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We present a technique for partitioning the total energy from a semi-local density functional theory calculation into contributions from individual electronic states in a localized Wannier basis. We use our technique to reveal the key role…

Materials Science · Physics 2025-10-15 Ethan T. Ritz , Guru Khalsa , Hsin-Yu Ko , Ju-an Zhang , Robert A. DiStasio , Nicole A. Benedek

We derive efficient and reliable goal-oriented error estimations, and devise adaptive mesh procedures for the finite element method that are based on the localization of a posteriori estimates. In our previous work [SIAM J. Sci. Comput.,…

Numerical Analysis · Mathematics 2020-03-23 Bernhard Endtmayer , Ulrich Langer , Thomas Wick

We consider a class of optimization problems that involve determining the maximum value that a function in a particular class can attain subject to a collection of difference constraints. We show that a particular linear programming…

Data Structures and Algorithms · Computer Science 2022-11-16 Sungjin Im , Benjamin Moseley , Hung Q. Ngo , Kirk Pruhs , Alireza Samadian

Physical simulation-based optimization is a common task in science and engineering. Many such simulations produce image- or tensor-based outputs where the desired objective is a function of those outputs, and optimization is performed over…

Machine Learning · Computer Science 2021-12-01 Wesley Maddox , Qing Feng , Max Balandat

In this paper, we present an overview of the recent developments of functional quantization of stochastic processes, with an emphasis on the quadratic case. Functional quantization is a way to approximate a process, viewed as a…

Probability · Mathematics 2013-04-03 Gilles Pagès

We present a joint implementation of dynamical-mean-field theory (DMFT) with the pseudopotential plane-wave approach, via Wannier functions, for the determination of the electronic properties of strongly correlated materials. The scheme…

Strongly Correlated Electrons · Physics 2018-08-08 G. Trimarchi , I. Leonov , N. Binggeli , Dm. Korotin , V. I. Anisimov

We show that the method of maximum-likelihood estimation, recently introduced in the context of quantum process tomography, can be applied to the determination of Mueller matrices characterizing the polarization properties of classical…

Optics · Physics 2009-11-11 A. Aiello , G. Puentes , D. Voigt , J. P. Woerdman

We establish the characterizations of commutators of several versions of maximal functions on spaces of homogeneous type. In addition, with the aid of interpolation theory, we provide weighted version of the commutator theorems by…

Functional Analysis · Mathematics 2019-07-29 Zunwei Fu , Elodie Pozzi , Qingyan Wu

The exponential localization of Wannier functions in two or three dimensions is proven for all insulators that display time-reversal symmetry, settling a long-standing conjecture. Our proof relies on the equivalence between the existence of…

Submodular function minimization is well studied, and existing algorithms solve it exactly or up to arbitrary accuracy. However, in many applications, such as structured sparse learning or batch Bayesian optimization, the objective function…

Machine Learning · Computer Science 2022-03-10 Marwa El Halabi , Stefanie Jegelka

Many large-scale machine learning problems--clustering, non-parametric learning, kernel machines, etc.--require selecting a small yet representative subset from a large dataset. Such problems can often be reduced to maximizing a submodular…

Machine Learning · Computer Science 2016-06-28 Baharan Mirzasoleiman , Amin Karbasi , Rik Sarkar , Andreas Krause

We study the placement of virtual functions aimed at minimizing the cost. We propose a novel algorithm, using ideas based on multi-armed bandits. We prove that these algorithms learn the optimal placement policy rapidly, and their regret…

Machine Learning · Computer Science 2025-06-04 Wei Huang , Richard Combes , Andrea Araldo , Hind Castel-Taleb , Badii Jouaber

Estimation of the level set of a function (i.e., regions where the function exceeds some value) is an important problem with applications in digital elevation mapping, medical imaging, astronomy, etc. In many applications, the function of…

Applications · Statistics 2018-03-06 Kalyani Krishnamurthy , Waheed U. Bajwa , Rebecca Willett

In this article we propose building general-purpose function approximators on top of Haar Scattering Networks. We advocate that this architecture enables a better comprehension of feature extraction, in addition to its implementation…

Machine Learning · Statistics 2018-04-11 Fernando Fernandes Neto

Simulation of mesoscopic nanostructures is a central challenge in condensed matter physics and device applications. First-principles methods provide accurate electronic structures but are computationally prohibitive for large systems, while…

Materials Science · Physics 2025-10-03 Guan-Hao Peng , Chin-Jui Huang , Wen-Teng Yang , Shun-Jen Cheng

Submodular optimization with bandit feedback has recently been studied in a variety of contexts. In a number of real-world applications such as diversified recommender systems and data summarization, the submodular function exhibits…

Machine Learning · Computer Science 2024-07-04 Wenjing Chen , Victoria G. Crawford

We present a quantum embedding method that allows for the calculation of local excited states embedded in a Kohn-Sham density functional theory (DFT) environment. Projection-based quantum embedding methodologies provide a rigorous framework…

Chemical Physics · Physics 2019-09-30 Xuelan Wen , Daniel S. Graham , Dhabih V. Chulhai , Jason D. Goodpaster

In this paper, we propose a maximum smoothed likelihood method to estimate the component density functions of mixture models, in which the mixing proportions are known and may differ among observations. The proposed estimates maximize a…

Methodology · Statistics 2014-07-14 Tao Yu , Pengfei Li , Jing Qin

A new implementation is proposed for including van der Waals (vdW) interactions in Density Functional Theory (DFT) using the Maximally-Localized Wannier functions (MLWFs), which is free from empirical parameters. With respect to the…

Chemical Physics · Physics 2019-05-22 Pier Luigi Silvestrelli , Alberto Ambrosetti

Machine learning is used to approximate density functionals. For the model problem of the kinetic energy of non-interacting fermions in 1d, mean absolute errors below 1 kcal/mol on test densities similar to the training set are reached with…

Computational Physics · Physics 2015-06-03 John C. Snyder , Matthias Rupp , Katja Hansen , Klaus-Robert Müller , Kieron Burke
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