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Single dye molecules at cryogenic temperatures display many spectroscopic phenomena known from free atoms and are thus promising candidates for fundamental quantum optical studies. However, the existing techniques for the detection of…

Quantum Physics · Physics 2008-02-12 Gert Wrigge , Ilja Gerhardt , Jaesuk Hwang , Gert Zumofen , Vahid Sandoghdar

Nonlinear single Compton scattering has been thoroughly investigated in the literature under the assumption that initially the electron has a definite momentum. Here, we study a more general initial state, and consider the electron as a…

High Energy Physics - Phenomenology · Physics 2016-05-04 A. Angioi , F. Mackenroth , A. Di Piazza

Single Photon Detectors are integral to quantum optics and quantum information. Superconducting Nanowire based detectors exhibit new levels of performance, but have no accepted quantum optical model that is valid for multiple input photons.…

Quantum Physics · Physics 2011-11-03 Mohsen K. Akhlaghi , A. Hamed Majedi , Jeff S. Lundeen

Quasi-elastic scattering processes have long been thought of providing the most promising signal for a first experimental detection of quantum vacuum nonlinearity. A prominent example of such a process is vacuum birefringence. However,…

Optics · Physics 2023-10-09 Chantal Sundqvist , Felix Karbstein

We investigate the effect of phase modulation of laser beams on the coherent and incoherent non-linear signals arising from the interaction of femtosecond pulses with matter. We observe that two collinear beams, whose phases are modulated…

Optics · Physics 2015-05-29 Khadga Jung Karki , Loni Kringle , Andrew H. Marcus , Tõnu Pullerits

Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…

Chemical Physics · Physics 2026-04-21 Yuta Fujihashi , Ozora Iso , Ryosuke Shimizu , Akihito Ishizaki

The correlated behavior of electrons determines the structure and optical properties of molecules, semiconductor and other systems. Valuable information on these correlations is provided by measuring the response to femtosecond laser…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Shaul Mukamel , Rafal Oszwaldowski , Lijun Yang

Precision spectroscopy of atomic systems is an invaluable tool for the advancement of our understanding of fundamental interactions and symmetries. Recently, highly charged ions (HCI) have been proposed for sensitive tests of physics beyond…

Well controlled nonlinear interactions between light field pulses and single atoms could be used to implement optical quantum information technologies based on qubits encoded in superpositions of coherent states of light. Here, we…

Quantum Physics · Physics 2014-07-28 Akihiro Yamaguchi , Holger F. Hofmann

We study coherent backscattering of a quasi-monochromatic laser by a dilute gas of cold two-level atoms. We consider the perturbative regime of weak intensities, where nonlinear effects arise from {\em inelastic} two-photon scattering…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 T. Wellens , B. Gremaud , D. Delande , C. Miniatura

An outstanding goal in quantum optics is the realization of fast optical non-linearities at the single-photon level. Such non-linearities would allow for the realization of optical devices with new functionalities such as a single-photon…

Mesoscale and Nanoscale Physics · Physics 2012-09-04 Thomas Volz , Andreas Reinhard , Martin Winger , Antonio Badolato , Kevin J. Hennessy , Evelyn L. Hu , Atac Imamoglu

In this work we develop an experimental procedure to interrogate the single- and multiphoton scattering matrices of an unknown quantum system interacting with propagating photons. Our proposal requires coherent state laser or microwave…

Quantum Physics · Physics 2017-10-17 Tomás Ramos , Juan José García-Ripoll

Single photons provide excellent quantum information carriers, but current schemes for preparing, processing and measuring them are inefficient. For example, down-conversion provides heralded, but randomly timed single photons, while…

Quantum Physics · Physics 2012-02-07 N. K. Langford , S. Ramelow , R. Prevedel , W. J. Munro , G. J. Milburn , A. Zeilinger

An optical source that produces single photon pulses on demand has potential applications in linear optics quantum computation, provided that stringent requirements on indistinguishability and collection efficiency of the generated photons…

Quantum Physics · Physics 2009-11-10 A. Kiraz , M. Atature , A. Imamoglu

Enhancing optical nonlinearities so that they become appreciable on the single photon level and lead to nonclassical light fields has been a central objective in quantum optics for many years. After this has been achieved in individual…

Quantum Physics · Physics 2016-09-20 Michael J. Hartmann

Recent advancements in quantum photonics have driven significant progress in photonic quantum computing (PQC), addressing challenges in scalability, efficiency, and fault tolerance. Experimental efforts have focused on integrated photonic…

Quantum Physics · Physics 2025-01-07 Dennis Delali Kwesi Wayo , Leonardo Goliatt , Darvish Ganji

We study coherent backscattering of a monochromatic laser by a dilute gas of cold two-level atoms in the weakly nonlinear regime. The nonlinear response of the atoms results in a modification of both the average field propagation (nonlinear…

Quantum Physics · Physics 2009-11-11 Thomas Wellens , Benoit Gremaud , Dominique Delande , Christian Miniatura

We investigate the generation of nonlinear operators with single photon sources, linear optical elements and appropriate measurements of auxiliary modes. We provide a framework for the construction of useful single-mode and two-mode quantum…

Quantum Physics · Physics 2009-11-10 Stefan Scheel , Kae Nemoto , William J. Munro , Peter L. Knight

Coupling light to ensembles of strongly interacting particles has emerged as a promising route toward achieving few photon nonlinearities. One specific way to implement this kind of nonlinearity is to interface light with highly excited…

Quantum Physics · Physics 2017-10-25 Callum R. Murray , Thomas Pohl

We introduce and demonstrate a new approach to measuring coherent electron wave packets using high-harmonic spectroscopy. By preparing a molecule in a coherent superposition of electronic states, we show that electronic coherence opens…

Chemical Physics · Physics 2014-07-09 P. M. Kraus , S. B. Zhang , A. Gijsbertsen , R. R. Lucchese , N. Rohringer , H. J. Wörner