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We study the temperature dependence of static and dynamic responses of Coulomb interacting particles in two-dimensional traps across the thermal crossover from an amorphous solid- to liquid-like behaviors. While static correlations, that…

Disordered Systems and Neural Networks · Physics 2017-10-11 Biswarup Ash , J. Chakrabarti , Amit Ghosal

Dynamical heterogeneities in a colloidal fluid close to gelation are studied by means of computer simulations. A clear distinction between some fast particles and the rest, slow ones, is observed, yielding a picture of the gel composed by…

Soft Condensed Matter · Physics 2009-11-10 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

Using extensive molecular dynamics simulations of an equilibrium, glass-forming Lennard-Jones mixture, we characterize in detail the local atomic motions. We show that spatial correlations exist among particles undergoing extremely large…

Soft Condensed Matter · Physics 2009-10-31 C. Donati , S. C. Glotzer , P. H. Poole , W. Kob , S. J. Plimpton

We examine the phenomenon of dynamical heterogeneity in computer simulations of an equilibrium, glass-forming liquid. We describe several approaches to quantify the spatial correlation of single-particle motion, and show that spatial…

Soft Condensed Matter · Physics 2009-09-25 Sharon C. Glotzer , Claudio Donati

The slow flow of amorphous solids exhibits striking heterogeneities: swift localised particle rearrangements take place in the midst of a more or less homogeneously deforming medium. Recently, experimental as well as numerical work has…

Soft Condensed Matter · Physics 2014-03-04 Alexandre Nicolas , Joerg Rottler , Jean-Louis Barrat

We use computer simulations to explore the manner in which the particle displacements on intermediate time scales in supercooled fluids correlate to their dynamic structural environment. The fluid we study, a binary mixture of hard spheres,…

Soft Condensed Matter · Physics 2010-05-11 William P. Krekelberg , Venkat Ganesan , Thomas M. Truskett

A large-scale molecular dynamics simulation is performed on a glass-forming Lennard-Jones mixture to determine the nature of dynamical heterogeneities which arise in this model fragile liquid. We observe that the most mobile particles…

Disordered Systems and Neural Networks · Physics 2009-10-30 Claudio Donati , Jack F. Douglas , Walter Kob , Steven J. Plimpton , Peter H. Poole , Sharon C. Glotzer

We prove the emergence of spatially correlated dynamics in slowly compacting dense granular media by analyzing analytically and numerically multi-point correlation functions in a simple particle model characterized by slow non-equilibrium…

Statistical Mechanics · Physics 2009-11-10 Alexandre Lefèvre , Ludovic Berthier , Robin Stinchcombe

We comprehend the role of imperfections in materials consisting of interacting particles, arising from different origins on their universal features. Specifically, we report the static and dynamic responses in a cluster of Coulomb…

Disordered Systems and Neural Networks · Physics 2023-04-26 Prashanti Jami , Biswarup Ash , Amit Ghosal

Tracking of individual particle and studying their motion serves as a direct means to understand the dynamics in crowded and complex environments. In this study, the dynamics of tracer particles in the matrix of dense soft-colloidal…

Soft Condensed Matter · Physics 2023-06-28 Jimpaul Samukcham , Lenin S. Shagolsem

Supercooled liquids exhibit spatial heterogeneity in the dynamics of their fluctuating atomic arrangements. The length and time scales of the heterogeneous dynamics are central to the glass transition and influence nucleation and growth of…

Materials Science · Physics 2018-05-09 Pei Zhang , Jason J. Maldonis , Ze Liu , Jan Schroers , Paul M. Voyles

We define a correlation function that quantifies the spatial correlation of single-particle displacements in liquids and amorphous materials. We show for an equilibrium liquid that this function is related to fluctuations in a bulk…

Soft Condensed Matter · Physics 2009-10-31 Claudio Donati , Sharon C. Glotzer , Peter H. Poole

We present the results of a large scale molecular dynamics computer simulation study in which we investigate whether a supercooled Lennard-Jones liquid exhibits dynamical heterogeneities. We evaluate the non-Gaussian parameter for the self…

Disordered Systems and Neural Networks · Physics 2009-10-30 Walter Kob , Claudio Donati , Steven J. Plimpton , Peter H. Poole , Sharon C. Glotzer

We present experimental confirmation of dynamic facilitation in monodisperse and bidisperse colloidal suspensions near the glass transition volume fraction. Correlations in particle dynamics are seen to exist not only in space (clusters and…

Soft Condensed Matter · Physics 2014-06-24 Scott V. Franklin , Eric R. Weeks

We identify the pattern of microscopic dynamical relaxation for a two dimensional glass forming liquid. On short timescales, bursts of irreversible particle motion, called cage jumps, aggregate into clusters. On larger time scales, clusters…

Soft Condensed Matter · Physics 2010-10-04 R. Candelier , A. Widmer-Cooper , J. K. Kummerfeld , O. Dauchot , G. Biroli , P. Harrowell , D. R. Reichman

Gels in soft-matter systems are an important nonergodic state of matter. We study a colloid-polymer mixture which is quenched by increasing the polymer concentration, from a fluid to a gel. Using confocal microscopy, we study both the…

Soft Condensed Matter · Physics 2009-04-20 Takehiro Ohtsuka , C. Patrick Royall , Hajime Tanaka

Granular simulations are used to probe the particle scale dynamics at short, intermediate, and long time scales for gravity driven, dense granular flows down an inclined plane. On approach to the angle of repose, where motion ceases, the…

Soft Condensed Matter · Physics 2009-11-11 L. E. Silbert

We have studied the breakup and subsequent fluid flow in very thin films of partially wetting liquid on solid substrates, using molecular dynamics simulations. The liquid is made of short chain molecules interacting with Lennard-Jones…

Soft Condensed Matter · Physics 2009-10-31 Joel Koplik , Jayanth R. Banavar

We use a confocal microscope to examine the motion of individual particles in a dense colloidal suspension. Close to the glass transition, particle motion is strongly spatially correlated. The correlations decay exponentially with particle…

Disordered Systems and Neural Networks · Physics 2007-08-09 Eric R. Weeks , John C. Crocker , David A. Weitz

Glass-forming liquids grow dramatically sluggish upon cooling. This slowdown has long been thought to be accompanied by a growing correlation length. Characteristic dynamical and static length scales, however, have been observed to grow at…

Disordered Systems and Neural Networks · Physics 2016-08-22 Patrick Charbonneau , Ethan Dyer , Jaehoon Lee , Sho Yaida
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