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We propose and demonstrate the method of population transfer by piecewise adiabatic passage between two quantum states. Coherent excitation of a two-level system with a train of ultrashort laser pulses is shown to reproduce the effect of an…

Atomic Physics · Physics 2009-11-13 S. Zhdanovich , E. A. Shapiro , M. Shapiro , J. W. Hepburn , V. Milner

The chirped-pulse interaction in the adiabatic coupling regime induces cyclic permutations of the energy states of a three-level system in the $V$-type configuration, which process is known as the three-level chirped rapid adiabatic…

Atomic Physics · Physics 2016-08-24 Yunheung Song , Han-gyeol Lee , Hanlae Jo , Jaewook Ahn

We analyze excitation of two ground state atoms to a double Rydberg state by a two-photon chirped optical pulse in the regime of adiabatic rapid passage. For intermediate Rydberg-Rydberg interaction strengths, relevant for atoms separated…

Quantum Physics · Physics 2015-06-11 Elena Kuznetsova

A semiclassical, four-level model of a nanosecond, chirped pulse interacting with all optically accessible hyperfine states in the ultracold Rb atom is analyzed aiming at population inversion within $5S_{1/2}$ electronic state. The nature…

Quantum Physics · Physics 2015-09-02 Gengyuan Liu , S. A. Malinovskaya

We implement a 4-level semiclassical model of a single pulse interacting with the hyperfine structure in ultracold rubidium aimed at control of population dynamics and quantum state preparation. We discuss a method based on pulse chirping…

Quantum Physics · Physics 2015-03-26 G. Liu , V. Zakharov , T. Collins , P. Gould , S. A. Malinovskaya

A two level system is considered which has no static dipole moment, e.g. molecule $H_2$ in its ground electronic state. If strong enough external field is applied, it will dynamically distort such a system and supply it with time (and…

Quantum Physics · Physics 2007-05-23 Duje Bonacci

We study the quantum dynamics of a two-level system driven by a pulse that starts near-resonant for small amplitudes, yielding nonadiabatic evolution, and induces an adiabatic evolution for larger amplitudes. This problem is analyzed in…

Quantum Physics · Physics 2009-11-10 L. P. Yatsenko , S. Guerin , H. R. Jauslin

We introduce and analyze theoretically a procedure that combines slow adiabatic STIRAP manipulation with short nonadiabatic Rabi pulses to produce any desired three-level state in a qutrit system. In this protocol, the fast pulses create…

We show how one can perform arbitrary rotation of any qubit, using delayed laser pulses through nonadiabatic evolution, i.e., via transitions among the adiabatic states. We use a double-Lambda scheme and use a set of control parameters such…

Quantum Physics · Physics 2007-05-23 Asoka Biswas , G. S. Agarwal

State selective preparation and manipulation of discrete-level quantum systems such as atoms, molecules or quantum dots is a the ultimate tool for many diverse fields such as laser control of chemical reactions, atom optics, high-precision…

Quantum Physics · Physics 2007-05-23 Duje Bonacci

We present a method for achieving complete population transfer in a two-state quantum system via adiabatic time evolution in which, contrary to conventional rapid adiabatic passage produced by chirped pulses, there occurs no crossing of…

Quantum Physics · Physics 2010-02-03 A. A. Rangelov , N. V. Vitanov , B. W. Shore

This theoretical paper presents numerical calculations for photoassociation of ultracold cesium atoms with a chirped laser pulse and detailed analysis of the results. In contrast with earlier work, the initial state is represented by a…

Atomic and Molecular Clusters · Physics 2009-11-10 E. Luc-Koenig , R. Kosloff , F. Masnou-Seeuws , M. Vatasescu

Shaped free electron vortices (SEVs) have recently been studied using atomic (1+2) resonance-enhanced multiphoton ionization (REMPI) by oppositely chirped counterrotating circularly polarized (OC-CRCP) femtosecond laser pulses. By…

Atomic Physics · Physics 2025-06-11 D. Köhnke , T. Bayer , M. Wollenhaupt

We report an ultrafast and efficient way to create the maximum coherence between the two lower states in a -like atomic systems, driven by two nonlinearly chirped few-cycle pulses. The phenomenon of coherent population trapping and…

Quantum Physics · Physics 2011-11-18 Amarendra K. Sarma , Parvendra Kumar

We have proposed and demonstrated a fast and robust method of population transfer between two quantum states using a quadratically chirped laser source. Incorporating the Jaynes-Cummings in a full quantum description of the interaction, and…

Atomic Physics · Physics 2019-09-04 Fatemeh Ahmadinouri , Mehdi Hosseini , Farrokh Sarreshtedari

We study the population dynamics in a two-atom setup in which each atom is driven independently by different light fields, but coupling the same Rydberg state. In particular, we look at how an offset in the Rabi frequencies between two…

Quantum Gases · Physics 2019-09-04 Vineesha Srivastava , Ankita Niranjan , Rejish Nath

Rabi oscillation of a two-level system driven by a pulse train is a basic process involved in quantum computation. We present a full quantum treatment of this process and show that the population inversion of this process collapses…

Quantum Physics · Physics 2015-03-17 Li Yang , Biyao Yang , Yufu Chen

A coherent mechanism of robust population inversion in atomic and molecular systems by a chirped field is presented. It is demonstrated that a field of sufficiently high chirp rate imposes a certain relative phase between a ground and…

Quantum Physics · Physics 2015-06-26 Jiri Vala , Ronnie Kosloff

In the previous paper on this topic it was shown how, for a pulse of arbitrary shape and duration, the drive frequency can be analytically optimized to maximize the amplitude of the population oscillations between the selected two levels in…

Quantum Physics · Physics 2007-05-23 Duje Bonacci

To coherently control a few-level quantum emitter, typically pulses with an energy resonant to the transition energy are applied making use of the Rabi mechanism, while a single off-resonant pulse does not result in a population inversion.…

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