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Light-manipulation of correlated electronic phases in solids offers the tantalizing prospect of realizing electronic devices operating at the ultrafast time-scale. In this context, the experimental realization of non-equilibrium transitions…

Strongly Correlated Electrons · Physics 2021-04-09 Francesco Grandi , Martin Eckstein

We present a theoretical investigation of the electronic structure of rutile (metallic) and M$_1$ and M$_2$ monoclinic (insulating) phases of VO$_2$ employing a fully self-consistent combination of density functional theory and embedded…

Strongly Correlated Electrons · Physics 2016-08-03 W. H. Brito , M. C. O. Aguiar , K. Haule , G. Kotliar

One of the early triumphs of quantum physics is the explanation why some materials are metallic whereas others are insulating. While a treatment based on single electron states correctly predicts the character of most materials this…

Strongly Correlated Electrons · Physics 2015-09-02 S. Friedemann , H. Chang , M. B. Gamża , P. Reiss , X. Chen , P. Alireza , W. A. Coniglio , D. Graf , S. Tozer , F. M. Grosche

The first-order metal-insulator transition (MIT) in paramagnetic $V_{2}O_{3}$ is studied within the ab-initio scheme LDA+DMFT, which merges the local density approximation (LDA) with dynamical mean field theory (DMFT). With a fixed value of…

Strongly Correlated Electrons · Physics 2009-11-07 M. S. Laad , L. Craco , E. Müller-Hartmann

We present a computationally efficient method to obtain the spectral function of bulk systems in the framework of steady-state density functional theory (i-DFT) using an idealized Scanning Tunneling Microscope (STM) setup. We calculate the…

Strongly Correlated Electrons · Physics 2020-11-30 David Jacob , Gianluca Stefanucci , Stefan Kurth

We study the non-equilibrium dynamics of a simple model for V2O3 that consists of a quarter-filled Hubbard model for two orbitals that are split by a weak crystal field. Peculiarities of this model are: (1) a Mott insulator whose gap…

Strongly Correlated Electrons · Physics 2015-05-05 Matteo Sandri , Michele Fabrizio

Metal-insulator transitions in clean, crystalline solids can be driven by two distinct mechanisms. In a conventional insulator, the charge carrier concentration vanishes, when an energy gap separates filled and unfilled electronic states.…

The insulating ground state of the 5d transition metal oxide CaIrO3 has been classified as a Mott-type insulator. Based on a systematic density functional theory (DFT) study with local, semilocal, and hybrid exchange-correlation…

Strongly Correlated Electrons · Physics 2015-09-04 Sun-Woo Kim , Chen Liu , Hyun-Jung Kim , Jun-Ho Lee , Yongxin Yao , Kai-Ming Ho , Jun-Hyung Cho

Frequency shifts and nuclear relaxations of 13C NMR of the metal-insulator alternating material, (Me-3,5-DIP)[Ni(dmit)2]2, are presented. The NMR absorption lines originating from metallic and insulating layers are well resolved, which…

Strongly Correlated Electrons · Physics 2009-11-13 Shigeki Fujiyama , A. Shitade , K. Kanoda , Y. Kosaka , H. M. Yamamoto , R. Kato

The (SrTiO$_3$)$_m$/(SrVO$_3$)$_n$ $d^0-d^1$ multilayer system is studied with first principles methods through the observed insulator-to-metal transition with increasing thickness of the SrVO$_3$ layer. When correlation effects with…

Strongly Correlated Electrons · Physics 2015-05-19 Victor Pardo , Warren E. Pickett

The current theoretical and experimental situations are reviewed for low-dimensional insulating systems with a low magnetic transition temperature TM and pronounced short-range magnetic order above this temperature. Both the standard and…

Strongly Correlated Electrons · Physics 2007-09-18 A A Katanin , V Yu Irkhin

Motivated by recent results of $N$th order muffin-tin orbital (NMTO) implementation of the density functional theory (DFT), we re-examine low-temperature ground-state properties of the anti-ferromagnetic insulating phase of vanadium…

Strongly Correlated Electrons · Physics 2015-05-13 N. B. Perkins , S. Di Matteo , C. R. Natoli

We study metal-insulator transitions between Mott insulators and metals. The transition mechanism completely different from the original dynamical mean field theory (DMFT) emerges from a cluster extension of it. A consistent picture…

Strongly Correlated Electrons · Physics 2007-07-18 Y. Z. Zhang , Masatoshi Imada

Density functional theory (DFT), the most widely adopted method in modern computational chemistry, fails to describe accurately the electronic structure of strongly correlated systems. Here we show that DFT can be formally and practically…

Chemical Physics · Physics 2022-04-18 Daniel Gibney , Jan-Niklas Boyn , David A. Mazziotti

The quasiparticle interferences (QPIs) of a Mott insulator are investigated using the $T$-matrix formalism implemented with the dynamical mean-field theory ($T$-DMFT). In Mott insulating state, because DMFT predicts a singularity in the…

Strongly Correlated Electrons · Physics 2015-12-07 Shantanu Mukherjee , Wei-Cheng Lee

Electronic properties of molecular conductors exhibiting antiferromagnetic (AFM) spin order and charge order (CO) owing to electron correlation are studied using first-principles density functional theory calculations. We investigate two…

Strongly Correlated Electrons · Physics 2024-11-21 Takao Tsumuraya , Tsuyoshi Miyazaki , Hitoshi Seo

Novel materials, which often exhibit surprising or even revolutionary physical properties, are necessary for critical advances in technologies. Simultaneous control of structural and physical properties via a small electrical current is of…

Strongly Correlated Electrons · Physics 2020-06-18 Gang Cao

Electronic correlations beyond static mean-field theories are of fundamental importance in describing the properties of complex materials - such as transition-metal oxides - where the low-energy physics is driven by localized d or f…

Strongly Correlated Electrons · Physics 2025-03-17 Mario Caserta , Tommaso Chiarotti , Marco Vanzini , Nicola Marzari

We study a bandwidth controlled Mott metal-insulator transition (MIT) between a Fermi liquid metal and a quantum spin-liquid insulator at half-filling in three dimensions (3D). Using a slave rotor approach, and incorporating gauge field…

Strongly Correlated Electrons · Physics 2013-05-29 Daniel Podolsky , Arun Paramekanti , Yong Baek Kim , T. Senthil

Negative differential resistance (NDR) behavior observed in several transition metal oxides is crucial for developing next-generation memory devices and neuromorphic computing systems. NbO2-based memristors exhibit two regions of NDR at…

Mesoscale and Nanoscale Physics · Physics 2024-11-12 Nitin Kumar , Jong E. Han , Karsten Beckmann , Nathaniel Cady , G. Sambandamurthy
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