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Related papers: Orbital Optimization in the Active Space Decomposi…

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We present a Gaussian-basis implementation of orbital-free density-functional theory (OF-DFT) in which the trust-region image method (TRIM) is used for optimization. This second-order optimization scheme has been constructed to provide…

Chemical Physics · Physics 2021-09-15 Matthew S. Ryley , Michael Withnall , Tom J. P. Irons , Trygve Helgaker , Andrew M. Teale

The occupation of d-orbitals controls the magnitude and anisotropy of the inter-atomic electron transfer in transition metal oxides and hence exerts a key influence on their chemical bonding and physical properties. Atomic-scale modulations…

The selection of a balanced active space is a critical step in multi-reference quantum chemistry calculations, particularly for systems with strong electron correlation. Likewise, active space selection is a key to unlock the potential of…

We present a new second order complete active space self-consistent field implementation to converge wavefunctions for both large active spaces and large atomic orbital (AO) bases. Our algorithm decouples the active space wavefunction…

Chemical Physics · Physics 2017-08-23 Qiming Sun , Jun Yang , Garnet Kin-Lic Chan

Complete active space self-consistent field (CASSCF) computations can be realized at polynomial cost via the variational optimization of the active-space two-electron reduced-density matrix (2-RDM). Like conventional approaches to CASSCF,…

Chemical Physics · Physics 2018-12-10 Mohammad Mostafanejad , A. Eugene DePrince

Fractional occupation numbers can be used in density functional theory to create a symmetric Kohn-Sham potential, resulting in orbitals with degenerate eigenvalues. We develop the corresponding perturbation theory and apply it to a system…

Materials Science · Physics 2016-09-09 Mark C. Palenik , Brett I. Dunlap

We introduce a new optimization procedure for Euclidean path integrals which compute wave functionals in conformal field theories (CFTs). We optimize the background metric in the space on which the path integration is performed.…

High Energy Physics - Theory · Physics 2017-08-30 Pawel Caputa , Nilay Kundu , Masamichi Miyaji , Tadashi Takayanagi , Kento Watanabe

We apply the Proper Orthogonal Decomposition (POD) method for the efficient simulation of several scenarios undergone by Micro-Electro-Mechanical-Systems, involving nonlinearites of geometric and electrostatic nature. The former type of…

Numerical Analysis · Mathematics 2022-02-22 Gobat G. , Opreni A. , Fresca S. , Manzoni A. , Frangi A

Hybrid density functional theory (DFT) remains intractable for large periodic systems due to the demanding computational cost of exact exchange. We apply the tensor hypercontraction (THC) (or interpolative separable density fitting)…

Computational Physics · Physics 2023-10-13 Adam Rettig , Joonho Lee , Martin Head-Gordon

The complete active space self-consistent field (CASSCF) method is the principal approach employed for studying strongly correlated systems. However, exact CASSCF can only be performed on small active spaces of ~20 electrons in ~20 orbitals…

Computational Physics · Physics 2021-12-22 Daniel S. Levine , Diptarka Hait , Norm M. Tubman , Susi Lehtola , K. Birgitta Whaley , Martin Head-Gordon

Quantum mechanical calculations of core electron binding energies (CEBEs) leading to 2p hole states are relevant to interpreting L-edge x-ray photo-electron spectroscopy (XPS), as well as higher edges. Orbital-optimized density functional…

Chemical Physics · Physics 2025-07-31 Richard Kang , Leonardo A. Cunha , Diptarka Hait , Martin Head-Gordon

We use the recently-developed Heat-bath Configuration Interaction (HCI) algorithm as an efficient active-space solver to perform multi-configuration self-consistent field calculations (HCISCF) with large active spaces. We give a detailed…

Chemical Physics · Physics 2018-11-08 James E. T. Smith , Adam A. Holmes , Bastien Mussard , Sandeep Sharma

We introduce the atomic valence active space (AVAS), a simple and well-defined automated technique for constructing active orbital spaces for use in multi-configuration and multireference (MR) electronic structure calculations. Concretely,…

Chemical Physics · Physics 2017-10-20 Elvira R. Sayfutyarova , Qiming Sun , Garnet K. -L. Chan , Gerald Knizia

A phase proper orthogonal decomposition (Phase POD) method is demonstrated, utilizing phase averaging for the decomposition of spatio-temporal behaviour of statistically non-stationary turbulent flows in an optimized manner. The proposed…

Fluid Dynamics · Physics 2024-03-01 Yisheng Zhang , Azur Hodzic , Fabien Evrard , Berend Van Wachem , Clara M. Velte

To improve the computational efficiencies of the real-space orbital-free density functional theory, this work develops a new single-grid solver by directly providing the closed-form solution to the inner iteration and using an improved…

Computational Physics · Physics 2023-05-16 Ling-Ze Bu , Wei Wang

The analytic energy gradients in the atomic orbital representation have recently been published (J. Chem. Phys. 146, 014102, 2017) within the framework of the natural orbital functional theory (NOFT). We provide here an alternative…

Chemical Physics · Physics 2018-02-19 Ion Mitxelena , Mario Piris

We introduce families of one-dimensional Lindblad equations describing open many-particle quantum systems that are exactly solvable in the following sense: $(i)$ the space of operators splits into exponentially many (in system size)…

Statistical Mechanics · Physics 2020-12-15 Fabian H. L. Essler , Lorenzo Piroli

State-specific orbital optimized approaches are more accurate at predicting core-level spectra than traditional linear-response protocols, but their utility had been restricted on account of the risk of `variational collapse' down to the…

Magnetic toroidal dipole (MTD) is one of a fundamental constituent to induce magneto-electric effects in the absence of both spatial inversion and time-reversal symmetries. We report on a microscopic investigation of the atomic-scale MTD in…

Strongly Correlated Electrons · Physics 2019-04-19 Megumi Yatsushiro , Satoru Hayami

We present a new methodology for decomposing flows with multiple transports that further extends the shifted proper orthogonal decomposition (sPOD). The sPOD tries to approximate transport-dominated flows by a sum of co-moving data fields.…

Numerical Analysis · Mathematics 2025-03-07 Philipp Krah , Arthur Marmin , Beata Zorawski , Julius Reiss , Kai Schneider