupied by plasmonic structures that provide a strong confinement of the…
We investigate the fluorescence properties of colloidal quantum dots attached to gold rod nanoantennas. These structures are fabricated by a two step electron beam lithography process in combination with a chemical linking method. By…
We demonstrate that the decay rates of a fluorescent molecule can be controlled by electrically shifting a transparency introduced by a Fano resonance. An auxiliary quantum object (QO), located at the hotspot of a plasmonic nanoparticle,…
We experimentally demonstrate the coherent control, i.e., phase-dependent enhancement and suppression, of the optical absorption in an array of metallic nanoantennas covered by a thin lu- minescent layer. The coherent control is achieved by…
A surrounding electromagnetic environment can engineer spontaneous emissions from quantum emitters through the Purcell effect. For instance, a plasmonic antenna can efficiently confine an electromagnetic field and enhance the fluorescent…
The distance-dependent interaction of an emitter with a plasmonic nanoparticle or surface forms the basis of the field of plexitonics. Semiconductor quantum dots (QDs) are robust emitters due to their photostability, and offer the…
We suggest a new method for quantum optical control with nanoscale resolution. Our method allows for coherent far-field manipulation of individual quantum systems with spatial selectivity that is not limited by the wavelength of radiation…
We introduce an approach to determining the required waveforms to coherently control the optical energy localization in plasmonic nanosystems. This approach is based on the impulsive localized excitation of the nanosystem and time reversal…
We report an experimental technique to map and exploit the local density of optical states of arbitrary planar nano-photonic structures. The method relies on positioning a spontaneous emitter attached to a scanning probe deterministically…
The possibility for controlling the probe-field optical gain and absorption switching and photon conversion by a surface-plasmon-polariton near field is explored for a quantum dot above the surface of a metal. In contrast to the linear…
We theoretically study on non-perturbative effective nonlinear responses of metal nanocomposites based on the intrinsic third-order nonlinear response of metal nanoparticles. The large intrinsic third-order nonlinear susceptibility of metal…
Plasmonically enhanced fluorescence is a widely studied and applied phenomenon, however only a comparative theoretical and experimental analyses of coupled fluorophores and plasmonic nanoresonators makes it possible to uncover, how this…
Tin-phthalocyanine molecules adsorbed on a NaCl ultrathin film on Au(111) exhibit electrofluorescence excited by a current across a scanning tunneling microscope junction. Exploring the dependence of the molecular monomer photon yield on…
We report on two orders of magnitude reduction in the fluorescence lifetime when a single molecule placed in a thin film is surrounded by two gold nanospheres across the film interface. By attaching one of the gold particles to the end of a…
Acoustic modulation of quantum dots allows one to control the scattering of photons. Here we theoretically characterize the degree of this acoustic control in the frequency domain. We formulate the theory of low-intensity resonance…
We demonstrate the ability to control the spontaneous emission dynamics of self-assembled quantum dots via the local density of optical modes in 2D-photonic crystals. We show that an incomplete 2D photonic bandgap is sufficient to…
Due to their ability to strongly modify the local electromagnetic (EM) field through the excitation of surface plasmon polaritons (SPPs), plasmonic nanostructures have been often used to reshape the emission direction and enhance the…
We study theoretically confinement related effects in the optical response of thin plasmonic films of controlled variable thickness. While being constant for relatively thick films, the plasma frequency is shown to acquire spatial…