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We use analytic theory and computer simulation to study patterns formed during the growth of two-component assemblies in 2D and 3D. We show that these patterns undergo a nonequilibrium phase transition, at a particular growth rate, between…

Statistical Mechanics · Physics 2014-05-12 Stephen Whitelam , Lester O. Hedges , Jeremy D. Schmit

We use computer simulation to study the layer-by-layer growth of particle structures in a lattice gas, taking the number of incorporated vacancies as a measure of the quality of the grown structure. By exploiting a dynamic scaling relation…

Statistical Mechanics · Physics 2017-08-07 Stephen Whitelam

We use simple analytic arguments and lattice-based computer simulations to study the growth of structures made from a large number of distinct component types. Components possess 'designed' interactions, chosen to stabilize an equilibrium…

Soft Condensed Matter · Physics 2014-08-25 Lester O. Hedges , Ranjan V. Mannige , Stephen Whitelam

The assembly of molecular networks into structures such as random tilings and glasses has recently been demonstrated for a number of two-dimensional systems. These structures are dynamically-arrested on experimental timescales so the…

Statistical Mechanics · Physics 2010-10-14 Andrew Stannard , Matthew O. Blunt , Peter H. Beton , Juan P. Garrahan

It is shown that a compound elastic structure, which displays a dynamic instability, may be designed as the union (or 'fusion') of two structures which are stable when separately analyzed. The compound elastic structure has two degrees of…

Classical Physics · Physics 2023-01-16 Marco Rossi , Andrea Piccolroaz , Davide Bigoni

Conserved growth models that exhibit a nonlinear instability in which the height (depth) of isolated pillars (grooves) grows in time are studied by numerical integration and stochastic simulation. When this instability is controlled by the…

Statistical Mechanics · Physics 2009-11-07 B. Chakrabarti , C. Dasgupta

Optimal growth of structures governed by spatially stochastic dynamics arises in many scientific settings, for example in processes such as solution-based crystallization and the formation of microbial biofilms on patterned substrates or…

Optimization and Control · Mathematics 2025-12-16 Maike C. de Jongh , Cristian Spitoni , Emilio N. M. Cirillo

Understanding non-equilibrium phenomena, such as growth, and connecting them to equilibrium phase behavior is a major challenge, in particular for complex multicomponent materials. We use X-ray reflectivity to determine the surface…

We comment on some recent, yet unpublished results concerning instabilities in complex systems and their applications. In particular, we briefly describe main observations during extensive computer simulations of two lattice nonequilibrium…

Statistical Mechanics · Physics 2009-11-07 J. Marro , J. M. Cortes , Pablo I. Hurtado

Theories of phase change and self-assembly often invoke the idea of a `quasiequilibrium', a regime in which the nonequilibrium association of building blocks results nonetheless in a structure whose properties are determined solely by an…

Statistical Mechanics · Physics 2013-07-22 Stephen Whitelam , Rebecca Schulman , Lester Hedges

In self-assembly processes, kinetic trapping effects often hinder the formation of thermodynamically stable ordered states. In a model of viral capsid assembly and in the phase transformation of a lattice gas, we show how simulations in a…

Biomolecules · Quantitative Biology 2015-05-28 Michael F. Hagan , Oren M. Elrad , Robert L. Jack

Alternative approach for description of the non-equilibrium phenomena arising in solids at a severe external loading is analyzed. The approach is based on the new form of kinetic equations in terms of the internal and modified free energy.…

Statistical Mechanics · Physics 2014-08-27 L. S. Metlov

For two-component assemblies, an inherent structure diagram (ISD) is the relationship between set inter-subunit energies and the types of kinetic traps (inherent structures) one may obtain from those energies. It has recently been shown…

Soft Condensed Matter · Physics 2016-01-20 Ranjan V. Mannige

We study long-range interacting systems driven by external stochastic forces that act collectively on all the particles constituting the system. Such a scenario is frequently encountered in the context of plasmas, self-gravitating systems,…

Statistical Mechanics · Physics 2013-12-03 Cesare Nardini , Shamik Gupta , Stefano Ruffo , Thierry Dauxois , Freddy Bouchet

The approach of nonequilibrium evolution thermodynamics earlier offered is developed. It helps to describe the processes of defect formation within the adiabatic approximation. The basic equations system depends on the initial defects…

Materials Science · Physics 2015-10-23 A. V. Khomenko , D. S. Troshchenko , L. S. Metlov

Numerous experimental data on the rapid solidification of binary systems exhibit the formation of metastable solid phases with the initial (nominal) chemical composition. This fact is explained by complete solute trapping leading to…

Materials Science · Physics 2009-11-13 Peter Galenko

Stochastic thermodynamics provides a useful set of tools to analyze and constrain the behavior of far from equilibrium systems. In this paper, we report an application of ideas from stochastic thermodynamics to the problem of membrane…

Soft Condensed Matter · Physics 2019-10-25 Michael Nguyen , Suriyanarayanan Vaikuntanathan

We show by numerical simulations that discretized versions of commonly studied continuum nonlinear growth equations (such as the Kardar-Parisi-Zhang equation and the Lai-Das Sarma equation) and related atomistic models of epitaxial growth…

Condensed Matter · Physics 2009-10-28 C. Dasgupta , J. M. Kim , M. Dutta , S. Das Sarma

A theory for kinetic arrest in isotropic systems of repulsive, radially-interacting particles is presented that predicts exponents for the scaling of various macroscopic quantities near the rigidity transition that are in agreement with…

Materials Science · Physics 2009-11-11 D. A. Head

The equilibrium behavior of binary mixtures can be understood through the competition of energy scales, which classifies their corresponding phase diagrams into distinct topological regimes (Types I-IV). However, in many soft-matter…

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