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We present an experimental study of the longitudinal electron-spin relaxation time (T1) of negatively charged nitrogen-vacancy (NV) ensembles in diamond. T1 was studied as a function of temperature from 5 to 475 K and magnetic field from 0…

Materials Science · Physics 2015-06-03 A. Jarmola , V. M. Acosta , K. Jensen , S. Chemerisov , D. Budker

We present systematic measurements of longitudinal relaxation rates ($1/T_1$) of spin polarization in the ground state of the nitrogen-vacancy (NV$^-$) color center in synthetic diamond as a function of NV$^-$ concentration and magnetic…

Quantum Physics · Physics 2015-12-17 A. Jarmola , A. Berzins , J. Smits , K. Smits , J. Prikulis , F. Gahbauer , R. Ferber , D. Erts , M. Auzinsh , D. Budker

We studied the spin depolarization of ensembles of nitrogen-vacancy (NV) centers in nitrogen-rich single crystal diamonds. We found a strong dependence of the evolution of the polarized state in the dark on the concentration of NV centers.…

Mesoscale and Nanoscale Physics · Physics 2018-07-11 R. Giri , F. Gorrini , C. Dorigoni , C. E. Avalos , M. Cazzanelli , S. Tambalo , A. Bifone

We report an experimental study of the longitudinal relaxation time ($T_1$) of the electron spin associated with single nitrogen-vacancy (NV) defects hosted in nanodiamonds (ND). We first show that $T_1$ decreases over three orders of…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 J. -P. Tetienne , T. Hingant , L. Rondin , A. Cavailles , L. Mayer , G. Dantelle , T. Gacoin , J. Wrachtrup , J. -F. Roch , V. Jacques

The negatively charged nitrogen-vacancy centre (NV$^-$) in diamond has been utilized in a wide variety of sensing applications. The centre's long spin coherence and relaxation times ($T_2^*$, $T_2$ and $T_1$) at room temperature are crucial…

We report the experimental study of the temperature-dependence of the longitudinal spin relaxation time $T_1$ of single Nitrogen-Vacancy (NV) centers hosted in nanodiamonds. To determine the relaxation mechanisms at stake, measurements of…

Mesoscale and Nanoscale Physics · Physics 2020-11-04 Timothée de Guillebon , Baptiste Vindolet , Jean-François Roch , Vincent Jacques , Loïc Rondin

We study spin relaxation and diffusion in an electron-spin ensemble of nitrogen impurities in diamond at low temperature (0.25-1.2 K) and polarizing magnetic field (80-300 mT). Measurements exploit mode- and temperature-dependent coupling…

Mesoscale and Nanoscale Physics · Physics 2013-02-13 V. Ranjan , G. de Lange , R. Schutjens , T. Debelhoir , J. P. Groen , D. Szombati , D. J. Thoen , T. M. Klapwijk , R. Hanson , L. DiCarlo

Negatively charged Nitrogen-Vacancy (NV$^-$) centers in diamond produced by ion implantation often show properties different from NVs created during the crystal growth. We observe that NVs created from nitrogen ions with four different…

We study the depolarization dynamics of a dense ensemble of dipolar interacting spins, associated with nitrogen-vacancy centers in diamond. We observe anomalously fast, density-dependent, and non-exponential spin relaxation. To explain…

Nanodiamonds (NDs) hosting nitrogen-vacancy (NV) centers are promising for applications of quantum sensing. Long spin relaxation times ($T_1$ and $T_2$) are critical for high sensitivity in quantum applications. It has been shown that…

Mesoscale and Nanoscale Physics · Physics 2020-08-11 Zaili Peng , Jax Dallas , Susumu Takahashi

We investigate nitrogen-vacancy center (NV) ensembles in diamond under the influence of strongly-correlated electron-spin baths. We thoroughly calculate the decoherence properties of the NV central spin for bath concentrations of 0.1-100…

Quantum Physics · Physics 2024-11-26 Reyhaneh Ghassemizadeh , Wolfgang Körner , Daniel F. Urban , Christian Elsässer

The application of magnetic resonance (MR) spectroscopy at progressively smaller length scales may eventually permit "chemical imaging" of spins at the surfaces of materials and biological complexes. In particular, the negatively charged…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Hai-Jing Wang , Chang S. Shin , Scott J. Seltzer , Claudia E. Avalos , Alexander Pines , Vikram S. Bajaj

We present an experimental and theoretical study of electronic spin decoherence in ensembles of nitrogen-vacancy (NV) color centers in bulk high-purity diamond at room temperature. Under appropriate conditions, we find ensemble NV spin…

Mesoscale and Nanoscale Physics · Physics 2011-01-25 P. L. Stanwix , L. M. Pham , J. R. Maze , D. Le Sage , T. K. Yeung , P. Cappellaro , P. R. Hemmer , A. Yacoby , M. D. Lukin , R. L. Walsworth

Understanding the limits to the spin-coherence of the nitrogen-vacancy (NV) center in diamond is vital to realizing the full potential of this quantum system. We show that relaxation on the $|m_{s}=-1\rangle \leftrightarrow…

Mesoscale and Nanoscale Physics · Physics 2021-02-17 M. C. Cambria , A. Gardill , Y. Li , A. Norambuena , J. R. Maze , S. Kolkowitz

Nitrogen-vacancy (NV) centers in diamond have become an important tool for quantum technologies. All of these applications rely on long coherence times of electron and nuclear spins associated with these centers. Here, we study the energy…

Quantum Physics · Physics 2020-12-02 K. Rama Koteswara Rao , Dieter Suter

We probe the relaxation dynamics of the full three-level spin system of near-surface nitrogen-vacancy (NV) centers in diamond to define a $T_{1}$ relaxation time that helps resolve the $T_{2} \leq 2T_{1}$ coherence limit of the NV's subset…

Mesoscale and Nanoscale Physics · Physics 2017-05-17 Bryan A. Myers , Amila Ariyaratne , Ania C. Bleszynski Jayich

We created dense ensembles of negatively charged nitrogen-vacancy (NV-) centers in diamond by neutron and electron irradiation for applications in hybrid quantum systems and magnetometry. We characterize fluorescence intensity, optical and…

We present a combined theoretical and experimental study of solid-state spin decoherence in an electronic spin bath, focusing specifically on ensembles of nitrogen vacancy (NV) color centers in diamond and the associated substitutional…

The nitrogen-vacancy (NV) defect in diamond is an efficient quantum sensor of randomly fluctuating signals via relaxometry measurements. In particular, the longitudinal spin relaxation of the NV defect accelerates in the presence of…

Mesoscale and Nanoscale Physics · Physics 2021-06-23 M. Rollo , A. Finco , R. Tanos , F. Fabre , T. Devolder , I. Robert-Philip , V. Jacques

We investigate the fundamental mechanism of spin phonon coupling in the negatively charged nitrogen vacancy center $(\mathrm{NV}^-)$ in diamond in order to calculate the spin lattice relaxation time $T_1$ and its temperature dependence from…

Mesoscale and Nanoscale Physics · Physics 2018-12-31 Johannes Gugler , Thomas Astner , Andreas Angerer , Jörg Schmiedmayer , Johannes Majer , Peter Mohn
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