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A large-scale relativistic configuration-interaction (CI) calculation is performed for the magnetic-dipole and the electric-quadrupole hyperfine structure splitting in ^{7,6}Li and ^9Be^+. Numerical results for the 2^2S, 3^2S, 2^2P_{1/2},…

Atomic Physics · Physics 2009-11-13 V. A. Yerokhin

In the construction of diabatic vibronic Hamiltonians for quantum dynamics in the excited-state manifold of molecules, the coupling constants are often extracted solely from information on the excited-state energies. Here, a new protocol is…

Chemical Physics · Physics 2018-04-02 Maria Fumanal , Felix Plasser , Sebastian Mai , Chantal Daniel , Etienne Gindensperger

Analytical formulas for the excitation energies as well as for the electric quadrupole reduced transition probabilities in the ground, beta and gamma bands were derived within the coherent state model for the near vibrational and well…

Nuclear Theory · Physics 2015-05-30 A. A. Raduta , R. Budaca , Amand Faessler

The hyperfine splitting of the ground state of H-, Li-, and B-like ions is investigated in details within the range of nuclear numbers Z = 7-28. The rigorous QED approach together with the large-scale configuration-interaction…

Atomic Physics · Physics 2009-11-13 A. V. Volotka , D. A. Glazov , I. I. Tupitsyn , N. S. Oreshkina , G. Plunien , V. M. Shabaev

Collisions of metastable antiprotonic helium atoms with atoms of the medium induce, among other processes, transitions between hyperfine structure (HFS) states, as well as shifts and broadening of microwave M1 spectral lines. In order to…

Nuclear Theory · Physics 2019-11-26 A. V. Bibikov , G. Ya. Korenman , S. N. Yudin

An effective Hamiltonian without symmetry restriction has been developed to model the rotational and fine structure of two nearly degenerate electronic states of an open-shell molecule. In addition to the rotational Hamiltonian for an…

Chemical Physics · Physics 2018-04-18 Jinjun Liu

We calculate accurate potential energy curves for a ground-state He$^+$ ion interacting with a He atom in the lowest-energy metastable $^3\!S$ electronic state. We employ the full configuration interaction method, equivalent to exact…

Atomic Physics · Physics 2023-11-30 Jacek Gȩbala , Michał Przybytek , Marcin Gronowski , Michał Tomza

A new approach for describing the effective electronic states of "atoms in compounds" to study the properties of molecules and condensed matter which are circumscribed by the operators heavily concentrated in atomic cores is proposed. Among…

Chemical Physics · Physics 2014-12-02 Anatoly V. Titov , Yuriy V. Lomachuk , Leonid V. Skripnikov

On the basis of quasipotential method in quantum electrodynamics we calculate corrections of order $\alpha^5$ and $\alpha^6$ to hyperfine structure of S-wave energy levels of muonic deuterium. Relativistic corrections, effects of vacuum…

High Energy Physics - Phenomenology · Physics 2014-07-30 R. N. Faustov , A. P. Martynenko , G. A. Martynenko , V. V. Sorokin

A model for photoassociation of ultracold atoms and molecules is presented, and applied to the case of $^{39}$K and $^{23}$Na$^{39}$K bosonic particles. The model relies on the assumption that photoaossociation is dominated by long-range…

Chemical Physics · Physics 2023-03-22 Baraa Shammout , Leon Karpa , Silke Ospelkaus , Eberhard Tiemann , Olivier Dulieu

Ultracold molecules with both electron spin and an electric dipole moment offer new possibilities in quantum science. We use density-functional theory to calculate hyperfine coupling constants for a selection of molecules important in this…

Atomic Physics · Physics 2018-04-25 Jesus Aldegunde , Jeremy M. Hutson

Ultracold molecules offer entirely new possibilities for the control of quantum processes due to their rich internal structure. Recently, near quantum degenerate gases of molecules have been prepared in their rovibronic ground state. For…

Atomic Physics · Physics 2015-05-14 S. Ospelkaus , K. -K. Ni , G. Quemener , B. Neyenhuis , D. Wang , M. H. G. de Miranda , J. L. Bohn , J. Ye , D. S. Jin

We use the phenomenon of electromagnetically-induced transparency in a three-level atomic system for hyperfine spectroscopy of upper states that are not directly coupled to the ground state. The three levels form a ladder system: the probe…

Optics · Physics 2007-05-23 Anusha Krishna , Kanhaiya Pandey , Ajay Wasan , Vasant Natarajan

We investigate the possibility of forming deeply bound ultracold RbCs molecules by a two-color photoassociation experiment. We compare the results with those for Rb_2 in order to understand the characteristic differences between…

Atomic Physics · Physics 2010-06-16 Subhas Ghosal , Richard J. Doyle , Christiane P. Koch , Jeremy M. Hutson

Hyperfine-structures of highly charged ions (HCIs) are favourable spectroscopic targets for exploring fundamental physics as well as nuclear properties. Recent proposals of HCI atomic clocks highlight their importance, especially for…

We report the creation of ultracold bosonic dipolar $^{23}\textrm{Na}^{39}\textrm{K}$ molecules in their absolute rovibrational ground state. Starting from weakly bound molecules immersed in an ultracold atomic mixture, we coherently…

The hyperfine structure constants of the lowest $s$ and $p_{1/2}$ states of superheavy elements Z=119 and Z= 120$^+$ are calculated using {\em ab initio} approach. Core polarization and dominating correlation effects are included to all…

Atomic Physics · Physics 2015-05-13 T. H. Dinh , V. A. Dzuba , V. V. Flambaum

We develop a model for predicting fine- and hyperfine intensities in the direct photoionization of molecules based on the separability of electron and nuclear spin states from vibrational-electronic states. Using spherical tensor algebra,…

Chemical Physics · Physics 2016-08-24 Matthias Germann , Stefan Willitsch

The purpose of this article is twofold. First, we attempt to give a brief overview of the different application areas of quantum electrodynamics (QED). These include fundamental physics (prediction of atomic energy levels), where the atom…

Atomic Physics · Physics 2014-01-17 U. D. Jentschura

We study a simple model describing superradiance in a system of two-level atoms interacting with a single-mode bosonic field. The model permits a continuous crossover between integrable and partially chaotic regimes and shows a complex…

Quantum Physics · Physics 2017-06-07 Michal Kloc , Pavel Stransky , Pavel Cejnar