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A core-softened model of a glass forming fluid is numerically studied in the limit of very low temperatures. The model shows two qualitatively different behaviors depending on the strength of the attraction between particles. For no or low…

Statistical Mechanics · Physics 2009-11-07 E. A. Jagla

Dynamical heterogeneity, in which transitory local fluctuations occur in the conformation and dynamics of constituent particles, is widely hypothesized to be essential to evolution of supercooled liquids into the structural glass state. Yet…

We study diffusion of colloids on a fluid-fluid interface using particle simulations and fluctuating hydrodynamics. Diffusion on a two-dimensional interface with three-dimensional hydrodynamics is known to be anomalous, with the collective…

Statistical Mechanics · Physics 2018-08-01 R. P. Peláez , F. Balboa Usabiaga , S. Panzuela , Q. Xiao , R. Delgado-Buscalioni , A. Donev

We monitor the transformation of a liquid into an amorphous solid in simulations of a glass forming liquid by measuring the variation of a structural order parameter with either changing temperature or potential energy to establish the…

Soft Condensed Matter · Physics 2023-06-07 Gang Sun , Peter Harrowell

Liquid water is well-known for its intriguing thermodynamic anomalies in the supercooled state. The phenomenological two-state models - based on the assumption of the existence of two types of competing local states (or, structures) in…

Chemical Physics · Physics 2022-11-23 Arijit Mondal , Gadha R. , Rakesh S. Singh

Glass-forming liquids grow dramatically sluggish upon cooling. This slowdown has long been thought to be accompanied by a growing correlation length. Characteristic dynamical and static length scales, however, have been observed to grow at…

Disordered Systems and Neural Networks · Physics 2016-08-22 Patrick Charbonneau , Ethan Dyer , Jaehoon Lee , Sho Yaida

The paper is devoted to the thermodynamics of normal surface electromagnetic fields within a nonuniform dispersive and absorptive system. This system is formed by vacuum and lossy medium separated by a plane interface. As a medium, we used…

Other Condensed Matter · Physics 2012-12-04 Illarion Dorofeyev

We investigate the energy landscape of two dimensional network models for covalent glasses by means of the lid algorithm. For three different particle densities and for a range of network sizes, we exhaustively analyse many configuration…

Statistical Mechanics · Physics 2009-10-31 J. Christian Schoen , Paolo Sibani

While the water molecule is simple, its condensed phase liquid behavior is so complex that no consensus description has emerged despite three centuries of effort. Here we identify features of its behavior that are the most peculiar, hence…

Chemical Physics · Physics 2014-04-16 Stacey L. Meadley , C. Austen Angell

The structure of liquid water in the proximity of an interface can deviate significantly from that of bulk water, with surface-induced structural perturbations typically converging to bulk values at about ~1 nm from the interface. While…

Soft Condensed Matter · Physics 2022-03-01 Piero Gasparotto , Martin Fitzner , Stephen J. Cox , Gabriele Cesare Sosso , Angelos Michaelides

In equilibrium and supercooled liquids, polymorphism is manifested by thermodynamic regions defined in the phase diagram, which are predominantly of different short- and medium-range order (local structure). It is found that on the phase…

Soft Condensed Matter · Physics 2024-03-19 Anatolii V. Mokshin , Roman V. Vlasov

We use a recently-derived reformulation of the diffusion constant [Stillinger F H and Debenedetti P G 2005 J. Phys. Chem. B 109 6604] to investigate heterogeneous dynamics and non-Gaussian diffusion in a binary Lennard-Jones mixture. Our…

Soft Condensed Matter · Physics 2007-05-23 M. Scott Shell , Pablo G. Debenedetti , Frank H. Stillinger

We analyse a one-dimensional model of hard particles, within ensembles of trajectories that are conditioned (or biased) to atypical values of the time-averaged dynamical activity. We analyse two phenomena that are associated with these…

Statistical Mechanics · Physics 2015-11-18 Ian R. Thompson , Robert L. Jack

Supercooled liquids exhibit complicated dynamical behaviors: At the microscopic level, the dynamics is heterogeneous spatially, known as dynamic heterogeneity. At the macroscopic level, the shear viscosity $\eta$ decreases as shear rate…

Soft Condensed Matter · Physics 2025-09-01 Ke-Qi Zeng , Dong-Xu Yu , Zhe Wang

Supercooled liquids exhibit spatial heterogeneity in the dynamics of their fluctuating atomic arrangements. The length and time scales of the heterogeneous dynamics are central to the glass transition and influence nucleation and growth of…

Materials Science · Physics 2018-05-09 Pei Zhang , Jason J. Maldonis , Ze Liu , Jan Schroers , Paul M. Voyles

Complex topographies exhibit universal properties when fluvial erosion dominates landscape evolution over other geomorphological processes. Similarly, we show that the solutions of a minimalist landscape evolution model display invariant…

Pattern Formation and Solitons · Physics 2024-01-10 Shashank Kumar Anand , Matteo B. Bertagni , Theodore D. Drivas , Amilcare Porporato

We study the transport properties of a system of active particles moving at constant speed in an heterogeneous two-dimensional space. The spatial heterogeneity is modeled by a random distribution of obstacles, which the active particles…

Biological Physics · Physics 2013-10-23 Oleksandr Chepizhko , Fernando Peruani

We introduce a new measure of the structure of a liquid which is the softness of the mean-field potential developed by us earlier. We find that this softness is sensitive to small changes in the structure. We then study its correlation with…

Soft Condensed Matter · Physics 2021-05-26 Manoj Kumar Nandi , Sarika Maitra Bhattacharyya

We study the vibrational spectra and the specific heat of disordered systems using an effective hydrodynamic framework. We consider the contribution of diffusive modes, i.e. the 'diffusons', to the density of states and the specific heat.…

Disordered Systems and Neural Networks · Physics 2019-08-21 Matteo Baggioli , Alessio Zaccone

Motivated by a series of experiments that revealed a temperature dependence of the dynamic scaling regime of growing surfaces, we investigate theoretically how a nonequilibrium growth process reacts to a sudden change of system parameters.…

Statistical Mechanics · Physics 2015-05-14 Yen-Liang Chou , Michel Pleimling , R. K. P. Zia