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We show that for a class of quantum light spectroscopy (QLS) experiments using n = 0,1,2,$\cdots$ classical light pulses and an entangled photon pair (a biphoton state) where one photon acts as a reference without interacting with the…

Quantum Physics · Physics 2024-02-26 Liwen Ko , Robert L. Cook , K. Birgitta Whaley

Nonlinear interactions between single quantum particles are at the heart of any quantum information system, including analog quantum simulation and fault-tolerant quantum computing. This remains a particularly difficult problem for photonic…

Laser cooling and trapping of atoms and atomic ions has led to numerous advances including the observation of exotic phases of matter, development of exquisite sensors and state-of-the-art atomic clocks. The same level of control in…

We report a significant advancement in ultra low power light-by-light phase modulation using open semiconductor microcavities in the strong light-matter coupling regime. We achieve cross-phase modulation of up to 247$\pm$17 mrad per…

Observing nonlinear optical quantum effects or implementing quantum information protocols using nonlinear optics requires moving to ever-smaller input light intensities. However, low light intensities generally mean weak optical…

Quantum Physics · Physics 2014-10-15 Audrey Dot , Evan Meyer-Scott , Raja Ahmad , Martin Rochette , Thomas Jennewein

The last two decades experimentally affirmed the quantum nature of free electron wavepackets by the rapid development of transmission electron microscopes into ultrafast, quantum-coherent systems. In particular, ultrafast electron pulses…

Optics · Physics 2022-09-30 Roy Shiloh , Tomas Chlouba , Peter Hommelhoff

The efficient interaction of light with quantum emitters is crucial to most applications in nano and quantum photonics, such as sensing or quantum information processing. Effective excitation and photon extraction are particularly important…

While experiments with one or two quantum emitters have become routine in various laboratories, scalable platforms for efficient optical coupling of many quantum systems remain elusive. To address this issue, we report on chip-based systems…

The working principles of linear optical quantum computing are based on photodetection, namely, projective measurements. The use of photodetection can provide efficient nonlinear interactions between photons at the single-photon level,…

Quantum Physics · Physics 2010-04-09 Hwang Lee , Pieter Kok , Colin P. Williams , Jonathan P. Dowling

Modern microscopy techniques are developing towards high-resolution imaging, and tremendous progress has been made in past decades; however, the imaging of individual biological macromolecules at atomic resolution using short-wavelength…

Optics · Physics 2022-01-12 Tatiana Latychevskaia

Optical spectroscopy of molecular radicals is an important tool in physical chemistry, and is a prerequisite for many experiments which use molecules for quantum science and precision measurement. However, even the simplest molecules have…

Chemical Physics · Physics 2025-05-07 Ashay N. Patel , Madison I. Howard , Timothy C. Steimle , Nicholas R. Hutzler

We experimentally observe the action of multiple light pulses on the transverse motion of a continuous beam of fullerenes. The light potential is generated by non-resonant ultra-short laser pulses in perpendicular spatial overlap with the…

Atomic and Molecular Clusters · Physics 2013-07-02 Paul Venn , Hendrik Ulbricht

A functioning quantum computer will be a machine that builds up, in a programmable way, nonclassical correlations in a multipartite quantum system. Linear optics quantum computation (LOQC) is an approach for achieving this function that…

Mesoscale and Nanoscale Physics · Physics 2010-06-09 Luca Chirolli , Guido Burkard , Shwetank Kumar , David P. DiVincenzo

Photonics is a promising architecture for the realisation of quantum information processing, since the two-photon interaction, or non-linearity, necessary to build logical gates can efficiently be realised by the use of interference with…

Quantum Physics · Physics 2011-12-06 Thomas Jennewein , Marco Barbieri , Andrew G. White

Optical solitary waves (solitons) that interact in a nonlinear system can bind and form a structure similar to a molecule. The rich dynamics of this process have created a demand for rapid spectral characterization to deepen the…

Optics · Physics 2023-06-21 Lukasz A. Sterczewski , Jaroslaw Sotor

The invention of laser immediately enabled us to detect nonlinearities of photon interaction in matter, as manifested for example by Franken et al.'s detection of second harmonic generation and the excitation of the Brillouin forward…

Quantum Physics · Physics 2010-06-24 Kensuke Homma , Dieter Habs , Toshiki Tajima

Weak cross-Kerr nonlinearities between single photons and coherent states are the basis for many applications in quantum information processing. These nonlinearities have so far mainly been discussed in terms of highly idealized single-mode…

Quantum Physics · Physics 2015-05-27 Bing He , Qing Lin , Christoph Simon

The tremendous progress in high-intensity laser technology and the establishment of dedicated high-field laboratories in recent years have paved the way towards a first observation of quantum vacuum nonlinearities at the high-intensity…

High Energy Physics - Phenomenology · Physics 2018-04-11 Holger Gies , Felix Karbstein , Christian Kohlfürst , Nico Seegert

Coherent quantum optics, where the interaction of a photon with an emitter does not scramble phase coherence, lies at the heart of many quantum optical effects and emerging technologies. Solid-state emitters coupled to nanophotonic…

Nonlinear spectroscopy is widely used for studying physical systems. Conventional nonlinear optical spectroscopy and magnetic resonance spectroscopy, which use classical probes such as electromagnetic waves, can only access certain types of…