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High resolution X-ray powder-diffraction experiments on a well-characterized polycrystalline sample of the spin liquid Tb2Ti2O7 reveal that it shows normal positive thermal-expansion above 4 K, which does not agree with the intriguing…

Strongly Correlated Electrons · Physics 2011-12-14 Kazuki Goto , Hiroshi Takatsu , Tomohiro Taniguchi , Hiroaki Kadowaki

We present here magnetization, specific heat and Raman studies on single-crystalline specimens of the first pyrochlore member $Sm_2Ti_2O_7$ of the rare-earth titanate series. Its analogous compound $Sm_2Zr_2O_7$ in the rare-earth zirconate…

Materials Science · Physics 2009-11-13 Surjeet Singh , Surajit Saha , S. K. Dhar , R. Suryanarayanan , A. K. Sood , A. Revcolevschi

Neutron scattering and magnetization measurements have been performed on the stuffed pyrochlore system Tb2+xTi2-2xNbxO7. We find that despite the introduction of chemical disorder and increasingly antiferromagnetic interactions, a spin…

Strongly Correlated Electrons · Physics 2010-02-25 B. G. Ueland , J. S. Gardner , A. J. Williams , M. L. Dahlberg , J. G. Kim , Y. Qiu , J. R. D. Copley , P. Schiffer , R. J. Cava

A new type of heavy transition metal carbide (TMC), Ru2C with a space group of p3 - m1(164) was synthesized experimentally at high pressurehigh temperature [J Phys. Condens. Matter. 2012 Sep 12; 24(36): 362202.] and it was consequently…

Materials Science · Physics 2015-06-17 Weiwei Sun , Sudip Chakraborty , Rajeev Ahuja

Recent high-throughput computational searches have predicted many novel ternary nitride compounds providing new opportunities for materials discovery in under explored phase spaces. Nevertheless, there are hardly any predictions and/or…

A comprehensive study of the structural properties of the heavily investigated rare-earth A2Ir2O7 series under extreme conditions is presented. The series is covered by studying iridates with A = Pr, Sm, Dy-Lu. Temperature- and…

Following long-standing predictions associated with hydrogen, high-temperature superconductivity has recently been observed in several hydride-based materials. Nevertheless, these high-$T_c$ phases only exist at extremely high pressures,…

We present here temperature-dependent Raman, x-ray diffraction and specific heat studies between room temperature and 12 K on single crystals of spin-ice pyrochlore compound $Dy_2Ti_2O_7$ and its non-magnetic analogue $Lu_2Ti_2O_7$. Raman…

Materials Science · Physics 2009-11-13 Surajit Saha , Surjeet Singh , B. Dkhil , S. Dhar , R. Suryanarayanan , G. Dhalenne , A. Revcolevschi , A. K. Sood

The low-pressure stabilization of superconducting hydrides with high critical temperatures ($T_c$s) remains a significant challenge, and experimentally verified superconducting hydrides are generally constrained to a limited number of…

We report synchrotron radiation diffraction and muon spin rotation (muSR) measurements on the frustrated pyrochlore magnet Tb2Ti2O7. The powder diffraction study of a crushed crystal fragment does not reveal any structural change down to 4…

Strongly Correlated Electrons · Physics 2014-12-22 P. Dalmas de Reotier , A. Yaouanc , A. Bertin , C. Marin , S. Vanishri , D. Sheptyakov , A. Cervellino , B. Roessli , C. Baines

Tl2Mn2O7 exhibits important differences with other colossal magnetoresistance (CMR) compounds, like the Mn-perovskites, in its crystal structure and electronic properties, indicating the possibility of different mechanisms for CMR being…

Strongly Correlated Electrons · Physics 2007-05-23 C. I. Ventura , M. A. Gusmao , .

The spin dynamics of geometrically frustrated pyrochlore antiferromagnets Y2Mo2O7 and Tb2Mo2O7 have been investigated using muon spin relaxation. A dramatic slowing down of the moment fluctuations occurs as one approaches the spin freezing…

Neutron powder diffraction and inelastic measurements were performed examining the 5d pyrochlore Y$_2$Ir$_2$O$_7$. Temperature dependent measurements were performed between 3.4 K and 290 K, spanning the magnetic transition at 155 K. No sign…

Strongly Correlated Electrons · Physics 2014-05-30 M. C. Shapiro , S. C. Riggs , M. B. Stone , C. R. de la Cruz , S. Chi , A. A. Podlesnyak , I. R. Fisher

Electron spin resonance study of frustrated pyrochlore Gd2Ti2O7 is performed in a wide frequency band for a temperature range 0.4-30 K, which covers paramagnetic and magnetically ordered phases. The paramagnetic resonance reveals the…

Strongly Correlated Electrons · Physics 2012-02-02 S. S. Sosin , A. I. Smirnov , L. A. Prozorova , G. Balakrishnan , M. E. Zhitomirsky

We present an experimental and theoretical study of the anisotropic pyrochlore phase diagram. Inelastic field-dependent neutron scattering on Yb$_2$Ti$_2$O$_7$ shows intrinsic broadening and a flat low-energy magnon mode which is partially…

Strongly Correlated Electrons · Physics 2025-11-20 Shang-Shun Zhang , Anish Bhardwaj , S. M. Koohpayeh , D. M. Pajerowski , Jeffrey G. Rau , Hitesh J. Changlani , Allen Scheie

Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of…

Strongly Correlated Electrons · Physics 2012-09-28 P. Dalmas de Reotier , A. Yaouanc , Y. Chapuis , S. H. Curnoe , B. Grenier , E. Ressouche , C. Marin , J. Lago , C. Baines , S. R. Giblin

In a recent letter [Phys. Rev. Lett. {\bf 82}, 1012 (1999)] it was found that the Tb$^{3+}$ magnetic moments in the Tb$_2$Ti$_2$O$_7$ pyrochlore lattice of corner-sharing tetrahedra remain in a {\it collective paramagnetic} state down to…

Disordered Systems and Neural Networks · Physics 2009-10-31 M. J. P. Gingras , B. C. den Hertog , M. Faucher , J. S. Gardner , L. J. Chang , B. D. Gaulin , N. P. Raju , J. E. Greedan

We present an interpretation of zero field diffuse neutron scattering and of high field magnetisation data at very low temperature in the frustrated pyrochlore system Tb2Ti2O7. This material has antiferromagnetic exchange interactions and…

Strongly Correlated Electrons · Physics 2013-12-16 P. Bonville , A. Gukasov , I. Mirebeau , S. Petit

Magnetic pyrochlores with non-Kramers rare-earth ions provide a platform for exploring emergent gauge physics and quantum spin-ice behavior, yet the influence of structural disorder on their ground states remains insufficiently understood.…

Geometrical frustration, as in pyrochlore lattices made of corner-sharing tetrahedra, precludes the onset of conventional magnetic ordering, enabling the stabilization of fluctuating spin states at low temperature. Disorder is a subtle…