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Holographic molecular binding assays use holographic video microscopy to directly detect molecules binding to the surfaces of micrometer-scale colloidal beads by monitoring associated changes in the beads' light-scattering properties.…

Soft Condensed Matter · Physics 2020-06-24 Lauren E. Altman , David G. Grier

We report surface shear rheological measurements on dense insoluble monolayers of micron sized colloidal spheres at the oil/water interface and of the protein $\beta$-lactoglobulin at the air/water surface. As expected, the elastic modulus…

Soft Condensed Matter · Physics 2009-11-10 Pietro Cicuta , Edward J. Stancik , Gerald G. Fuller

When a drop containing colloidal particles evaporates on a surface, a circular stain made of these particles is often observed due to an internal flow toward the contact line. To hinder this effect, several approaches have been proposed…

Soft Condensed Matter · Physics 2016-01-06 François Boulogne , François Ingremeau , Julien Dervaux , Laurent Limat , Howard A. Stone

The adsorption of polymer and surfactant molecules onto colloidal particles or droplets in solution can be characterized non-destructively by scattering techniques. In a first part, the general framework of Dynamic Light Scattering, Small…

Soft Condensed Matter · Physics 2007-05-24 Julian Oberdisse

From biological tissues to layers of paint, macroscopic non-porous materials with the capacity to swell when brought in contact with an appropriate solvent are ubiquitous. Here, we study experimentally and theoretically one of the…

Soft Condensed Matter · Physics 2022-04-18 Merlin A. Etzold , George T. Fortune , Julien R. Landel , Stuart B. Dalziel

Enhanced optical absorption of molecules in the vicinity of metallic nanostructures is key to a number of surface-enhanced spectroscopies and of great general interest to the fields of plasmonics and nano-optics. Yet, experimental access to…

Holographic molecular binding assays detect macromolecules binding to colloidal probe beads by monitoring nanometer-scale changes in the beads' diameters with holographic microscopy. Measured changes are interpreted with Maxwell Garnett…

Soft Condensed Matter · Physics 2026-02-10 Kaitlynn Snyder , Andrew D. Hollingsworth , Fook Chiong Cheong , Rushna Quddus , David G. Grier

The effect of the adsorption of a polypeptide on the lateral interaction of dimyristoylphosphatidylserine molecules in different phase states on the surface of a 10\,mM KCl aqueous solution has been studied. Changes in the surface pressure…

The study of competitive and cooperative adsorption of functionalized molecules such as polymers, rheology modifiers and surfactant molecules on colloidal particles immersed in a solvent is undertaken using coarse grained, dissipative…

Soft Condensed Matter · Physics 2014-06-13 A. Gama Goicochea

We use digital holographic microscopy and Mie scattering theory to simultaneously characterize and track individual colloidal particles. Each holographic snapshot provides enough information to measure a colloidal sphere's radius and…

Surface creasing in swelling polymer gels is commonly attributed to compressive strain or interlayer mismatch, yet its general control remains unclear. Here we show that solvent polymerization degree $N_{\rm s}$ provides an independent…

We induce and investigate the coarsening and melting dynamics of an initially static nanoparticle colloidal monolayer at an ionic liquid-vacuum interface, driven by a focused, scanning electron beam. Coarsening occurs through grain…

Soft Condensed Matter · Physics 2020-09-29 Connor G. Bischak , Jonathan G. Raybin , Jonathon W. Kruppe , Naomi S. Ginsberg

We model the behaviour of a single colloid embedded in a cross-linked polymer gel, immersed in a viscous background fluid. External fields actuate the particle into a periodic motion, which deforms the embedding matrix and creates a local…

Soft Condensed Matter · Physics 2022-11-09 Guido L. A. Kusters , Cornelis Storm , Paul van der Schoot

Thermo-responsive hydrogels are a promising material for creating controllable actuators for use in micro-scale devices, since they expand and contract significantly (absorbing or expelling fluid) in response to relatively small temperature…

Soft Condensed Matter · Physics 2022-08-18 Matthew D. Butler , Thomas D. Montenegro-Johnson

Building structures with hierarchical order through the self-assembly of smaller blocks is not only a prerogative of nature, but also a strategy to design artificial materials with tailored functions. We explore in simulation the…

Soft Condensed Matter · Physics 2020-02-17 Santi Prestipino , Domenico Gazzillo , Gianmarco Munaò , Dino Costa

Thermoresponsive microgels are polymeric colloidal networks that can change their size in response to a temperature variation. This peculiar feature is driven by the nature of the solvent-polymer interactions, which triggers the so-called…

Soft Condensed Matter · Physics 2019-02-08 Fabrizio Camerin , Nicoletta Gnan , Lorenzo Rovigatti , Emanuela Zaccarelli

The hydrodynamic effects of macromolecular crowding inside cells is often studied in vitro by using polymers as crowding reagents. Confinement of polymers inside cell-sized droplets has been shown to affect the diffusion of small molecules.…

Soft Condensed Matter · Physics 2023-04-28 Yaam Deckel , Lauren A. Lowe , Siddharth Rawat , Matthew Turner , James Luong , Anna Wang

Cholesteric liquid crystals can exhibit spatial patterns in molecular alignment at interfaces that can be exploited for particle assembly. These patterns emerge from the competition between bulk and surface energies, tunable with the system…

Soft Condensed Matter · Physics 2023-11-30 Lisa Tran , Kyle J. M. Bishop

Soft membranes are commonly employed in shape-morphing applications, where the material is programmed to achieve a target shape upon activation by an external trigger, and as coating layers that alter the surface characteristics of bulk…

Soft Condensed Matter · Physics 2016-02-05 Alessandro Lucantonio , Luciano Teresi , Antonio DeSimone

We consider a model mixture of hard colloidal spheres and non-adsorbing polymer chains in a theta solvent. The polymer component is modelled as a polydisperse mixture of effective spheres, mutually noninteracting but excluded from the…

Soft Condensed Matter · Physics 2009-11-10 A. R. Denton , M. Schmidt
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