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The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper…

Statistical Mechanics · Physics 2007-05-23 Hamid R. Molavian , Michel J. P. Gingras , Benjamin Canals

The magnetization processes of the spin-3/2 antiferromagnet LiInCr4O8 comprising a "breathing" pyrochlore lattice, which is an alternating array of small and large tetrahedra, are studied under ultrahigh magnetic fields of up to 130 T using…

A new modification of KOs2O6, the representative of a new structural type (Pearson symbol aP18, a=5.5668(1)A, b=6.4519(2)A, c=7.2356(2)A, space group P-1, no.2) was synthesized employing high pressure technique. Its structure was determined…

Superconductivity · Physics 2010-03-03 S. Katrych , Q. F. Gu , Z. Bukowski , N. D. Zhigadlo , G. Krauss , J. Karpinski

The cubic symmetry of pyrochlore iridium oxides R2Ir2O7 (R = Nd, Eu, and Pr) has been investigated by high resolution X-ray diffraction experiments down to 4 K,in order to clarify the relationship between the metal-insulator transition…

Strongly Correlated Electrons · Physics 2014-12-12 Hiroshi Takatsu , Kunihiko Watanabe , Kazuki Goto , Hiroaki Kadowaki

A combination of competing exchange interactions and substitutional disorder gives rise to magnetic inhomogeneities in the [Y$_{2-x}$Mn$_x$]MnMnMn$_4$O$_{12}$ $x = 0.23$ and $x = 0.16$ quadruple perovskite manganites. Our neutron powder…

Strongly Correlated Electrons · Physics 2023-08-16 A. M. Vibhakar , D. D. Khalyavin , P. Manuel , N. J. Steinke , L. Zhang , K. Yamaura , A. A. Belik , R. D. Johnson

We discuss the magnetic properties of a Sm$_{2}$Mo$_{2}$O$_{7}$ single crystal as investigated by means of different experimental techniques. In the literature, a conventional itinerant ferromagnetic state is reported for the Mo$^{4+}$…

Strongly Correlated Electrons · Physics 2014-08-13 G. Prando , P. Carretta , A. U. B. Wolter , R. Saint-Martin , A. Revcolevschi , B. Büchner

The recent discovery of high-temperature superconductivity in the Ruddlesden-Popper phase La3Ni2O7 under high pressure marks a significant breakthrough in the field of 3d transition-metal oxide superconductors. For an emerging novel class…

Using 170-Yb and 155-Gd Mossbauer measurements down to 0.03K, we have examined the semiconducting pyrochlore Yb2Mo2O7 where the Mo intra-sublattice interaction is anti-ferromagnetic and the metallic pyrochlore Gd2Mo2O7 where this…

Condensed Matter · Physics 2009-11-10 J. A. Hodges , P. Bonville , A. Forget , J. P. Sanchez , P. Vulliet , M. Rams , K. Krolas

Synthesis and crystal structures are described for the compounds Ln2(Ti2-xLnx)O7-x/2, where Ln = Tb, Dy, Ho, Er, Tm, Yb, Lu, and x ranges from 0 to 0.67. Rietveld refinements on X-ray powder diffraction data indicate that in Tb and Dy…

Strongly Correlated Electrons · Physics 2009-08-11 G. C. Lau , B. D. Muegge , T. M. McQueen , E. L. Duncan , R. J. Cava

Pyrochlore erbium titanate samples in the form of powders (with nominal compositions of Er2Ti2+xO7) and bulk single crystals were prepared to elucidate the effect of synthesis and growth conditions on their composition, structure, and…

Materials Science · Physics 2018-12-14 Q. Wang , A. Ghasemi , A. Scheie , S. M. Koohpayeh

The pyrochlore compound \tbti\ is known to remain in a spin-liquid state down to the lowest attainable temperature (0.05\,K), whereas current theories predict it should order into an antiferromagnetic structure. A number of models have been…

Strongly Correlated Electrons · Physics 2011-04-11 P. Bonville , I. Mirebeau , A. Gukasov , S. Petit , J. Robert

We report on the crystal structure of the quantum magnet (CuCl)LaNb2O7 that was controversially described with respect to its structural organization and magnetic behavior. Using high-resolution synchrotron powder x-ray diffraction,…

Materials Science · Physics 2015-03-17 Alexander A. Tsirlin , Artem M. Abakumov , Gustaaf Van Tendeloo , Helge Rosner

Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

Strongly Correlated Electrons · Physics 2015-03-19 Songrui Zhao. J. M. Mackie , D. E. MacLaughlin , O. O. Bernal , J. J. Ishikawa , Y. Ohta , S. Nakatsuji

The frustrated pyrochlore iridate Pr$_2$Ir$_2$O$_7$ was proposed as a metallic quantum spin liquid located at a zero-field quantum critical point. Here we present the ultralow-temperature thermal conductivity measurements on the…

Strongly Correlated Electrons · Physics 2022-08-23 J. M. Ni , Y. Y. Huang , E. J. Cheng , Y. J. Yu , B. L. Pan , Q. Li , L. M. Xu , Z. M. Tian , S. Y. Li

We have studied (Tb$_{1-x}$La$_x$)$_2$Mo$_2$O$_7$ pyrochlores by neutron diffraction and $\mu$SR at ambient and under applied pressure. Substitution of Tb for La expands the lattice and induces a change from a spin-glass like state…

Strongly Correlated Electrons · Physics 2007-05-23 A. Apetrei , I. Mirebeau , I. Goncharenko , D. Andreica , P. Bonville

Mn3TeO6 (MTO) has been experimentally found to adopt a P21/n structure under high pressure, which exhibits a significantly smaller band gap compared to the atmospheric R-3 phase. In this study, we systematically investigate the magnetism,…

Materials Science · Physics 2024-07-23 Xiao-Long Pan , Hao Wang , Lei Liu , Xiang-Rong Chen , Hua Y. Geng

Pb$_2$CoOsO$_6$ is a newly synthesized polar metal in which inversion symmetry is broken by the magnetic frustration in an antiferromagnetic ordering of Co and Os sublattices. The coupled magnetic and structural transition occurs at 45 K at…

Cd2Os2O7 crystallizes in the pyrochlore structure and undergoes a metal-insulator transition (MIT) near 226 K. We have characterized the MIT in Cd2Os2O7 using X-ray diffraction, resistivity at ambient and high pressure, specific heat,…

Strongly Correlated Electrons · Physics 2007-05-23 D. Mandrus , J. R. Thompson , R. Gaal , L. Forro , J. C. Bryan , B. C. Chakoumakos , L. M. Woods , B. C. Sales , R. S. Fishman , V. Keppens

We report inelastic neutron scattering measurements from our newly synthesized single crystals of the structurally metastable antiferromagnetic pyrochlore Yb$_{2}$Ge$_{2}$O$_{7}$. We determine the four symmetry-allowed nearest-neighbor…

The pyrochlore vanadates are compelling candidates for next-generation dissipationless devices. Lu2V2O7 and Y2V2O7 are ferromagnetic insulators (Tc ~ 70 K) that are believed to exhibit the magnon Hall effect and are expected to host…

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