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Attaining accurate average structural properties in a molecular simulation should be considered a prerequisite if one aims to elicit meaningful insights into a system's behavior. For charged surfaces in contact with an electrolyte solution,…

Materials Science · Physics 2021-03-25 Thomas Sayer , Stephen J. Cox

Classical theory of the electric double layer is based on the fundamental assumption of a dilute solution of point ions. There are a number of situations such as high applied voltages, high concentration of electrolytes, systems with…

Fluid Dynamics · Physics 2015-06-11 Brian D. Storey , Martin Z. Bazant

We compute the force acting on a free, static electric charge outside a uniform dielectric sphere. We view this force as a self-interaction force, and compute it by applying the Lorentz force directly to the charge's electric field at its…

Classical Physics · Physics 2009-11-07 Lior M. Burko

Image charge effect is a fundamental problem in electrostatics. However, a proper treatment at the continuum level for many-ion systems, such as electrolyte solutions or ionic liquids, remains an open theoretical question. Here, we…

Soft Condensed Matter · Physics 2024-10-23 Tingtao Zhou , Dorian Bruch , Zhen-Gang Wang

Charged colloidal monolayers at the interface between water and air (or oil) are used in a large number of chemical, physical and biological applications. Although a considerable experimental and theoretical effort has been devoted in the…

Soft Condensed Matter · Physics 2018-12-03 Aviv Karnieli , Tomer Markovich , David Andelman

We have developed a simulation model to describe particle adsorption to and desorption from liquid interfaces. Using this model we formulate a closed interfacial equation of state for repulsive elastic spheres. The effect of a long-range…

Soft Condensed Matter · Physics 2011-02-24 Robert D. Groot , Simeon D. Stoyanov

We demonstrate that the attractive interaction measured between like-charged colloidal spheres near a wall can be accounted for by a nonequilibrium hydrodynamic effect. We present both analytical results and Brownian dynamics simulations…

Soft Condensed Matter · Physics 2009-10-31 Todd M. Squires , Michael P. Brenner

The Coulomb's formula for the force FC of electrostatic interaction between two point charges is well known. In reality, however, interactions occur not between point charges, but between charged bodies of certain geometric form, size and…

Soft Condensed Matter · Physics 2016-04-26 Kiril Kolikov

Spatially separated electron systems remain strongly coupled by electron-electron interactions even when they cannot exchange particles, provided that the layer separation d is comparable to a characteristic distance l between charge…

We study the effective forces acting between colloidal particles trapped at a fluid interface which itself is exposed to a pressure field. To this end we apply what we call the ``force approach'', which relies solely on the condition of…

Soft Condensed Matter · Physics 2008-03-31 Alvaro Dominguez , Martin Oettel , Siegfried Dietrich

Interplay of Coulomb interaction energy, free ion entropy, and conformational elasticity is a fascinating aspect in polyelectrolytes (PEs). We develop a theory for complexation of two oppositely charged PEs, a process known to be the…

Soft Condensed Matter · Physics 2022-09-15 Soumik Mitra , Arindam Kundagrami

Using an Atomic Force Microscope (AFM) we measure the interaction between two identically charged silica surfaces in the presence of saline solution. For pure NaCl the interaction is always repulsive. Upon addition of cobalt hexamine ions,…

Soft Condensed Matter · Physics 2009-11-11 Ohad Zohar , Ilya Leizerson , Uri Sivan

We consider two point-like charges in electrostatic interaction between them within the framework of a nonlinear model, associated with QED, that provides finiteness of their field energy. We find the common field of the two charges in a…

Classical Physics · Physics 2018-01-22 A. I. Breev , A. E. Shabad

Cononsolvency occurs when two miscible, competing good solvents for a polymer are mixed, resulting in a loss of solubility. In this study, we demonstrate through simulations, supported by theory, that cononsolvency can be driven solely by…

Soft Condensed Matter · Physics 2024-10-07 Hitesh Garg , Divya Nayar , Satyavani Vemparala

We consider an interaction of charged bodies under the following simplified conditions: the distribution of charge over each body is stable; the interaction of bodies is governed by electrical forces only. Physically, these assumptions can…

Mathematical Physics · Physics 2012-07-06 A. A. Kolpakov , A. G. Kolpakov

The Debye-H\" uckel formula for ionic activity coefficients is extended for concentrated solutions by solving a simple model of many-body Coulomb correlations and adding the Born solvation energy. Given the bulk permittivity, our formula is…

Chemical Physics · Physics 2017-09-12 Sven Schlumpberger , Martin Z. Bazant

Electric double layers (EDL) with counterions only, say electrons with the elementary charge $-e$, in thermal equilibrium at the inverse temperature $\beta$ are considered. In particular, we study the effect of the surface charge modulation…

Statistical Mechanics · Physics 2022-07-26 Ladislav Šamaj

This paper builds on two previous works, Lindgren et al. J. Comp. Phys. 371, 712-731 (2018) and Quan et al. arXiv:1807.05384 (2018), to devise a new method to solve the problem of calculating electrostatic interactions in a system composed…

Soft Condensed Matter · Physics 2019-02-20 Eric B. Lindgren , Chaoyu Quan , Benjamin Stamm

When two macromolecules come very near in a fluid, the surrounding molecules, having finite volume, are less likely to get in between. This leads to a pressure difference manifesting as an entropic attraction, called depletion force. Here…

Soft Condensed Matter · Physics 2020-02-26 Nathaniel Rupprecht , Dervis Can Vural

We show that a kind of displacement induced temporary electric force of a single point charge can be derived by using Maxwell stress analysis. This force comes from the variation of the charge's electric intensities that follow Coulomb's…

Classical Physics · Physics 2013-06-14 Zhixian Yu , Liang Yu
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