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A "supercooled" liquid develops when a fluid does not crystallize upon cooling below its ordering temperature. Instead, the microscopic relaxation times diverge so rapidly that, upon further cooling, equilibration eventually becomes…

Ho2Ti2O7 and Dy2Ti2O7 spin ices exhibit elementary excitations akin to magnetic monopoles. Here we focus on Tb2Ti2O7 spin liquid, where correlated magnetic moments keep fluctuating down to very low temperatures. Using a monopole picture, we…

Strongly Correlated Electrons · Physics 2015-06-05 A. P. Sazonov , A. Gukasov , I. Mirebeau , P. Bonville

The pyrochlore material Nd$_2$Zr$_2$O$_7$ with an "all-in-all-out" (AIAO) magnetic order shows novel quantum moment fragmentation with gapped flat dynamical spin ice modes. The parameterized spin Hamiltonian with a dominant frustrated…

Materials Science · Physics 2020-03-11 J. Xu , Owen Benton , A. T. M. N. Islam , T. Guidi , G. Ehlers , B. Lake

A frustrated system is one whose symmetry precludes the possibility that every pairwise interaction (``bond'') in the system can be satisfied at the same time. Such systems are common in all areas of physical and biological science. In the…

Disordered Systems and Neural Networks · Physics 2009-11-07 Steven T. Bramwell , Michel J. -P. Gingras

The very nature of the ground state of the pyrochlore compound Yb$_2$Ti$_2$O$_7$ is much debated, as experimental results demonstrate evidence for both a disordered or a long-range ordered ground state. Indeed, the delicate balance of…

Strongly Correlated Electrons · Physics 2014-05-13 E. Lhotel , S. R. Giblin , M. R. Lees , G. Balakrishnan , L. J. Chang , Y. Yasui

Partially-ordered magnets are distinct from both spin liquids and conventional ordered magnets because order and disorder coexist in the same magnetic phase. Here, we determine the nature of partial order in the canonical frustrated…

Detailed knowledge of the phase diagram and the nature of the competing magnetic and superconducting phases is imperative for an understanding of the physics of iron-based superconductivity. Here, we show using thermodynamic probes that the…

Superconductivity · Physics 2015-08-19 A. E. Böhmer , F. Hardy , L. Wang , T. Wolf , P. Schweiss , C. Meingast

We study magnetic behaviour of the Yb$^{3+}$ ions on a frustrated pyrochlore lattice in the spinel {\CYS}. The crystal-electric field parameters deduced from high-energy inelastic neutron scattering reveal well-isolated ytterbium ground…

Strongly Correlated Electrons · Physics 2019-09-18 K. Guratinder , Jeffrey G. Rau , V. Tsurkan , C. Ritter , J. Embs , T. Fennell , H. C. Walker , M. Medarde , T. Shang , A. Cervellino , Ch. Rüegg , O. Zaharko

The pyrochlore insulator Yb2Ti2O7 has attracted the attention of experimentalists and theoreticians alike for about 15 years. Conflicting neutron diffraction data on the possible existence of magnetic Bragg reflections at low temperature…

Strongly Correlated Electrons · Physics 2016-08-26 A. Yaouanc , P. Dalmas de Reotier , L. Keller , B. Roessli , A. Forget

By many-body quantum-chemical calculations, we investigate the role of two structural effects - local ligand distortions and the anisotropic Cd-ion coordination - on the magnetic state of Cd2Os2O7, a spin S=3/2 pyrochlore. We find that…

Strongly Correlated Electrons · Physics 2013-03-28 Nikolay A. Bogdanov , Rémi Maurice , Ioannis Rousochatzakis , Jeroen van den Brink , Liviu Hozoi

The rich phase diagrams of magnetically frustrated pyrochlores have maintained a high level of interest over the past 20 years. To experimentally explore these phase diagrams requires a means of tuning the relevant interactions. One…

Strongly Correlated Electrons · Physics 2015-03-24 A. M. Hallas , A. M. Arevalo-Lopez , A. Z. Sharma , T. Munsie , J. P. Attfield , C. R. Wiebe , G. M. Luke

Ordered mechanical systems typically have one or only a few stable rest configurations, and hence are not considered useful for encoding memory. Multistable and history-dependent responses usually emerge from quenched disorder, for example…

Soft Condensed Matter · Physics 2024-05-22 Chaviva Sirote-Katz , Dor Shohat , Carl Merrigan , Yoav Lahini , Cristiano Nisoli , Yair Shokef

The pyrochlore antiferromagnet Tb2Ti2O7 has proven to be an enigma to experimentalists and theorists working on frustrated magnetic systems. The experimentally determined energy level structure suggests a local <111> Ising antiferromagnet…

Statistical Mechanics · Physics 2009-11-10 M. Enjalran , M. J. P. Gingras , Y. -J. Kao , A. Del Maestro , H. R. Molavian

The frustrated pyrochlore magnet Yb$_2$Ti$_2$O$_7$ has the remarkable property that it orders magnetically, but has no propagating magnons over wide regions of the Brillouin zone. Here we use inelastic neutron scattering to follow how the…

Strongly Correlated Electrons · Physics 2017-08-08 J. D. Thompson , P. A. McClarty , D. Prabhakaran , I. Cabrera , T. Guidi , R. Coldea

Frustration in spin system can give rise to unique ordered states and as a consequence several physical phenomena are expected such as multiferroics, high temperature superconductors and anomalous hall effect. Here we report the "new…

Strongly Correlated Electrons · Physics 2018-08-01 GiBaik Sim , SungBin Lee

We consider a system of spins on the sites of a three-dimensional pyrochlore lattice of corner-sharing tetrahedra interacting with a predominant effective $xy$ exchange. In particular, we investigate the selection of a long-range ordered…

Statistical Mechanics · Physics 2015-06-22 Behnam Javanparast , Alexander G. R. Day , Zhihao Hao , Michel J. P. Gingras

Frustrated magnets provide a platform for exploring exotic phases beyond conventional ordering, with potential relevance to functional materials and information technologies. In this work, we use Monte Carlo simulations to map the…

Strongly Correlated Electrons · Physics 2025-12-16 Prakash Timsina , Andres Chappa , Deema Alyones , Igor Vasiliev , Ludi Miao

Frustration refers to the inability to satisfy competing interactions simultaneously, often leading to a large number of degenerate ground states. This can suppress ordering tendencies, sometimes resulting in a spin liquid phase. An…

Strongly Correlated Electrons · Physics 2014-07-30 Stefan Buhrandt , Lars Fritz

We present a comprehensive experimental and theoretical study of the pyrochlore Tb$_2$Ge$_2$O$_7$, an exemplary realization of a material whose properties are dominated by competition between magnetic dipolar and electric quadrupolar…

Here we establish the systematic existence of a U(1) degeneracy of all symmetry-allowed Hamiltonians quadratic in the spins on the pyrochlore lattice, at the mean-field level. By extracting the Hamiltonian of Er2Ti2O7 from inelastic neutron…

Strongly Correlated Electrons · Physics 2013-01-08 Lucile Savary , Kate A. Ross , Bruce D. Gaulin , Jacob P. C. Ruff , Leon Balents