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Progress in electron-beam spectroscopies has recently enabled the study of optical excitations with combined space, energy and time resolution in the nanometer, millielectronvolt and femtosecond domain, thus providing unique access into…

Optics · Physics 2019-11-13 Albert Polman , Mathieu Kociak , F. Javier García de Abajo

The bright exciton emission of semiconducting carbon nanotubes is appealing for optoelectronic and quantum photonic devices as well as fundamental studies of light-matter interaction in one-dimensional nanostructures. The photophysics of…

Mesoscale and Nanoscale Physics · Physics 2017-05-09 Ibrahim Sarpkaya , Zhengyi Zhang , William Walden-Newman , Xuesi Wang , James Hone , Chee Wei Wong , Stefan Strauf

We have measured the electroluminescence and photoluminescence of (9,7) semiconducting carbon nanotube devices and demonstrate that the electroluminescence wavelength is determined by the nanotube's chiral index (n,m). The devices were…

Current methods for producing single-walled carbon nanotubes (SWNTs) lead to heterogeneous samples containing mixtures of metallic and semiconducting species with a variety of lengths and defects. Optical detection at the single nanotube…

We present a first-principles study of semiconducting carbon nanotubes adsorbed on the unpassivated Si(100) surface. We have found metallicity for the combined system caused by n-doping of the silicon slab representing the surface by the…

Materials Science · Physics 2007-05-23 Salvador Barraza-Lopez , Peter M. Albrecht , Nichols A. Romero , Karl Hess

Excitonic effects in 1D semiconductors can be qualitatively different from those in higher dimensions. In particular, the Sommerfeld factor, the ratio of the above-band-edge excitonic continuum absorption to free electron-hole pair…

One- and two-photon luminescence excitation spectroscopy showed a series of distinct excitonic states in single-walled carbon nanotubes. The energy splitting between one- and two-photon-active exciton states of different wavefunction…

Materials Science · Physics 2007-05-23 J. Maultzsch , R. Pomraenke , S. Reich , E. Chang , D. Prezzi , A. Ruini , E. Molinari , M. S. Strano , C. Thomsen , C. Lienau

We present a theoretical approach to calculate the {\it local} absorption spectrum of excitons confined in a semiconductor nanostructure. Using the density-matrix formalism, we derive a microscopic expression for the non-local…

Materials Science · Physics 2009-10-31 O. Mauritz , G. Goldoni , E. Molinari , F. Rossi

We present a detailed electron diffraction study of individual single-walled carbon nanotubes. A novel sample preparation procedure provides well-separated, long and straight individual single-shell nanotubes. Diffraction experiments are…

Materials Science · Physics 2007-05-23 Jannik C. Meyer , Matthieu Paillet , Georg S. Duesberg , Siegmar Roth

The use of optics in microelectronic circuits to overcome the limitation of metallic interconnects is more and more considered as a viable solution. Among future silicon compatible materials, carbon nanotubes are promising candidates thanks…

Dielectrophoresis can potentially be used as an efficient trapping tool in the fabrication of molecular devices. For nanoscale objects, however, the Brownian motion poses a challenge. We show that the use of carbon nanotube electrodes makes…

Carbon based optoelectronic devices promise to revolutionize modern integrated circuits by combining outstanding electrical and optical properties into a unified technology. By coupling nanoelectronic devices to nanophotonic structures…

Mesoscale and Nanoscale Physics · Physics 2013-06-25 Svetlana Khasminskaya , Feliks Pyatkov , Benjamin S. Flavel , Wolfram H. P. Pernice , Ralph Krupke

We report correlated-electron calculations of optically excited states in ten semiconducting single-walled carbon nanotubes with a wide range of diameters. Optical excitation occurs to excitons whose binding energies decrease with the…

Materials Science · Physics 2007-05-23 Hongbo Zhao , Sumit Mazumdar

A new method to characterize microwave electromagnetic absorption of a bulk carbon nanotube material is proposed and experimentally evaluated in this paper. The method is based on the measurement of microwave transmission through a…

Applied Physics · Physics 2020-08-26 O. Malyuskin , P. Brunet , D. Mariotti , R. McGlynn , P. Maguire

We study both experimentally and theoretically the fundamental interplay of exciton localization and polarization in semiconducting single-walled carbon nanotubes. From Stark spectroscopy of individual carbon nanotubes at cryogenic…

The high aspect ratio of carbon nanotubes makes them prone to bending. To know how bending affects the tubes is therefore crucial for tube identification and for electrical component design. Very few studies, however, have investigated…

Mesoscale and Nanoscale Physics · Physics 2010-11-24 Pekka Koskinen

Carbon nanotubes (CNTs) are a one-dimensional material system with intriguing physical properties that lead to emerging applications. While CNTs are unusually strain resistant compared to bulk materials, their optical-absorption spectrum is…

Computational Physics · Physics 2019-02-22 Christian Wagner , Jörg Schuster , André Schleife

Photoluminescence is commonly used to identify the electronic structure of individual nanotubes. But, nanotubes naturally occur in bundles. Thus, we investigate photoluminescence of nanotube bundles. We show that their complex spectra are…

Materials Science · Physics 2015-05-13 P. H. Tan , A. G. Rozhin , T. Hasan , P. Hu , V. Scardaci , W. I. Milne , A. C. Ferrari

We report a comparative ab-initio study of different types of adsorbates and their adsorption mechanism on the field-emission performance of single-walled carbon nanotubes by analyzing electrical properties and transport characteristics and…

Materials Science · Physics 2019-02-15 Ehsanur Rahman , Alireza Nojeh

Luminescence properties of carbon nanotubes are strongly affected by exciton diffusion, which plays an important role in various nonradiative decay processes. Here we perform photoluminescence microscopy on hundreds of individual…

Mesoscale and Nanoscale Physics · Physics 2015-03-23 A. Ishii , M. Yoshida , Y. K. Kato