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Infrared reflectance measurements were made on the single crystal pyrochlore Cd$_{2}$Os$_{2}$O$_{7}$ in order to examine the transformations of the electronic structure and crystal lattice across the boundary of the metal insulator…

Strongly Correlated Electrons · Physics 2009-11-07 W. J. Padilla , D. N. Basov , D. Mandrus

The interplay between spin and orbital degrees of freedom gives rise to a variety of emergent phases in correlated 4d and 5d transition-metal systems. Strong spin-orbit coupling (SOC) significantly alters Jahn-Teller (JT) physics, often…

Strongly Correlated Electrons · Physics 2025-05-28 A. S. Miñarro , G. Herranz

Strong electron correlation and spin-orbit coupling (SOC) provide two non-trivial threads to condensed matter physics. When these two strands of physics come together, a plethora of quantum phenomena with novel topological order have been…

Mesoscale and Nanoscale Physics · Physics 2024-02-26 Jiang-Xiazi Lin , Ya-Hui Zhang , Erin Morissette , Zhi Wang , Song Liu , Daniel Rhodes , K. Watanabe , T. Taniguchi , James Hone , J. I. A. Li

Spin-orbit coupling (SOC) lifts molecular orbital degeneracy, enabling bi-level electronic platforms suitable for next-generation digital devices. However, common light-atom molecular feedstocks exhibit weak SOC due to the absence of heavy…

Materials Science · Physics 2025-05-07 Zihao Wang , Wan-Lu Li , Shaowei Li

We investigate the electronic and magnetic structures and the character and direction of spin and orbital moments of the recently synthesized quadruple perovskite cobaltovanadate CaCo3V4O12 using a selection of methods from density…

Strongly Correlated Electrons · Physics 2014-11-19 H. B. Rhee , W. E. Pickett

Conduction band-edge spin-orbit splitting (SOS) in monolayer transition metal dichalcogenides determines a competition between bright and dark excitons and sets conditions for spintronics applications of these semiconductors. Here, we…

Mesoscale and Nanoscale Physics · Physics 2026-02-11 Igor Rozhansky , Michele Masseroni , Ricardo Pisoni , Suad Alshammari , Xue Li , Thomas Ihn , Klaus Ensslin , James McHugh , Vladimir Fal'ko

$Fe_3O_4$ is a mixed-valence strongly correlated transition metal oxide which displays the intriguing metal to insulator Verwey transition. Here we investigate the electronic and magnetic structure of $Fe_3O_4$ by a unique combination of…

Strongly Correlated Electrons · Physics 2018-11-13 H. Elnaggar , R. Wang , S. Lafuerza , E. Paris , A. C. Komarek , H. Guo , Y. Tseng , D. McNally , F. Frati , M. W. Haverkort , M. Sikora , T. Schmitt , F. M. F. de Groot

One of the main characteristics of the new family of two-dimensional crystals of semiconducting transition metal dichalcogenides (TMD) is the strong spin-orbit interaction, which makes them very promising for future applications in…

Mesoscale and Nanoscale Physics · Physics 2015-11-11 R. Roldán , M. P. López-Sancho , E. Cappelluti , J. A. Silva-Guillén , P. Ordejón , F. Guinea

The 5$d$ transition metal oxides, in particular iridates, host novel electronic and magnetic phases due to the interplay between onsite Coulomb repulsion ($U$) and spin-orbit coupling (SOC). The reduced dimensionality brings another degree…

Strongly Correlated Electrons · Physics 2022-02-08 Amit Chauhan , B. R. K. Nanda

The interplay between spin-orbit coupling (SOC) and electron correlation ($U$) is considered for many exotic phenomena in iridium oxides. We have investigated the evolution of structural, magnetic and electronic properties in pyrochlore…

Strongly Correlated Electrons · Physics 2017-03-08 Harish Kumar , R. S. Dhaka , A. K. Pramanik

We have studied in detail the electronic structure of IrO$_2$ including spin-orbit coupling (SOC) and electron-electron interaction, both within the GGA+U and GGA+DMFT approximations. Our calculations reveal that the Ir t$_{2g}$ states at…

Strongly Correlated Electrons · Physics 2014-04-25 S. K. Panda , S. Bhowal , A. Delin , O. Eriksson , I. Dasgupta

We explore possible superconducting states in $t_{2g}$ multi-orbital correlated electron systems with strong spin-orbit coupling (SOC). In order to study such systems in a controlled manner, we employ large-scale dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2014-10-24 Zi Yang Meng , Yong Baek Kim , Hae-Young Kee

4$d$ transition metal oxide (TMO) offers an intriguing puzzle for their electronic and magnetic ground state. They are in the cross-over regime of strong spin orbit interaction (SOI) and electron-electron correlation ($U$) with quenched…

Strongly Correlated Electrons · Physics 2025-12-15 Asha Ann Abraham , Roumita Roy , Ruta Kulkarni , Sudipta Kanungo , Soham Manni

The iso-electronic $d^{4}$ compounds of the $4d$ series show rich phase diagrams due to competing spin, charge and orbital degrees of freedom in presence of strong correlations and structural distortions. One such iso-electronic series,…

Strongly Correlated Electrons · Physics 2018-07-10 Swagata Acharya , Dibyendu Dey , T Maitra , A Taraphder

Spin-orbit coupling (SOC) often gives rise to interesting electronic and magnetic phases in an otherwise ordinary pool of paramagnetic heavy metal oxides. In presence of strong SOC, assumed to be working in $j$-$j$ coupling regime, 5$d^4$…

Spin-orbit coupling has been reported to be responsible for the insulating nature of the 5d$^1$ osmate double perovskite Ba$_2$NaOsO$_6$ (BNOO). However, whether spin-orbit coupling indeed drives the metal-to-insulator transition (MIT) in…

Strongly Correlated Electrons · Physics 2024-01-17 Dario Fiore Mosca , Hermann Schnait , Lorenzo Celiberti , Markus Aichhorn , Cesare Franchini

While it was speculated that 5$d^4$ systems would possess non-magnetic $J$~=~0 ground state due to strong Spin-Orbit Coupling (SOC), all such systems have invariably shown presence of magnetic moments so far. A puzzling case is that of…

The Ruddlesden-Popper (RP) series of iridates (Srn+1IrnO3n+1) have been the subject of much recent attention due to the anticipation of emergent physics arising from the cooperative action of spin-orbit (SO) driven band splitting and…

Mott insulators based on $4d$ and $5d$ transition-metal ions, where spin-orbit interaction plays a key role, can exhibit various forms of unusual magnetism. A particular example is the antiferromagnet Ca$_2$RuO$_4$ containing $d^4$…

Strongly Correlated Electrons · Physics 2025-05-16 Jan Revenda , Krzysztof Wohlfeld , Jiří Chaloupka

Entanglement of spin and orbital degrees of freedom drives the formation of novel quantum and topological physical states. Discovering new spin-orbit entangled ground states and emergent phases of matter requires both experimentally probing…

Strongly Correlated Electrons · Physics 2017-05-18 A. E. Taylor , S. Calder , R. Morrow , H. L. Feng , M. H. Upton , M. D. Lumsden , K. Yamaura , P. M. Woodward , A. D. Christianson