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We perform successive umbrella sampling grand canonical Monte Carlo computer simulations of the original ST2 model of water in the vicinity of the proposed liquid-liquid critical point, at temperatures above and below the critical…

Soft Condensed Matter · Physics 2011-08-31 Sciortino Francesco , Saika-Voivod Ivan , Poole Peter

Generative models are a promising tool to address the sampling problem in multi-body and condensed-matter systems in the framework of statistical mechanics. In this work, we show that normalizing flows can be used to learn a transformation…

Computational Physics · Physics 2022-08-23 Alessandro Coretti , Sebastian Falkner , Phillip Geissler , Christoph Dellago

A recently proposed master equation in the Lindblad form is studied with respect to covariance properties and existence of a stationary solution. The master equation describes the interaction of a test particle with a quantum fluid, the…

Quantum Physics · Physics 2009-11-07 B. Vacchini

Using the molecular dynamics simulations we investigate properties of velocity autocorrelation function of Lennard-Jones fluid at long and intermediate time scales in wide ranges of temperature and density. We show that the amplitudes of…

Soft Condensed Matter · Physics 2014-09-30 R. E. Ryltsev , N. M. Chtchelkatchev

The thermodynamic behavior of a fluid near a vapor-liquid and, hence, asymmetric critical point is discussed within a general ``complete'' scaling theory incorporating pressure mixing in the nonlinear scaling fields as well as corrections…

Statistical Mechanics · Physics 2009-11-07 Young C. Kim , Michael E. Fisher , G. Orkoulas

Dynamical properties of a Lennard-Jones binary mixture embedded in an off lattice matrix of soft spheres are studied in the direct space upon supercooling by molecular dynamics simulations. On lowering temperature the smaller particles tend…

Soft Condensed Matter · Physics 2009-11-10 P. Gallo , R. Pellarin , M. Rovere

We have developed a new and general theory of nonuniform fluids that naturally incorporates molecular scale information into the classical van der Waals theory of slowly varying interfaces. Here the theory is applied to the liquid-vapor…

Statistical Mechanics · Physics 2007-05-23 Kirill Katsov , John D. Weeks

From a minimal set made of four scale factors defined at the liquid-gas critical point of a pure fluid, and one adjustable parameter which accounts for particle quantum effects, we demonstrate here a master singular behavior of the…

Statistical Mechanics · Physics 2007-05-23 Yves Garrabos

We use molecular dynamics simulations to study the behavior of a compressible Lennard-Jones fluid in simple shear flow in a two-dimensional nanochannel. The system is equilibrated in the fluid phase close to the triple point at which gas,…

Soft Condensed Matter · Physics 2017-03-31 Madhu Priya , Yitzhak Rabin

This note examines the second virial coefficient for an imperfect gas subject to a 2n-n interparticle potential in any dimension d between 0 and n. A compact analytic expression is presented for this quantity which shows that, apart from a…

Statistical Mechanics · Physics 2016-08-31 M. Lawrence Glasser

We investigate the low temperature properties of two-dimensional Lennard-Jones glass films, prepared in silico both by liquid cooling and by physical vapor deposition. We identify deep in the solid phase a crossover temperature $T^*$, at…

Soft Condensed Matter · Physics 2018-01-30 Beatriz Seoane , Daniel R. Reid , Juan J. de Pablo , Francesco Zamponi

Wetting and drying of a rigid substrate by a Lennard-Jones fluid in molecular dynamics simulations is reported. The size of the substrate particles, being smaller than the fluid particles in former simulations, is now taken to be equal to,…

Soft Condensed Matter · Physics 2015-06-25 C. Bruin

Gravity-driven convection of fluid at parameters near its thermodynamic critical point inside a porous layer heated from below (Rayleigh-Darcy convection) is studied. The fluid having the temperature slightly above the critical one is…

Fluid Dynamics · Physics 2010-01-26 E. B. Soboleva

The liquid-vapour phase transition near a weakly attractive surface is studied by simulations of the coexistence curves of water in hydrophobic pores. There is a pronounced gradual density depletion of the liquid phase near the surface…

Statistical Mechanics · Physics 2009-11-10 I. Brovchenko , A. Geiger , A. Oleinikova

We propose a modified form of pair potential for metals. The parameters of the potential are obtained by fitting the cold curve of the potential to that obtained from the ab-initio calculations. Parameters have been obtained for Aluminum,…

Materials Science · Physics 2013-10-25 A. Sai Venkata Ramana

Metastable states in first-order phase transitions reveal interesting behavior about a wide range of systems in statistical mechanics, including spin systems, cellular automata and condensed matter systems. These metastable states are often…

Statistical Mechanics · Physics 2019-08-23 Vivianne Olguín-Arias , Sergio Davis , Gonzalo Gutiérrez

In the present paper, using a molecular dynamics simulation, we study a nature of melting of a two-dimensional ($2D$) system of classical particles interacting through a purely repulsive isotropic core-softened potential which is used for…

Soft Condensed Matter · Physics 2015-06-22 D. E. Dudalov , Yu. D. Fomin , E. N. Tsiok , V. N. Ryzhov

Previous works for a liquid suddenly contacting a gas at a supercritical pressure show the coexistence of both phases and the generation of diffusion layers on both sides of the liquid-gas interface due to thermodynamic phase equilibrium. A…

Fluid Dynamics · Physics 2022-04-25 Jordi Poblador-Ibanez , Branson Davis , William A. Sirignano

We show that a number of model liquids at fixed volume exhibit strong correlations between equilibrium fluctuations of the configurational parts of (instantaneous) pressure and energy. We present detailed results for thirteen systems,…

Soft Condensed Matter · Physics 2009-11-13 Nicholas P. Bailey , Ulf R. Pedersen , Nicoletta Gnan , Thomas B. Schrøder , Jeppe C. Dyre

A self-consistent theory of bulk electrolytes incorporating electrostatic and hard-core interactions on an equal level is applied to the two-dimensional Coulomb liquid with finite ion size. The ionic pair distributions, the structure…

Soft Condensed Matter · Physics 2026-04-10 Sahin Buyukdagli