Related papers: Crystal structure and magnetism in $\alpha$-RuCl3:…
The Kitaev material $\alpha$-RuCl$_3$ is among the most prominent candidates to host a quantum spin-liquid state endowed with fractionalized excitations. Recent experimental and theoretical investigations have separately revealed the…
Kitaev quantum spin liquids have attracted significant attention in condensed matter physics over the past decade. To understand their emergent quantum phenomena, high-quality single crystals of substantial size are essential. Here, we…
Recent theoretical studies have suggested that Kitaev physics and such effects as formation of a mysterious spin-liquid state can be expected not only in RuCl3 and iridates, but also in conventional $3d$ transition metal compounds. Using DC…
$\alpha$-RuCl$_3$ is a leading material for proximate Kitaev magnetism. We address the origin of the broad, $\Gamma$-point centered excitation continuum observed by inelastic neutron scattering at elevated temperatures in this compound.…
Finding new materials with antiferromagnetic (AFM) Kitaev interaction is an urgent issue to broaden and enrich the quantum magnetism research significantly. By carrying out inelastic neutron scattering experiments and subsequent analysis,…
The present studies show that long-range magnetic order takes place in RuBr$_3$ at $\approx$ 34 K. The observations of clear oscillations in the muon time spectra demonstrate the presence of well-defined internal fields at the muon sites.…
We theoretically investigate the electronic band structures and magnetic properties of ilmenites with edge-sharing IrO$_6$ honeycomb layers, $A$IrO$_3$ with $A=$ Mg, Zn, and Mn, in comparison with a collinear antiferromagnet MnTiO$_3$. The…
In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…
While the enhancement of the spin-space symmetry from the usual $\mathrm{SU}(2)$ to $\mathrm{SU}(N)$ is promising for finding nontrivial quantum spin liquids, its realization in magnetic materials remains challenging. Here we propose a new…
The honeycomb magnet $\alpha$-RuCl$_{3}$ has been a leading candidate for realizing the Kitaev quantum spin liquid (QSL), but its intrinsic spin dynamics have remained obscured by crystal twinning. Here we apply biaxial anisotropic strain…
Magnetic materials are composed of the simple building blocks of magnetic moments on a crystal lattice that interact via magnetic exchange. Yet from this simplicity emerges a remarkable diversity of magnetic states. Some reveal the deep…
The realization of Kitaev's honeycomb magnetic model in real materials has become one of the most pursued topics in condensed matter physics and materials science. If found, it is expected to host exotic quantum phases of matter and offers…
The frustrated magnet $\alpha$-RuCl$_3$ constitutes a fascinating quantum material platform that harbors the intriguing Kitaev physics. However, a consensus on its intricate spin interactions and field-induced quantum phases has not been…
Kitaev exchange, a new paradigm in quantum magnetism research, occurs for 90$^{\circ}$ metal-ligand-metal links, $t_{2g}^5$ transition ions, and sizable spin-orbit coupling. It is being studied in honeycomb compounds but also on triangular…
In quantum magnetism spin dimers are typically associated with spin-singlet states. To date, $triplet$ $dimerization$ has not been observed in any 3D or quasi-2D material. With this in mind we here discuss the electronic structure of the…
Ru$_3$Sn$_7$, an intermetallic compound with advanced catalytic properties, exhibits a complex crystal structure and intriguing electronic properties, making it an attractive candidate for investigations under high-pressure (HP). The…
Ferromagnetism in the two-dimensional CrI$_3$ has generated a lot of excitement, and it was recently proposed that the spin-orbit coupling (SOC) in Iodine may generate bond-dependent spin interactions leading to magnetic anisotropy. Here we…
Substitution effects of Os for Ru in {\alpha}-RuCl3 are investigated in a wide composition range of 0 =< x =< 0.67 in Ru1-xOsxCl3 by X-ray and electron diffraction, magnetic susceptibility, heat capacity, and Raman spectroscopy…
We report structural studies of the spin-orbit Mott insulator family K$_x$Ir$_y$O$_2$, with triangular layers of edge-sharing IrO$_6$ octahedra bonded by potassium ions. The potassium content acts as a chemical tuning parameter to control…
We have performed an {\it ab initio} study of the electronic structure of two isostructural quantum spin systems, KCuCl$_{3}$ and TlCuCl$_{3}$, which have recently attracted much attention due to their unconventional magnetic properties.…