English

Spontaneous emission enhancement of a single molecule by a double-sphere nanoantenna across an interface

Optics 2015-06-11 v1 Quantum Physics

Abstract

We report on two orders of magnitude reduction in the fluorescence lifetime when a single molecule placed in a thin film is surrounded by two gold nanospheres across the film interface. By attaching one of the gold particles to the end of a glass fiber tip, we could control the modification of the molecular fluorescence at will. We find a good agreement between our experimental data and the outcome of numerical calculations.

Keywords

Cite

@article{arxiv.1208.1113,
  title  = {Spontaneous emission enhancement of a single molecule by a double-sphere nanoantenna across an interface},
  author = {K. -G. Lee and H. Eghlidi and X-W. Chen and A. Renn and S. Götzinger and V. Sandoghdar},
  journal= {arXiv preprint arXiv:1208.1113},
  year   = {2015}
}